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91.
Xu Cai Yu Xiao Bingwen Zhang Yanhui Yang Jun Wang Huamin Chen Guozhen Shen 《Advanced functional materials》2023,33(43):2304456
MXene materials emerge as promising candidates for energy harvesting and storage application. In this study, the effect of the surface chemistry on the work function of MXenes, which determines the performance of MXene-based triboelectric nanogenerator (TENG), is elucidated. First-principles calculations reveal that the surface functional group greatly influences MXene work function: OH termination reduces the work function with respect to that of bare surface, while F and Cl increase it. Then, work functions are experimentally determined by Kelvin probe force microscopy. The MXene prepared by gentle etching at 40 °C for 48 h (GE40/48) has the largest work function. Furthermore, an electron-cloud potential-well model is established to explain the mechanism of electron emission-dominated charge transfer and assemble a triboelectric device to verify experimentally its conclusions. It is found that GE40/48 has the best performance with a 281 V open-circuit voltage, 9.7 µA short-current current, and storing 1.019 µC of charge, which is consistent with the model. Last, a patterned TENG is demonstrated for self-powered human–machine interaction application. This finding enhances the understanding of the inherent mechanism between the surface structure and the output performance of MXene-based TENG, which can be applied to other TENG based on 2D materials. 相似文献
92.
Tuning Surface Structure and Strain in Pd–Pt Core–Shell Nanocrystals for Enhanced Electrocatalytic Oxygen Reduction 下载免费PDF全文
93.
Most of the published literature on robust design is basically concerned with a single response. However, the reality is that common industrial problems usually involve several quality characteristics, which are often correlated. Traditional approaches to multidimensional quality do not offer much information on how much better or worse a process is when finding optimal settings. Köksoy and Fan [Engineering Optimization 44 (8): 935–945] pointed out that the upside-down normal loss function provides a more reasonable risk assessment to the losses of being off-target in product engineering research. However, they only consider the single-response case. This article generalizes their idea to more than one response under possible correlations and co-movement effects of responses on the process loss. The response surface methodology has been adapted, estimating the expected multivariate upside-down normal loss function of a multidimensional system to find the optimal control factor settings of a given problem. The procedure and its merits are illustrated through an example. 相似文献
94.
Yike Li Zhenhua Wu Congcan Shi Yizhuo Xu Aotian Chen Bin Su 《Advanced Engineering Materials》2023,25(20):2300703
Flush toilets waste a significant amount of water every day due to the unavoidable adhesions between human waste and the toilet surfaces. Super-slippery surfaces can repel complex fluids and various viscoelastic solids, however, are easily broken by mechanical abrasions. Herein, the fabrication of an abrasion-resistant super-slippery flush toilet (ARSFT) is reported using a selective laser sintering 3D printing technology. Unlike traditional super-slippery surfaces with limited thicknesses which can be easily worn away, the powder-sintered strategy endows the ARSFT not only with a self-supporting 3D complex shape but also with a porous structure that can accommodate considerable lubricants for an abrasion-resistant super-slippery property. As a result, the as-prepared ARSFT remains clean after contacting with various liquids such as milk, yogurt, highly sticky honey, and starch gel mixed congee, demonstrating excellent repellence to complex fluids. Besides liquids, the ARSFT exhibits a high resistance to sticky synthetic feces. Notably, even after being abraded to 1,000 cycles of abrasion using sandpaper, the ARSFT maintains its record-breaking super-slippery capability. The concept of the 3D-printed object with a superior abrasion-resistant slippery ability will improve the development of super-slippery materials and further save water consumption in the human society. 相似文献
95.
建立几何体数据文件是计算机图形显示的首要任务,本文介绍了简单几何体和不规则体的数据建立过程,并在微机上用C语言实现了这些算法. 相似文献
96.
The first measurement of a turnover rate with respect to surface intermediate concentration in a high pressure heterogeneous catalytic reaction is reported. By using infrared-visible sum frequency generation to study the hydrogenation of ethylene on Pt(111), it was found that the surface concentration of -bonded ethylene, the key reaction intermediate, represented approximately 4% of a monolayer. Thus the absolute turnover rate per surface adsorbed ethylene molecule is 25 times faster than the rate measured per platinum atom. To explain these results, we propose a model of weakly adsorbed ethylene intermediates reacting on atop sites. 相似文献
97.
Richard Lobb 《The Visual computer》1996,12(8):373-389
This paper describes a method for rounding edges and corners of arbitrary polyhedra that uses a fast approximation to convolutional filtering. The approximation defines an implicit surface, which is rendered with a specialised ray-tracing algorithm. By varying the radius of the smoothing filter, a wide range of effects can be obtained, from perfect polyhedra to blobby models. Small rounding radii give polyhedra a softer, more natural look, with edges well delineated by shadows and highlights. The rounded surfaces are much easier to specify and compute than those obtained by traditional filleting and surface-blending techniques, and are far more economical in storage. 相似文献
98.
This paper presents a whole body surface imaging system based on stereo vision technology. We have adopted a compact and economical configuration which involves only four stereo units to image the frontal and rear sides of the body. The success of the system depends on a stereo matching process that can effectively segment the body from the background in addition to recovering sufficient geometric details. For this purpose, we have developed a novel sub-pixel, dense stereo matching algorithm which includes two major phases. In the first phase, the foreground is accurately segmented with the help of a predefined virtual interface in the disparity space image, and a coarse disparity map is generated with block matching. In the second phase, local least squares matching is performed in combination with global optimization within a regularization framework, so as to ensure both accuracy and reliability. Our experimental results show that the system can realistically capture smooth and complete whole body shapes with high accuracy. 相似文献
99.
In this paper, a new multi-sensor calibration approach, called iterative registration and fusion (IRF), is presented. The key idea of this approach is to use surfaces reconstructed from multiple point clouds to enhance the registration accuracy and robustness. It calibrates the relative position and orientation of the spatial coordinate systems among multiple sensors by iteratively registering the discrete 3D sensor data against an evolving reconstructed B-spline surface, which results from the Kalman filter-based multi-sensor data fusion. Upon each registration, the sensor data gets closer to the surface. Upon fusing the newly registered sensor data with the surface, the updated surface represents the sensor data more accurately. We prove that such an iterative registration and fusion process is guaranteed to converge. We further demonstrate in experiments that the IRF can result in more accurate and more stable calibration than many classical point cloud registration methods. 相似文献
100.