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排序方式: 共有3370条查询结果,搜索用时 31 毫秒
21.
Y. Zhang G.R. Lumpkin H. Li M.G. Blackford M. Colella M.L. Carter E.R. Vance 《Journal of Nuclear Materials》2006,350(3):293-300
An amorphous natural brannerite sample was chosen to study the annealing of the radiation damage through thermal recrystallisation, and subsequently to evaluate the effect of radiation damage on its aqueous durability. Microstructural characterisation of the natural brannerite revealed minor alteration along the rim of the crystal and within cracks. The formation of UO2 particles and soluble Pb–Ca-rich aluminosilicate glass is responsible for the higher U and Pb releases from the recrystallised brannerite. In general, natural brannerite has been shown to be resistant to dissolution over geological time, therefore minor brannerite inclusions in ceramic formulations for immobilisation of actinide-rich radioactive wastes should not have a detrimental effect on the long-term chemical durability of the wasteforms. 相似文献
22.
Maciej Winiewski Artur Jakubiak Jan Szymanowski 《Journal of chemical technology and biotechnology (Oxford, Oxfordshire : 1986)》1995,63(3):209-214
Decyl isonicotiniate and decyl nicotiniate permit a rapid extraction of palladium(II) from its hydrochloride solutions. Decyl picoliniate is not a suitable extractant. 4-Octylphenylamine can act as a phase transfer catalyst when its concentration in the organic phase is at least 2·5 × 10?4 M . It seems that the interfacial adsorption of pyridine carboxylates and of 4-octylphenylamine is not the decisive phenomenon in palladium(II) extraction. The negligible protonation of the pyridine-type extractants and the phase transfer catalysis explains well the quick extraction of palladium(II) with the commercial and highly hydrophobic extractant ACORGA CLX-50. 相似文献
23.
本文报道了1985年鄱阳湖湖底沉积物放射性水平的调查结果。沉积物中 U、Th、~(226)Ra、~(40)(?)和~(137)Cs 的比活度分别为64.8、67.9,58.9、676.1和3.5Bq/kg;用~(137)Cs 测龄方法作了沉积物泥芯垂直深度的年代定位,由此得知1985—1958年对应深度沉积物中 U、Th、~(226)Ra 和~(40)K 的比活度与1957—1930年对应深度沉积物比较无显著性差异;U、Th 和~(226)Ra 的浓集因予分别为5.2×10~413.9×10~4和4.8×10~4L/kg。 相似文献
24.
M.M.M. El Telbany M.R. Mokhtarzadeh-Dehghan A.J. Reynolds 《Building and Environment》1985,20(1):25-32
This paper extends an earlier report of measurements and computer predictions of flows in a cubical cavity exposed on one side to the scavenging effect of an external stream. Further measurements and photographs are presented; they are consistent with each other and with the predictions of the computational model. Specifically, comparisons are made between measured and predicted mean velocities and turbulent shear stresses, and photographs are used to elucidate features of the shear layers generated by accelerating and decelerating external flows. The computer model is used to deduce approximate relations between internal turbulent activity (measured by mean velocity, turbulence energy and shear stress) and external velocity, percentage ‘window’ opening and relative position of the plane walls upstream and downstream of the cavity. 相似文献
25.
研究了浓缩235U内照射诱发人淋巴细胞白血病细胞株Molt-4细胞和巨噬细胞株Ana-1细胞的细胞调亡。估算了浓缩235U在不同阶段培养细胞中的辐射累积吸收剂量。通过电镜对免疫细胞的形态观察,发现Molt-4和Ana-1细胞在受235U内照射作用下可呈现核染质边聚,DNA链断裂和膜包裹的凋亡小体形成。对Molt-4和Ana-1细胞的DNA抽提,进行DNA琼脂糖凝胶电泳也显示出阶梯状条带形成的细胞调亡特征。从而证实了浓缩235U内照射可导致免疫细胞Molt-4和Ana-1细胞的凋亡发生。 相似文献
26.
