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101.
Bicrystal Si(BiSi) substrates for grain boundary (GB) Josephson junctions (GBJJs) have been fabricated by a direct bonding technique using a hot press method. The fracture strength and structure of the bonding interfaces were investigated to obtain substrates suitable for the junctions. It was found that an increase in the pressure of the hot press improves the reproducibility of the GBJJs. YBa2Cu3O7 − y GBJJs were successfully fabricated on Bi-Si substrates with a misorientation angle of 15 ° bonded under a pressure of 90 kgf cm−2 at 1200 °C in a vacuum of ≈10−3 Pa. These junctions showed typical I-V curves described by the RSJ model. The Shapiro steps induced by millimetre wave irradiation of 101 GHz were clearly observed in the I-V curves up to 3 mV, corresponding to at least 1.5 THz (, where e is the unit charge, V the voltage and h Planck's constant). 相似文献
102.
Zhenzhen Li Yutie Gong Aihua Xu Jiayu Zhao Qiong Li Lijie Dong Chuanxi Xiong Ming Jiang 《Advanced functional materials》2023,33(40):2301009
Thermo-responsive dielectric materials are in urgent demand owing to the rapid development of smart electronic/electrical systems. Although different types and structures of thermally responsive dielectric materials have been continuously reported, their dielectric response behaviors all originate from thermodynamic phase transitions. Herein, it is demonstrated that structural relaxation in poly(vinylidene fluoride) (PVDF), a non-thermodynamic phase transition, can induce a significant thermal dielectric pulse at room temperature. The dielectric pulse strength of up to 6.3 × 105 at 20 Hz, with a dielectric pulsing temperature of 24 °C, is achieved from polyethylene glycol (PEG)-PVDF coaxial nanofibrous films (PVDF@PEG), fabricated via a continuous blow spinning method. Moreover, the films exhibit excellent flexibility, adjustable strength and toughness, switchable hydrophilicity/hydrophobicity, and effective thermal management capability. The relaxation-induced dielectric pulsing effect, outstanding multifunctionality, and simple preparation combine to promote further scalability and prospects of PVDF@PEG. In particular, the work contributes to the discovery of the relaxation-induced dielectric response mechanism, which provides a new strategy for the generation of thermo-responsive dielectric materials. 相似文献
103.
Zhuoran Lv Baixin Peng Ximeng Lv Yusha Gao Keyan Hu Wujie Dong Gengfeng Zheng Fuqiang Huang 《Advanced functional materials》2023,33(16):2214370
Alloying-type metal sulfides with high theoretical capacities are promising anodes for sodium-ion batteries, but suffer from sluggish sodiation kinetics and huge volume expansion. Introducing intercalative motifs into alloying-type metal sulfides is an efficient strategy to solve the above issues. Herein, robust intercalative In S motifs are grafted to high-capacity layered Bi2S3 to form a cation-disordered (BiIn)2S3, synergistically realizing high-rate and large-capacity sodium storage. The In S motif with strong bonding serves as a space-confinement unit to buffer the volume expansion, maintaining superior structural stability. Moreover, the grafted high-metallicity Indium increases the bonding covalency of Bi S, realizing controllable reconstruction of Bi S bond during cycling to effectively prevent the migration and aggregation of atomic Bi. The novel (BiIn)2S3 anode delivers a high capacity of 537 mAh g−1 at 0.4 C and a superior high-rate stability of 247 mAh g−1 at 40 C over 10000 cycles. Further in situ and ex situ characterizations reveal the in-depth reaction mechanism and the breakage and formation of reversible Bi S bonds. The proposed space confinement and bonding covalency enhancement strategy via grafting intercalative motifs can be conducive to developing novel high-rate and large-capacity anodes. 相似文献
104.
为满足某橡胶/金属粘接结构产品的批量化检测需求,提升检测效率和自动化水平,设计开发了一套基于真空加载的激光错位散斑自动化检测系统。该系统集成了轻量化框架和紧凑型光路,并通过检测软件和检测流程优化,得到了较为理想的散斑检测图像;同时结合产品结构特点和检测灵敏度要求,设计了基于PLC控制的真空舱和运动控制装置,实现了产品粘接质量的自动化检测应用。结果表明,该系统可检测出检测试块上预置的人工缺陷,与原有手动检测模式相比,在保证检测产品检测灵敏度要求的前提下,极大地提升了检测效率,降低了检测人员的劳动强度,具有良好的工程应用价值。 相似文献
105.
纤维混凝土的韧性来源于纤维的桥接作用,而桥接作用的核心问题是纤维与水泥基体的黏结性能。为了探究纤维对混凝土的增韧机理,本文开展了不同养护龄期(0~28 d)、拔出速率(1~30 mm/min)、纤维锚固长度(10~60 mm)以及粉煤灰掺量(0~30%)下聚丙烯纤维水泥基砂浆的单根纤维拔出试验(single fiber pull-out test,SFPT),基于能量耗散原理和试验数据,建立了聚丙烯纤维水泥基砂浆韧性指数与纤维拔出过程中吸能指数的数学关系,提出了基于广义灰色关联理论的界面黏结强度影响因素计算分析方法。研究结果表明:随着养护龄期、拔出速率和纤维锚固长度的增加,聚丙烯纤维水泥基体界面黏结强度均逐渐增大,但纤维的韧性指数在养护18 h时较佳,拔出速率6 mm/min、锚固长度20 mm时最佳。当粉煤灰掺量为20%左右,纤维-水泥基体界面黏结性能最佳。并基于广义灰色关联分析法,阐明了四种因素与界面黏结强度的数学关联,研究成果可以为纤维水泥基砂浆的设计与应用提供理论支撑。 相似文献
106.
Sandwiched Thin‐Film Anode of Chemically Bonded Black Phosphorus/Graphene Hybrid for Lithium‐Ion Battery 下载免费PDF全文
Hanwen Liu Yuqin Zou Li Tao Zhaoling Ma Dongdong Liu Peng Zhou Hongbo Liu Shuangyin Wang 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(33)
A facile vacuum filtration method is applied for the first time to construct sandwich‐structure anode. Two layers of graphene stacks sandwich a composite of black phosphorus (BP), which not only protect BP from quickly degenerating but also serve as current collector instead of copper foil. The BP composite, reduced graphene oxide coated on BP via chemical bonding, is simply synthesized by solvothermal reaction at 140 °C. The sandwiched film anode used for lithium‐ion battery exhibits reversible capacities of 1401 mAh g?1 during the 200th cycle at current density of 100 mA g?1 indicating superior cycle performance. Besides, this facile vacuum filtration method may also be available for other anode material with well dispersion in N‐methyl pyrrolidone (NMP). 相似文献
107.
建立含中心半穿透圆孔的损伤金属板修补结构的三维有限元模型,以应力集中系数(Stress Concentration Factor,SCF)和挠度w作为复合材料胶接修复效果的指标,分析单向拉伸条件下,正方形补片的长度、厚度和铺层方式对修复效果的影响。结果表明:补片长度取孔直径的3.5倍、厚度取孔深度的0.6~0.8倍、铺层方式取0°/90°铺层时,复合材料单面修复含损伤裂纹板的效果较好。根据分析结果制备了实验件,进行了单向静拉伸实验,修补实验件的破坏强度比未修补实验件提高了10.1%。 相似文献
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