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381.
382.
We demonstrate that the electrochemical properties of the electrode material can have a dramatic impact on the performance of light-emitting electrochemical cells (LECs). Specifically, we report results from planar wide-gap LECs containing a blend of poly(2-methoxy,5-(2′-ethylhexyloxy)-p-phenylene vinylene) (MEH-PPV), poly(ethylene oxide) and LiCF3SO3 as the active material. We find that Au electrodes are preferable over Al electrodes, since Au-electrode devices exhibit fast turn-on (i.e., p-n junction formation time) and clearly visible light emission during operation at 5 V and 360 K, while Al-electrode devices exhibit slow turn-on (due to a delayed onset of p-doping progression) and no visible light emission. These results are rationalized with a cyclic voltammetry study, which demonstrates that Al is oxidized at a lower potential than the p-doping (oxidation) potential of MEH-PPV, while Au is electrochemically inert over the entire voltage range spanned by the p- and n-doping potentials of MEH-PPV. Consequently, the oxidation charge injected into Al-electrode devices results in a combination of p-doping of MEH-PPV and formation of Al ions. The latter process is undesired since it results in a slow turn-on time and quenched light emission. Finally, we find that planar LECs in a bottom-electrode configuration exhibit a faster turn-on time than identical devices with the electrodes on top of the active material. 相似文献
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在深入研究文献的基础上,探讨了促进宋代印刷技术进步的主要因素:纸业兴盛品质优良,为印刷业提供了优质的承印材料;制墨技艺突飞猛进,为印刷业提供了上乘的转印介质;专业写版群体出现,提高了写版速度与印刷文字的艺术性;刻工家族已然形成,使雕刻技艺得以提高;刷印技术专人承担,进一步提高了印刷质量。 相似文献
388.
Hashimoto H Abe M Hirata A Noda Y Adachi H Yoda K 《Yeast (Chichester, England)》2002,19(16):1413-1424
The Golgi compartments of the yeast Saccharomyces cerevisiaeare dispersed within the cytoplasm, in contrast to the stacked cisternae in the mammalian cell, and consequently are observed as a punctate pattern by immunofluorescent staining of Golgi-marker proteins. The VIG4/VRG4 gene encodes the essential yeast GDP-mannose transporter, which is a polytopic membrane protein in the early and medial Golgi compartments. Upon overexpression of this gene by the aid of a strong promoter and multicopy vector, we found that stacked multivesicular structures, which resembled the cisternae of mammalian Golgi apparatus, had developed in S. cerevisiae. Immuno-electron microscopy showed that the GDP-mannose transporter was located on the stacked cisternae. Immuno-isolation and immunoblotting analyses of the vesicles showed that the overproduced GDP-mannose transporter also co-localized with the Golgi glycosyltransferases, but not with the ER- or late Golgi-marker proteins as in the control cell. We propose that the localization mechanism of the GDP-mannose transporter in the Golgi compartment would be efficient and hardly saturable, and therefore the overproduced protein induced a progression of Golgi-like compartments rather than being mislocalized in other compartments, such as the ER or a vacuole. 相似文献
389.
Audrain-McGovern Janet; Rodriguez Daniel; Tercyak Kenneth P.; Epstein Leonard H.; Goldman Paula; Wileyto E. Paul 《Canadian Metallurgical Quarterly》2004,18(1):64
Adolescents' choice to smoke may depend on substitute reinforcers for smoking, complementary activities to smoking, and individual differences in reinforcer value. The influence of these variables on smoking was determined among 983 adolescents. Substitutes were school involvement, academic performance, physical activity, and sports team participation: complements were peer smoking and substance use; delay discounting assessed individual differences in reinforcer value. Latent growth modeling indicated that substitute reinforcers reduced the odds of smoking progression almost two-fold, complementary reinforcers increased the odds by 1.14. and delay discounting indirectly influenced the odds of smoking progression through complementary reinforcers. Adolescents who smoke may have fewer reinforcers that protect against smoking and more reinforcers that promote smoking. Discounting of future rewards affects smoking through reinforcer type. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
390.
S. P. Lynch D. P. Edwards R. B. Nethercott J. L. Davidson 《Journal of Failure Analysis and Prevention》2002,2(6):50-61
Failures of various types of hydraulic couplings used to connect pipes in a naval vessel are described and used to illustrate
some of the general procedures for failure analysis. Cracking of couplings, which were manufactured from nickel-aluminum-bronze
extruded bar, occurred in both seawater and air environments. Cracks initiated at an unusually wide variety of sites and propagated
in either longitudinal or circumferential directions with respect to the axis of the couplings. Fracture surfaces were intergranular
and exhibited little or no sign of corrosion (for couplings cracked in air), and there was very limited plasticity. Macroscopic
progression markings were observed on fracture surfaces of several couplings but were not generally evident. At very high
magnifications, numerous slip lines, progression markings, and striations were observed. In a few cases, where complete separation
had occurred in service, small areas of dimpled overload fracture were observed. It was concluded from these observations,
and from comparisons of cracks produced in service with cracks produced by laboratory testing under various conditions, that
cracking had occurred by fatigue. The primary cause of failure was probably the unanticipated presence of high-frequency stress
cycles with very low amplitudes, possibly due to vibration, resonance, or acoustic waves transmitted through the hydraulic
fluid. Secondary causes of failure included the presence of high tensile residual stresses in one type of coupling, undue
stress concentrations at some of the crack-initiation sites, and overtorquing of some couplings during installation. Recommendations
on ways to prevent further failures based on these causes are discussed. 相似文献