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71.
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The idea behind this work was to acquire one dimensional lasing in the Rhodamine 6G dye doped collagen fibers with the control of random lasing phenomenon properties by changing the dye molecular arrangement. We show that a simple manipulation of the dye concentration in biopolymeric fibril matrix bulk and an additional use of α-cyclodextrin (α-CD) molecules determine formation of specific dye aggregates and as a consequence the shift of the random lasing emission wavelength in the desired direction. The analysis of the light transport mean free path in function of the dye and (α-CD) concentration was done with the use of coherent back scattering technique. 相似文献
73.
Y-α-sialon ceramics with different compositions were hot-press sintered. Varying the m or n value in theα-Sialon general formula, both the α-sialon grain morphology and phase assemblages present diversification, therefore, affecting the toughness and hardness. Meanwhile, varying the compositional parameters also influenced the composition and structure of the intergranular glass phase, as well as its oxidation behavior at 1100-1200 ℃. The oxidation of the intergranular phase Mt in the Y-α-sialon ceramics was significantly enhanced with further rising the oxidation temperature to 1300 ℃. 相似文献
74.
The effects of pH and thermal treatments on conformation and association state of Ca2+-depleted bovine α-lactalbumin (apo-α-LA) have been studied by fluorescence spectroscopy, and molecular modelling. The experimental results demonstrate a third-state model for heat-induced unfolding of apo-α-LA, at pH 2.0, and an all-or-none transition of apo-α-LA, at pH 4.5 and 7.0, respectively. The heat-induced changes in the secondary and tertiary structure of α-LA were outlined after running molecular dynamics simulations at 25 °C and 80 °C, at neutral pH, therefore supporting the experimental observations. Our data provides insight into the mechanism of pH- and heat-dependent structural changes and oligomerization of α-LA, and will be helpful in understanding the ability of this protein to interact with certain compounds of biological interest. 相似文献
75.
Oxygen homeostasis in normal and tumor cells is mediated by hypoxia-inducible factors (HIFs), which are active as heterodimer complexes, such as HIF-2α–aryl hydrocarbon receptor nuclear translocator (ARNT) and HIF-1α–ARNT. A series of mutations on the interfaces between HIF-2α and ARNT and on the domain–domain interface within HIF-2α has been reported to exert varying effects on HIF-2α–ARNT dimerization. In the present study, molecular dynamic simulations were conducted to evaluate HIF-2α mutations, namely R171A, V192D, and R171A/V192D, which are not involved in the interaction with ARNT but impede HIF-2α–ARNT dimerization. Our results indicate that these mutations induct local conformation leading to a shortened (by V192D) or widened (by R171A and R171A/V192D) Y91–E346 separation distance, where E346 and Y91 are located on the HIF-2α and interact with ARNT according to electrostatic and geometrical shape complementarity, respectively. 相似文献
76.
AbstractThe quasi-two-dimensional molecular conductor α-(BEDT-TTF)2I3 exhibits anomalous transport phenomena where the temperature dependence of resistivity is weak but the ratio of the Hall coefficient at 10 K to that at room temperature is of the order of 104. These puzzling phenomena were solved by predicting massless Dirac fermions, whose motions are described using the tilted Weyl equation with anisotropic velocity. α-(BEDT-TTF)2I3 is a unique material among several materials with Dirac fermions, i.e. graphene, bismuth, and quantum wells such as HgTe, from the view-points of both the structure and electronic states described as follows. α-(BEDT-TTF)2I3 has the layered structure with highly two-dimensional massless Dirac fermions. The anisotropic velocity and incommensurate momenta of the contact points, ±k0, originate from the inequivalency of the BEDT-TTF sites in the unit cell, where ±k0 moves in the first Brillouin zone with increasing pressure. The massless Dirac fermions exist in the presence of the charge disproportionation and are robust against the increase in pressure. The electron densities on those inequivalent BEDT-TTF sites exhibit anomalous momentum distributions, reflecting the angular dependences of the wave functions around the contact points. Those unique electronic properties affect the spatial oscillations of the electron densities in the vicinity of an impurity. A marked behavior of the Hall coefficient, where the sign of the Hall coefficient reverses sharply but continuously at low temperatures around 5 K, is investigated by treating the interband effects of the magnetic field exactly. It is shown that such behavior is possible by assuming the existence of the extremely small amount of electron doping. The enhancement of the orbital diamagnetism is also expected. The results of the present research shed light on a new aspect of Dirac fermion physics, i.e. the emergence of unique electronic properties owing to the structure of the material. 相似文献
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78.
Abstract The paper argues in favour of reasoning methods that process positional information, i.e. information about the position of the input with respect to the class prototype, and thus achieve a better specification of the corresponding output class. It is shown that such an approach leads to reducing or cancelling unwanted nonlinearities (of input-output characteristic) imposed by reasoning methods, nonlinearities that alter the dependence expressed in the knowledge base. Two methods which use positional information are presented: (a) the mapping of o-cut borders (MACB) (Stoica, 1993, Proc. Fifth IFSA World Congress, pp. 1266-1269), inspired from a particular interpretation of the representation theorem and (b) the Left/Right Centre of Gravity (L/R COG) (Ghanayem, 1995, Proc. IEA/AIE, pp. 41 -45). The methods are tested in implementing a power system stabiliser (PSS) Simulation results show better performance of methods that use positional information, as compared with classic Mamdani (Mamdani, 1975, International Journal of Man-Machine Studies, 7, 1-13) reasoning. Reflections on a “best” reasoning method conclude the paper. 相似文献
79.