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介绍湛江东兴炼油厂的重整装置由200kt/a扩能至300kt/a中有关催化重整反应动力学模拟计算软件的应用、反应工艺技术的改造、装置标定的情况。结合装置实际情况,采用两段装填、两段混氢技术提升了装置的技术水平。标定结果表明,改造后的装置达到了预期目的。 相似文献
25.
Burcu Selen alayan Ahmet K. Avc Z. lsen
nsan A. Erhan Aksoylu 《Applied Catalysis A: General》2005,280(2):181-188
Indirect partial oxidation (IPOX) of propane was studied over bimetallic 0.2 wt.% Pt–15 wt.% Ni/δ-Al2O3 catalyst in the 623–743 K temperature range. The unreduced and reduced forms of the catalyst were characterized by ESEM–EDAX and X-ray diffraction (XRD). In the IPOX tests, the effects of steam to carbon ratio (S/C), carbon to oxygen ratio (C/O2) and residence time (W/F (gcat h/mol HC)) on the hydrogen production activity, selectivity and product distribution were studied in detail. The effect of temperature program applied (increasing from 623 to 743 K, ITP; decreasing from 743 to 623 K, DTP) during reaction was also tested. The results showed that the Pt–Ni bimetallic system has superior performance characteristics compared to the monometallic catalysts reported in literature. The reason is thought to be the utilization of the catalyst particles as micro heat exchangers during IPOX; the heat generated by Pt sites during exothermic total oxidation (TOX) being readily transferred through the catalyst particles acting as micro heat exchangers to the Ni sites, which promote endothermic steam reforming (SR). The optimal conditions were found as S/C = 3, C/O2 = 2.70 and W/F = 0.51 gcat h/mol HC for IPOX of propane on the basis of high hydrogen productivity and selectivity between 623 and 748 K for the experimental conditions tested. The thermo-neutral points obtained showed the sustainability of reaction in terms of energy. 相似文献
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Tony Maillet Jacques Barbier Jr. Daniel Duprez 《Applied catalysis. B, Environmental》1996,9(1-4):251-266
A 1% Pd catalyst (38% dispersion) was prepared by impregnating a γ-alumina with palladium acetylacetonate dissolved in acetone. The behaviour of this catalyst in oxidation and steam reforming (SR) of propane was investigated. Temperature-programmed reactions of C3H8 with O2 or with O2 + H2O were carried out with different stoichiometric ratios S(S =[O2]/5[C3H8]). The conversion profiles of C3H8 for the reaction carried out in substoichiometry of O2 (S < 1) showed two discrete domains of conversion: oxidation at temperatures below 350°C and SR at temperatures above 350°C. The presence of steam in the inlet gases is not necessary for SR to occur: there is sufficient water produced in the oxidation to form H2 and carbon oxides by this reaction. Contrary to what was observed with Pt, an apparent deactivation between 310 and 385°C could be observed with Pd in oxidation. This is due to a reduction of PdOx into Pd0, which is much less active than the oxide in propane oxidation. Steam added to the reactants inhibits oxidation while it prevents the reduction of PdOx into Pd0. Compared to Pt and to Rh, Pd has a higher thermal resistance: no deactivation occurred after treatment up to 700°C and limited deactivation after treatment up to 900°C, provided that the catalyst is maintained in an oxygen-rich atmosphere during the cooling. 相似文献
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Kelogg合成氨工艺进展 总被引:1,自引:0,他引:1
综述了以先进合成氨工艺和转化换热系统技术为代表的Kelogg第二代合成氨工艺。较详细介绍了钌基催化剂和转化换热器 相似文献
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高发射率节能涂料及其应用 总被引:19,自引:0,他引:19
讨论了高发射率涂料节能的条件,了一种在1000℃仍保持高发射率的优质涂料,并解决了涂料与金属基体的粘结工艺,用此涂料制成增强辐射电阻带和复合炉衬,得到的新炉比旧炉节能20-40%。 相似文献
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建筑节能发展缓慢的原因及其对策 总被引:9,自引:0,他引:9
张旭 《徐州建筑职业技术学院学报》2005,5(1):55-57
我国实施建筑节能已近10年,但仍然只停留在试点、示范的层面上,尚未扩大到整体.分析了造成建筑节能发展缓慢的原因,并提出了推行和普及建筑节能的对策. 相似文献