磷酸异戊酯萃取U,Np,Pu性能的研究 总被引:1,自引:0,他引:1
测定磷酸异戊酯(TiAP)对U(Ⅵ)、Np(Ⅳ)、Np(Ⅴ)、Np(Ⅵ)、Pu(Ⅳ)和Pu(Ⅲ)的萃取性能及对Th(代替Pu)的萃取容量。研究了二乙三胺五乙酸(DTPA)络合剂对上述核素形成配合物的条件。结果表明,在用TBP和TiAP作萃取剂时,可用DTPA络合Np(Ⅵ)、Pu(Ⅲ).从而改善乏燃料后处理中U产品对Np、Pu和Pu产品对Np的去污。 相似文献
27.
未知钍—铀比的误差分析 总被引:6,自引:1,他引:5
研究了在任意Th、U含量和Th-U比覆盖整个范围(即0≤Th/U≤∝)时总α计数率对年剂量的转换因子及其误差。结果表明,当不测定Th-U比而只测量总α计数率时,最终引起的年龄误差对0≤Th/U≤∝来说为±5.1%-±8.3%,对1.1≤Th/U≤9.5来说只有±2.5%%-±4.1%。 相似文献
28.
《Calphad》2021
U–Mo and U–Nb alloys are both extensively used in nuclear industry. γ phase in U–Mo or U–Nb alloy is a solid solution, being metastable in low temperature region. In this work, the effect of alloying on stability of grain boundary in meta-stable γ phase in U–Mo and U–Nb alloys are investigate through first-principles calculations. At first, crystal structure and elastic constants of Mo, Nb and γ-U metals are calculated and the obtain results show the mechanical unstable nature of γ phase at 0 K, no matter with GGA or GGA + U treatment, which agrees with most of the theoretical results in the literature. Furthermore, from the calculated symmetric tilt grain boundary (STGB) formation energies of Σ3[110]/(111) and Σ5[001]/(310) in Mo, Nb, and γ-U, it is found that due to the mechanical unstable character of the γ-U phase, negative GB formation energy is predicted at 0 K for Σ5[001]/(310) if the STGB model is relaxed with all degrees of freedom. Therefore, by using special quasirandom structure (SQS) method, Σ5[001]/(310) and Σ3[110]/(111) STGBs with different solute concentrations in U-rich side in U–Mo and U–Nb systems are further investigated. It is found that, when alloying with Mo or Nb, unlike Σ3[110]/(111), although the fixed-atom constraint is applied, the GB formation energy of Σ5[001]/(310) STGB is becoming negative when the solute concentration is in U-rich side. Only when the concentration of Mo or Nb is larger than 27 at.% or 30 at.%, respectively, or sufficient small, the GB formation energy is becoming positive, suggesting a cooperative effects of solute concentration, unstable character, and grain size on GB structures in γ phase. The predicted different stability of alloyed GB structures at 0 K suggest that although γ phase is metastable at low temperature, its metastability can be controlled through alloying with different solutes, or with different GBs. And grain refinement should be relatively easy in U-rich part than U-poor part of the U–Mo and U–Nb systems. 相似文献
29.
Francesca Truzzi Camilla Tibaldi Anne Whittaker Silvia Dilloo Enzo Spisni Giovanni Dinelli 《International journal of molecular sciences》2021,22(1)
There is a need to assess the relationship between improved rheological properties and the immunogenic potential of wheat proteins. The present study aimed to investigate the in vitro effects of total protein extracts from three modern and two landrace Triticum aestivum commercial flour mixes, with significant differences in gluten strength (GS), on cell lines. Cytotoxicity and innate immune responses induced by wheat proteins were investigated using Caco-2 monocultures, two dimensional (2D) Caco-2/U937 co-cultures, and three dimensional (3D) co-cultures simulating the intestinal mucosa with Caco-2 epithelial cells situated above an extra-cellular matrix containing U937 monocytes and L929 fibroblasts. Modern wheat proteins, with increased GS, significantly reduced Caco-2 cell proliferation and vitality in monoculture and 2D co-cultures than landrace proteins. Modern wheat proteins also augmented Caco-2 monolayer disruption and tight junction protein, occludin, redistribution in 3D co-cultures. Release of interleukin-8 into the cell medium and increased U937 monocyte migration in both 2D and 3D co-cultures were similarly apparent. Immuno-activation of migrating U937 cells was evidenced from cluster of differentiation 14 (CD14) staining and CD11b-related differentiation into macrophages. The modern wheat proteins, with gluten polymorphism relatedness and increased GS, were shown to be more cytotoxic and immunogenic than the landrace wheat proteins. 相似文献
30.