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71.
Analysis of Optical Losses in a Photoelectrochemical Cell: A Tool for Precise Absorptance Estimation 下载免费PDF全文
Peter Cendula Ludmilla Steier Paolo A. Losio Michael Grätzel Jürgen O. Schumacher 《Advanced functional materials》2018,28(1)
Optical losses in a photoelectrochemical (PEC) cell account for a substantial part of solar‐to‐hydrogen conversion losses, but limited attention is paid to the detailed investigation of optical losses in PEC cells. In this work, an optical model of combined coherent and incoherent light propagation in all layers of the PEC cell based on spectroscopic measurements is presented. Specifically, photoelectrodes using transparent conductive substrates such as F:SnO2 coated with thin absorber films are focused. The optical model is verified for hematite photoanodes fabricated by atomic layer deposition and successfully used to determine wavelength‐dependent reflection, transmission, layer absorptances, and charge generation rates. Furthermore, the calculated absorptances enable 20–30% more accurate calculations of the absorbed photon‐to‐current efficiency of PEC cells. Our optical model is a powerful tool for the optimization of the optical performance of PEC cells focusing on single absorber or tandem configurations and represents a cornerstone of a complete (optical and electrical) model for PEC water splitting cells. 相似文献
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A. LaTorre L. Alonso-Nanclares S. Muelas J.M. Peña J. DeFelipe 《Expert systems with applications》2013,40(16):6521-6530
In this paper we present an algorithm to segment the nuclei of neuronal cells in confocal microscopy images, a key technical problem in many experimental studies in the field of neuroscience. We describe the whole procedure, from the original images to the segmented individual nuclei, paying particular attention to the binarization of the images, which is not straightforward due to the technical difficulties related to the visualization of nuclei as individual objects and incomplete and irregular staining. We have focused on the division of clusters of nuclei that appear frequently in these images. Thus we have developed a clump-splitting algorithm to separate touching or overlapping nuclei allowing us to accurate account for both the number and size of the nuclei. The results presented in the paper show that the proposed algorithm performs well on different sets of images from different layers of the cerebral cortex. 相似文献
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Alpesh Kumar B. V. Rathish Kumar 《International Journal for Computational Methods in Engineering Science and Mechanics》2019,20(5):451-459
AbstractIn this article, we presented a method for option pricing problem under regime-switching jump-diffusion models. We have proposed a numerical method for solving a partial integro-differential equation (PIDE) for pricing European option and for solving linear complementarity problem (LCP), to evaluate the price of American options. We use implicit explicit method for time semi discretization, followed by radial basis function based finite difference (RBF-FD) method for spatial discretization to solve PIDE. The proposed method is further extended to solve the LCP by coupling it with operator splitting method. Numerical simulation is done for European and American option to demonstrate efficiency and accuracy of the proposed method. 相似文献
76.
CuS(y)–ZnxCd1−xS (where 0.3 ≤ x ≤ 0.8, 0% ≤ y ≤ 15.8%) nanospheres with a Zn and Cu-rich surface were synthesized via a one-step method in ethylene glycol. Structural, morphological and optical properties of the samples have been investigated by XRD, TEM, XPS, ICP, N2 physisorption and UV–vis DRS techniques. The cubic phased nanospheres of approximately 20–30 nm in diameter are comprised of nanocrystals of about 5 nm. Due to the reactivity difference among the metal ions in the organic solvent, the surface of the nanospheres was found enriched with Zn and Cu sulfide layers. In the absence of Cu, sample Zn0.65Cd0.35S gives a H2 production rate of 29 μmol/h under the irradiation of a 300 W Xenon lamp with a cut-off filter (λ ≥ 420 nm) in aqueous solutions containing S2− and SO32−. The activity, which can only be increased by four times by a traditional Pt cocatalyst for the as-prepared Zn0.65Cd0.35S sample, can be enhanced by around 20 times to 550 μmol/h and 624 μmol/h after adding 5.9 mol% and 11.1 mol% (metal basis) of Cu during the synthesis to form a Cu-rich surface. It is believed that the surface Cu2+ 3d impurity levels can function as the same role of the noble metal cocatalysts as charge accommodation sites for the charge separation, and hence increase the photocatalytic performance for water splitting. 相似文献
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When Cubic Cobalt Sulfide Meets Layered Molybdenum Disulfide: A Core–Shell System Toward Synergetic Electrocatalytic Water Splitting 下载免费PDF全文
79.
Solid waste management is a serious problem over the world. Therefore, reduction, re-use and recycling of waste have become major issues in recent days. Gypsum waste plasterboard is considered one example of these waste materials. This study evaluates the use of recycled bassanite, which is derived from gypsum waste plasterboard, to enhance the performance of two types of cohesion-less soil. Recycled bassanite was utilized as a stabilizing agent to improve both compressive and splitting strengths of the tested soil. The effect of bassanite content, soil type, water content and curing time were investigated to explore the behavior of treated soil with recycled bassanite. Test results showed that increase of bassanite content is associated with increase in optimal moisture content, while no significant increase in the dry unit weight was observed. Both compressive and splitting tensile strengths enhanced with the additives of recycled bassanite. The increase of bassanite content had a more significant effect on the compressive strength compared with the effect on tensile strength. The use of recycled bassanite to enhance the strength of sandy soil had a more significant effect compared with silty soil. The effect of curing time on the strength of treated samples was more significant in early curing ages compared with late curing ages. The strength decreased significantly in case of stabilized samples prepared with water content at the wet-side of the compaction curve. However, insignificant decrease in the strength of the stabilized sample was detected with moisture content at the dry-side of compaction curve. This research meets the challenges of our society to reduce the quantities of gypsum wastes, producing useful material from waste materials that will help to a sustainable society. 相似文献
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