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121.
U. Schmidhammer V. DeWaele S. Mintova E. Riedle T. Bein 《Advanced functional materials》2005,15(12):1973-1978
The ultrafast deprotonation of 2‐(2′‐hydroxyphenyl)benzothiazole (HBT) hosted in nanometer‐sized FAU and MFI zeolites is reported. Samples are prepared via in‐situ incorporation of HBT in the precursor colloidal solutions resulting in the formation of nanometer‐sized zeolites under hydrothermal treatment. The diameter of the zeolite particles formed in the crystalline suspensions is determined by dynamic light scattering and high‐resolution transmission microscopy to lie in the range 40–100 nm. It is shown that the HBT loading does not influence the degree of the zeolite crystallinity but does change the size and the morphology of the individual zeolite nanoparticles. Colloidal suspensions containing the crystalline nanoparticles are well suited for optical investigations since they are sufficiently transparent and clear. The photochemical properties of the HBT guest in the zeolite‐host systems are studied with femtosecond transient transmission spectroscopy. Depending on the acid–base properties either the enol or the keto tautomer of HBT is found to be hosted in the internal voids of the zeolites; upon UV excitation, the HBT‐keto tautomer is converted to the enol form in both MFI‐ and FAU‐type hosts. The HBT photoconversion takes place via an ultrafast deprotonation within 1.5 ps as detected by femtosecond transient absorption spectroscopy. 相似文献
122.
After considering the stabilization of a specific class of stochastic nonlinear systems in a companion paper, in this second part, we address the classical question of when is a stabilizing (in probability) controller optimal and show that for every system with a stochastic control Lyapunov function it is possible to construct a controller which is optimal with respect to a meaningful cost functional. Then we return to the problem from Part I and design an optimal backstepping controller whose cost functional includes penalty on control effort and which has an infinite gain margin. 相似文献
123.
The structure of the nonlinear H∞-filter in the neighborhood of the estimated trajectory is investigated and a bound on the size of the neighborhood that allows this structure is determined, both for finite and infinite horizons. Riccati inequalities that depend on the estimated trajectory are derived for finding the filter gain matrix and an algorithm for calculating the bound on the size of the above neighborhood is presented. Explicit formulas are obtained in the infinite horizon case for the minimum achievable disturbance attenuation level, the size of the neighborhood, and the corresponding filter gain. 相似文献
124.
Gert van der Horn Johan H. Huijsing 《Analog Integrated Circuits and Signal Processing》1997,14(3):207-222
In many applications electronic sensors are used toimprove performance and reliability of measurement systems. Suchsensors should provide a correct transfer from the physical signalto be measured to the electrical output signal. One importantstep to achieve this, is to calibrate each sensor by applyingdifferent reference input signals and adjusting the sensor transferaccordingly. Besides expensive reference equipment the calibrationprocess takes much time and attention per individual sensor,which means a considerable increase in sensor production costs.By including at the sensor or sensor interface chip a programmablecalibration facility the calibration of such smart sensors caneasily be automated and can be executed for a batch of sensorsat a time, thus minimizing the calibration time and costs. Thispaper presents a calibration method and options for integrationin the smart sensor concept, in hardware as well as in software.An advantage of the proposed method is that it does not needa large matrix of calibration data, which needs to be storedin a look-up table or converted into a correction formula, butinstead it uses a step-by-step approach to correct the sensortransfer at each calibration measurement until the error is sufficientlysmall. 相似文献
125.
126.
While information systems continue to be promoted within organizations as tools to support strategic decision-making, there is growing concern over the ability of such systems to model the social and political complexity of the situations to which they are being applied. This paper examines the nature of organizational decision-making and the use of computer-based systems to support this activity. The debate queries the extent to which such artifacts should be allowed to become enmeshed and embedded within the strategic decision-making activities of organizations which operate within increasingly complex environments. 相似文献
127.
This paper shows a few possibilities for the application of Community OR in a Third World country based on experience in Venezuela. These possibilities are discussed in a framework of the relationship between the state and community organizations. Emphasis lies in showing that Community OR in Venezuela requires a deep critical commitment to emancipation in order to help community organizations develop in a rather hostile environment. Lastly, results in dealing with community organizations in Venezuela using the Interpretive Systemology approach are presented. 相似文献
128.
129.
实现水电厂电量快速微机巡回检测,温度采集较其它信号更为困难,本文着重讨论温度信号转换及与微机系统的连接。且介绍某水电厂微机控系统中非电量检测装置的硬件结构和软件编制。 相似文献
130.
In this paper, a sensor system, called a fuzzy pulse discriminator, is developed to classify various discharge pulses in electrical discharge machining (EDM). The fuzzy rules of the pulse discriminator are obtained based on the features of the gap voltage and gap current between the tool workpiece. The membership functions of the fuzzy pulse discriminator are automatically synthesized by using genetic algorithms. The effectiveness of this approach is verified under different cutting parameters. 相似文献