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971.
Yue Wang Jingyi Qiu Zhongbao Yu Hai Ming Meng Li Songtong Zhang Yusheng Yang 《Ceramics International》2018,44(2):1312-1320
Surface-interface reaction between the electrode and electrolyte plays a key role in lithium-ion storage properties, especially for high voltage cathode such as LiCoPO4 and Ni-riched cathode. Generally, surface modification is an effective method to improve the electrochemical performance of electrode materials. Herein, in order to revise the LiCoPO4 cathode with desirable properties, uniform AlF3-modified LiCoPO4 (LiCoPO4@AlF3) cathode materials in nano-sized distribution are synthesized. XRD result indicates that there is no structural transformation observed after AlF3 coating. TEM characterization and XPS analysis reveal that the surface of LiCoPO4 particle is coated by a nano-sized uniform AlF3 layer. Further, the electrochemical results indicate that AlF3 layer significantly improves the cycling and rate performances of LiCoPO4 cathode within the voltage range of 3.0–5.0 V. After a series of optimization, 4 mol% AlF3-coated LiCoPO4 material exhibits the best properties including an initial discharge capacity of 159 mA h g?1 at 0.1 C with 91% capacity retention after 50 cycles, especially a discharge capacity of 90 mA h g?1 can be obtained at 1 C rate. CV curves indicate that the polarization of cathode is reduced by AlF3 layer and EIS curves reveal that AlF3 layer relieves the increase of resistance to facilitate Li-ion transfer at the interface between electrode and electrolyte during the cycling process. The enhanced electrochemical performances are attributed to that the AlF3 layer can stabilize the interface between the cathode and electrolyte, form steady SEI film and suppress the electrolyte continuous decomposition at 5 V high voltages. This feasible strategy and novel characteristics of LiCoPO4@AlF3 could promise the prospective applications in the stat-art of special lithium-ion battery with high energy and/or power density. 相似文献
972.
Yiguang Jiang Benxue Jiang Qihua Zhu Nan Jiang Pande Zhang Shuilin Chen Xu Hu Ge Zhang Jintai Fan Liangbi Su Jiang Li Long Zhang 《Journal of the European Ceramic Society》2018,38(5):2404-2409
Different deformation rates of Nd,Y-codoped CaF2 transparent ceramics were prepared by ceramization of single crystals. The deformation rate effects on the crystallization behaviors, microstructures, mechanical properties, and optical performances were investigated for the first time. The results indicate that the comprehensive performances of Nd,Y-codoped CaF2 ceramic (△a?=?62%) are the most optimal compared with other ceramics having different deformation rates (△a?=?34%, 40%, 50%, and 75%). In further investigations of the optical properties, the Nd,Y-codoped CaF2 ceramic (△a?=?62%) sample exhibited a high transparency (Ta?>?91%, 3-mm thick,250?~?1200?nm), low light scattering, superior fracture toughness (K1c?~?0.71?MPa·m1/2), strong fluorescence emission, long lifetime (τ?=?348.72?μs), and broad FWHM (29.2?nm), promising a good candidate for high-power laser material. 相似文献
973.
Perovskite oxides LaCoO_3 prepared by templating, co-precipitation and sol-gel method with different complexants were systematically characterized and its catalytic performances for CO oxidation were investigated. The samples were characterized by X-ray diffraction, thermogravimetry analysis and differential scanning calorimetry, N_2 physisorption, transmission electron microscopy, temperature program reduction of hydrogen, temperature program desorption of oxygen and X-ray photoelectron spectroscopy measurement, results of which show that the properties of LaCoO_3, such as surface morphology, surface area, surface compositions, redox capability, oxygen vacancy, as well as the calcination temperature and formation mechanism, depend intimately on the preparation method. Catalytic tests indicate that the sample prepared by carbon templating method shows the best activity for CO oxidation, with full CO conversion obtained at 135 ℃. In particular, the catalyst can be activated and significant increase of activity can be obtained with the increase of reaction time. The cyclic and longterm stability of catalysts were discussed and compared. 相似文献
974.
