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61.
Yuping Jia Xiaojuan Sun Zhiming Shi Ke Jiang Henan Liu Jianwei Ben Dabing Li 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(26)
Silicon carbide (SiC) with epitaxial graphene (EG/SiC) shows a great potential in the applications of electronic and photoelectric devices. The performance of devices is primarily dependent on the interfacial heterojunction between graphene and SiC. Here, the band structure of the EG/SiC heterojunction is experimentally investigated by Kelvin probe force microscopy. The dependence of the barrier height at the EG/SiC heterojunction to the initial surface state of SiC is revealed. Both the barrier height and band bending tendency of the heterojunction can be modulated by controlling the surface state of SiC, leading to the tuned carrier transport behavior at the EG/SiC interface. The barrier height at the EG/SiC(000‐1) interface is almost ten times that of the EG/SiC(0001) interface. As a result, the amount of carrier transport at the EG/SiC(000‐1) interface is about ten times that of the EG/SiC(0001) interface. These results offer insights into the carrier transport behavior at the EG/SiC heterojunction by controlling the initial surface state of SiC, and this strategy can be extended in all devices with graphene as the top layer. 相似文献
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Ceramic foams are made of zinc oxide using different amounts of Sb2O3 and Bi2O3 as sintering aids. The effect of a ball milling processing of the starting powders and the sintering temperature on the microstructure and the properties of the ZnO foams is investigated. The focus is set on the evolution of the secondary phases formed within the microstructure of ZnO. A determining effect is identified in the amount of an Al2O3 impurity which is introduced by abrasion of the milling vessels during ball milling. Alumina is partially dissolved in a spinel α–Zn7Sb2O12 secondary phase which is stabilized by a reduction of the unit cell volume. Remaining Al2O3 is incorporated into zinc oxide under formation of a defect wurtzite phase. The phase evolution is a complex function of the content of sintering aids, the Al2O3 impurity level and the sintering temperature. The shrinkage during sintering and the porosity evolution are correlated to the phase composition within the ZnO material. The thermal conductivity and the compressive strength of the foams are determined, normalized with respect to their porosity, and correlated to the microstructure and phase composition of the ZnO strut material. 相似文献
64.
The use a stabilized lithium structure as cathode material for batteries could be a fundamental alternative in the development of next-generation energy storage devices. However, the lithium structure severely limits battery life causes safety concerns due to the growth of lithium (Li) dendrites during rapid charge/discharge cycles. Solid electrolytes, which are used in high-density energy storage devices and avoid the instability of liquid electrolytes, can be a promising alternative for next-generation batteries. Nevertheless, poor lithium ion conductivity and structural defects at room temperature have been pointed out as limitations. In this study, through the application of a low-dimensional graphene quantum dot (GQD) layer structure, stable operation characteristics were demonstrated based on Li+ ion conductivity and excellent electrochemical performance. Moreover, the device based on the modified graphene quantum dots (GQDs) in solid state exhibited retention properties of 95.3% for 100 cycles at 0.5 C and room temperature (RT). Transmission electron microscopy analysis was performed to elucidate the Li+ ion action mechanism in the modified GQD/electrolyte heterostructure. The low-dimensional structure of the GQD-based solid electrolyte has provided an important strategy for stably-scalable solid-state lithium battery applications at room temperature. It was demonstrated that lithiated graphene quantum dots (Li-GQDs) inhibit the growth of Li dendrites by regulating the modified Li+ ion flux during charge/discharge cycling at current densities of 2.2–5.5 mA cm, acting as a modified Li diffusion heterointerface. A full Li GQD-based device was fabricated to demonstrate the practicality of the modified Li structure using the Li–GQD hetero-interface. This study indicates that the low-dimensional carbon structure in Li–GQDs can be an effective approach for stabilization of solid-state Li matrix architecture. 相似文献
65.
K. Malik F. Ahmad N. A. Yunus T. Nakato E. Mouri S. Dawood I. R. Memon 《Materialwissenschaft und Werkstofftechnik》2023,54(9):1157-1166
This research aims to develop a method for the amalgamation of graphene nanoplatelets in glass/epoxy composites. The poor interface bonding between the fiber and matrix is critical and hinders the full performance of the composites. Glass fabric and epoxy were used as reinforcement and matrix in the composite, respectively. Graphene nanoplatelets were utilized as an additional nano-materials filler for the composites. Glass/graphene/epoxy and glass/epoxy composites were fabricated via vacuum infusion molding. The new method of applying graphene nanoplatelets as secondary reinforcement in the composite was developed based on proper functionalization in the sonication process. The physical, tensile, flexural, and short beam interlaminar properties of fabricated composites were examined to analyze the method's effectiveness. The results showed that density decreased by around 5 %; however, thickness increased by around 34 % after introducing graphene nanoplatelets into the composites. The tensile strength and modulus of the composites declined by approximately 19 %, on the other hand, flexural strength and modulus increased by around 63.3 % and 8.3 %, respectively, after the addition of graphene nanoplatelets into the composites. Moreover, interlaminar shear strength of the composite was enhanced by approximately 50 %. 相似文献
66.
R. PearceAuthor Vitae T. IakimovM. AnderssonAuthor Vitae L. HultmanAuthor VitaeA. Lloyd SpetzAuthor Vitae R. YakimovaAuthor Vitae 《Sensors and actuators. B, Chemical》2011,155(2):451-455
Epitaxially grown single layer and multi layer graphene on SiC devices were fabricated and compared for response towards NO2. Due to electron donation from SiC, single layer graphene is n-type with a very low carrier concentration. The choice of substrate is demonstrated to enable tailoring of the electronic properties of graphene, with a SiC substrate realising simple resistive devices tuned for extremely sensitive NO2 detection. The gas exposed uppermost layer of the multi layer device is screened from the SiC by the intermediate layers leading to a p-type nature with a higher concentration of charge carriers and therefore, a lower gas response. The single layer graphene device is thought to undergo an n-p transition upon exposure to increasing concentrations of NO2 indicated by a change in response direction. This transition is likely to be due to the transfer of electrons to NO2 making holes the majority carriers. 相似文献
67.
There is an open discussion between those who defend mass-distributed models for humanoid robots and those in favor of simple concentrated models. Even though each of them has its advantages and disadvantages, little research has been conducted analyzing the control performance due to the mismatch between the model and the real robot, and how the simplifications affect the controller’s output. In this article we address this problem by combining a reduced model of the humanoid robot, which has an easier mathematical formulation and implementation, with a fractional order controller, which is robust to changes in the model parameters. This controller is a generalization of the well-known proportional–integral–derivative (PID) structure obtained from the application of Fractional Calculus for control, as will be discussed in this article. This control strategy guarantees the robustness of the system, minimizing the effects from the assumption that the robot has a simple mass distribution. The humanoid robot is modeled and identified as a triple inverted pendulum and, using a gain scheduling strategy, the performances of a classical PID controller and a fractional order PID controller are compared, tuning the controller parameters with a genetic algorithm. 相似文献
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