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1.
Golam Haider Krishna Sampathkumar Tim Verhagen Lukáš Nádvorník Farjana J. Sonia Václav Valeš Jan Sýkora Peter Kapusta Petr Němec Martin Hof Otakar Frank Yang-Fang Chen Jana Vejpravová Martin Kalbáč 《Advanced functional materials》2021,31(29):2102196
Recent advancements in isolation and stacking of layered van der Waals materials have created an unprecedented paradigm for demonstrating varieties of 2D quantum materials. Rationally designed van der Waals heterostructures composed of monolayer transition-metal dichalcogenides (TMDs) and few-layer hBN show several unique optoelectronic features driven by correlations. However, entangled superradiant excitonic species in such systems have not been observed before. In this report, it is demonstrated that strong suppression of phonon population at low temperature results in a formation of a coherent excitonic-dipoles ensemble in the heterostructure, and the collective oscillation of those dipoles stimulates a robust phase synchronized ultra-narrow band superradiant emission even at extremely low pumping intensity. Such emitters are in high demand for a multitude of applications, including fundamental research on many-body correlations and other state-of-the-art technologies. This timely demonstration paves the way for further exploration of ultralow-threshold quantum-emitting devices with unmatched design freedom and spectral tunability. 相似文献
2.
Lili Hou Axel Olesund Shameel Thurakkal Xiaoyan Zhang Bo Albinsson 《Advanced functional materials》2021,31(47):2106198
Developing high-performance visible-to-UV photon upconversion systems based on triplet–triplet annihilation photon upconversion (TTA-UC) is highly desired, as it provides a potential approach for UV light-induced photosynthesis and photocatalysis. However, the quantum yield and spectral range of visible-to-UV TTA-UC based on nanocrystals (NCs) are still far from satisfactory. Here, three different sized CdS NCs are systematically investigated with triplet energy transfer to four mediators and four annihilators, thus substantially expanding the available materials for visible-to-UV TTA-UC. By improving the quality of CdS NCs, introducing the mediator via a direct mixing fashion, and matching the energy levels, a high TTA-UC quantum yield of 10.4% (out of a 50% maximum) is achieved in one case, which represents a record performance in TTA-UC based on NCs without doping. In another case, TTA-UC photons approaching 4 eV are observed, which is on par with the highest energies observed in optimized organic systems. Importantly, the in-depth investigation reveals that the direct mixing approach to introduce the mediator is a key factor that leads to close to unity efficiencies of triplet energy transfer, which ultimately governs the performance of NC-based TTA-UC systems. These findings provide guidelines for the design of high-performance TTA-UC systems toward solar energy harvesting. 相似文献
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《Ceramics International》2022,48(2):1814-1819
Sr3Al2-xBxO5Cl2:Eu2+, Dy3+ (x = 0, 0.2, 0.4) long persistent phosphors were prepared via solid-state process. The pristine Sr3Al2O5Cl2:Eu2+, Dy3+ phosphor exhibits orange/red broad band emission around 609 nm, which can be attributed to the electric radiation transitions 4f65 d1→4f7 of Eu2+. Upon the same excitation, the B3+-doped Sr3Al2-xBxO5Cl2:Eu2+, Dy3+ phosphors display red-shift from 609 nm to 625 nm with increasing B3+ concentrations. The XRD patterns show that Al3+ can be replaced by B3+ in the host lattice at the tetrahedral site, which causes lattice contraction and crystal field enhancement, and thereafter achieves the red-shift on the emission spectrum. The XPS investigation provides direct evidence of the dominant 2-valent europium in the phosphor, which can be ascribed for the broad band emission of the prepared phosphors. The afterglow of all phosphors show standard double exponential decay behavior, and the afterglow of Sr3Al2O5Cl2:Eu2+, Dy3+is rather weak, while the sample co-doped with B3+shows longer and stronger afterglow, as confirmed after the curve simulation. The analysis of thermally stimulated luminescence showed that, when B3+ is introduced, a much deeper trap is created, and the density of the electron trap is also significantly increased. As a result, B3+ ions caused redshift and enhanced afterglow for the Sr3Al2-xBxO5Cl2:Eu2+, Dy3+ phosphor. 相似文献
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The fabrication and characterization of two‐photon polymerized features written within and outside of colloidal crystals is presented. Two‐photon polymerization (TPP) response diagrams are introduced and developed to map the polymerization and damage thresholds for features written via modulated beam rastering. The use of tris[4‐(7‐benzothiazol‐2‐yl‐9,9‐diethylfluoren‐2‐yl)phenyl]amine (AF‐350) as an initiator for TPP is demonstrated for the first time and TPP response diagrams illustrate the polymerization window. These diagrams also demonstrate that the polymerization behavior within and outside of colloidal crystals is similar and electron microscopy reveals nearly identical resolution. Fluorescence confocal microscopy further enables visualization of non‐self‐supporting, three‐dimensional TPP features within self‐assembled photonic crystals. Finally, microspot spectroscopy is collected from a two‐photon feature written within a colloidal crystal and this is compared with simulation. 相似文献
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Nd:碲酸盐玻璃的光谱和激光性质 总被引:2,自引:0,他引:2
对比了各种激光玻璃的光谱性质,指出碲酸盐玻璃是一咱理想的激光介质,并资产在室温下实现了钛宝石激光器泵浦了Nd:碲酸盐块体玻璃的激光发射,激光阈值4.20mJ,斜率效率14.7%。 相似文献
9.
我们于1985年对我院1984年开展肝单光子发射计算机断层以来的52例肝病人进行了分析总结。结果表明,肝单光子发射断层在诊断肝内占位性病变方面比普通肝静态γ照相有许多优点。需要指出的是,肝单光予发射断层的若干优点及诊断的准确性是与物理条件的正确选择和应用密切相关的。本文根据至今积累的近100例断层经验,从技术方面介绍了影响单 相似文献
10.
本文介绍单光子时间分辨在线谱仪系统中的多道分析器与IBM PC/XT微型计算机接口的工作原理及控制程序。 相似文献