In this paper, we systematically summarized existing research on the driving factors of CO2 emissions and found that changes in technology gap may be one of the key driving factors of CO2 emissions. Technology efficiency, technology progress, and technology gap were decomposed by using the Meta-frontier Malmquist index (MMI), which was then combined it with the Index Decomposition Analysis (IDA) and the Production-theoretical Decomposition Analysis (PDA). Our framework was applied to Chinese provincial data from 2000 to 2016. We identified nine factors to explain changes of regional CO2 emissions. Results demonstrate that economic scale, energy technology efficiency, and output technology efficiency increased CO2 emissions in Eastern, Central, and Western regions of China, with the economic scale being the largest contributor. Energy structure, energy intensity, energy technology progress, and output technology progress decreased regional CO2 emissions, with the energy technology progress playing the strongest role. Energy technology gap and output technology gap led to an increase in CO2 emissions in Central China and, to a lesser extent, in Western China. The effects of each driving factor on CO2 emissions varied across provinces. Finally, policy implications are suggested to reduce CO2 emissions in China. 相似文献
975.
Two kinds of Cu-Al_2O_3 composites(with and without La) were prepared via mechanical alloying-spark plasma sintering(MA-SPS) method. Microstructure, mechanical properties and electrical resistivity were investigated systematically using metallography, scanning electron microscopy, transmission electron microscopy, mechanical and electrical properties testing. The results indicate that an appropriate amount of La can homogenize the distribution of Al_2O_3. As such, yield strength, ultimate tensile strength and elongation of Cu-Al_2O_3-La are greatly increased. Some semi-coherent interface between Cu and Al_2O_3 is found, which means a low interface energy. The grain shape of Cu changes to irregular band with the addition of La. This change results in a density decrease of grain boundary and reduces electrical resistance. Lanthanum may exist in the form of La_2O_3. 相似文献
976.
Yi Fang Jie Teng Xiaoqiang Ding 《Hemodialysis international. International Symposium on Home Hemodialysis》2015,19(1):2-10
China has a large population and bears a heavy burden of kidney diseases. Acute kidney injury (AKI) is increasingly prevalent in China and is associated with severe morbidity and mortality. The inadequacies of early diagnosis and management remain the major challenges to Chinese nephrologists. There is an urgent need for a nationwide, or even a global effort to increase an awareness of the devastating effects of AKI, to develop professional preventive strategies, as well as to achieve early diagnosis and early intervention. In this article, we review the increasing incidence of AKI and complexity behind prevention and management, focusing on differences in various clinical settings in China. 相似文献
977.
《新编鲁般营造正式》中详细记载了门尺法的原理和应用,分析其应用规则,以此为线索解读民间传统匠人的营造技术和营造思想。 相似文献
978.
Based on the investigation reports for two major railway accidents in China and the USA, as well as the analysis of related systems, this paper compares the differences between Chinese and American railway accident investigation modes along different dimensions. The four aspects attended to are the investigation purpose, institutional basis, scope and process, and type of conclusion. The results reveal the role of social factors in shaping the investigation pattern of engineering accidents, and show engineering accidents can serve as a window to understanding a society and the ways that learning from engineering accidents is a socially institutionalized process. A final discussion considers possible improvements that might be introduced into the Chinese mode of engineering accident investigation. 相似文献
979.
《Energy Policy》2015
Because of its resource potential and clean burning advantages, the development of shale gas can significantly increase the supply of cleaner energy while offering the associated benefits. To foster shale gas development, many policy incentives have been introduced in China. However, the current incentives have not been sufficiently aggressive, and the shale gas industry has been slow to develop. Existing policies thus need to be further improved. To provide effective support for decision makers in China, a technical and economic evaluation is performed in this study to explore the profitability of shale gas production in pilot zones. The results show that shale gas production is subeconomic under the current technical and economic conditions. Based on this evaluation, a policy analysis is conducted to investigate the profitability improvement offered by the major policies available in China to elucidate a path toward improving incentive policies. The results indicate that policy instruments related to gas prices, financial subsidies, corporate income taxes or combinations thereof could be used as priority options to improve policy incentives. Based on these results, recommendations are presented to improve the current incentive polices aimed at accelerating shale gas development. 相似文献
980.
在南海某珊瑚岛礁的工程勘察中,采用快速高效的浅层水域地震反射波勘探方法配合钻探进行联合勘察,将钻孔的“点”与物探的“线”结合起来,相互对比、佐证,进行综合解释,查明了岛礁珊瑚松散沉积物的厚度、基岩起伏形态及大范围内的连续地质剖面。勘探结果为岛礁岩土工程性状调查、水文地质调查以及工程建设提供了可靠的地质依据和设计参数,取得了理想的效果。水域地震反射波对岛礁的不同地貌单元内礁坪、向海坡、潟湖、外海的沉积层界面反映清晰,但在外礁坪区域由于现代海滩岩的发育,声波较难穿透。 相似文献