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141.
沈继祖 《食品与生物技术学报》1990,9(3)
本文分析了速度正反馈变带宽伺服系统特点,它在精度及快速性方面接近于再生反馈系统,但结构简单、工作可靠、调整维护方便。通过线性仿真,定量分析了系统动态指标,验证了理论设计参数合理性。通过非线性仿真,定量分析了理论分析比较困难的动态响应问题,得到了一些有益的结论。 相似文献
142.
FIR数字滤波器的递推最小二乘设计算法 总被引:24,自引:0,他引:24
本文考虑对称系数及反对称系数的FIR数字滤波器的设计问题,设计准则选为最小加权平方误差准则,并将这个设计问题看成一个线性系统的辨识问题,辨识系统参数所需的输入数据由一随机抽样法产生,辨识算法采用递推最小二乘法.按随机抽样法产生的数据具有很强的激励,保证了被辨识参数的收敛性,同时又自然地实现了最小加权平方误差准则.两个设计范例说明了本文提出的设计方法的有效性. 相似文献
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从大客量数字微波通信系统传输过程中发生的多径衰落入手,介绍了数字微波通信系统中空间分集接收机的加权评估合成技术。 相似文献
145.
Min Yan Jia‐Yan Liang Tong‐Tong Zuo Ya‐Xia Yin Sen Xin Shuang‐Jie Tan Yu‐Guo Guo Li‐Jun Wan 《Advanced functional materials》2020,30(6)
Solid polymer electrolytes (SPEs) are promising candidates for developing high‐energy‐density Li metal batteries due to their flexible processability. However, the low mechanical strength as well as the inferior interfacial regulation of ions between SPEs and Li metal anode limit the suppress ion of Li dendrites and destabilize the Li anode. To meet these challenges, interfacial engineering aiming to homogenize the distribution of Li+/electron accompanied with enhanced mechanical strength by Mg3N2 layer decorating polyethylene oxide is demonstrated. The intermediary Mg3N2 in situ transforms to a mixed ion/electron conducting interlayer consisting of a fast ionic conductor Li3N and a benign electronic conductor Mg metal, which can buffer the Li+ concentration gradient and level the nonuniform electric current distribution during cycling, as demonstrated by a COMSOL Multiphysics simulation. These characteristics endow the solid full cell with a dendrite‐free Li anode and enhanced cycling stability and kinetics. The innovative interface design will accelerate the commercial application of high‐energy‐density solid batteries. 相似文献
146.
Indranil Mondal Hyunhwa Lee Heeyoung Kim Jeong Young Park 《Advanced functional materials》2020,30(11)
Precise control of the topology of metal nanocrystals and appropriate modulation of the metal–semiconductor heterostructure is an important way to understand the relationship between structure and material properties for plasmon‐induced solar‐to‐chemical energy conversion. Here, a bottom‐up wet chemical approach to synthesize Au/Ni2P heterostructures via Pt‐catalyzed quasi‐epitaxial overgrowth of Ni on Au nanorods (NR) is presented. The structural motif of the Ni2P is controlled using the aspect ratio of the Au NR and the effective micelle concentration of the C16TAB capping agent. Highly ordered Au/Pt/Ni2P nanostructures are employed as the photoelectrocatalytic anode system for water splitting. Electrochemical and ultrafast absorption spectroscopy characterization indicates that the structural motif of the Ni2P (controlled by the outer‐shell deposition of Ni) helps to manipulate hot electron transfer during surface plasmon decay. With optimized Ni2P thickness, Pt‐tipped Au NR with an aspect ratio of 5.2 exhibits a geometric current density of 10 mA cm?2 with an overpotential of 140 mV. The photoanode displays unprecedented long‐term stability with continuous chronoamperometric performance of 50 h at an input potential of 1.5 V with over 30 days. This work provides definitive guidance for designing plasmonic–catalytic nanomaterials for enhanced solar‐to‐chemical energy conversion. 相似文献
147.
Wenshu Chen Jiajun Gu Yongping Du Fang Song Fanxing Bu Jinghan Li Yang Yuan Ruichun Luo Qinglei Liu Di Zhang 《Advanced functional materials》2020,30(25)
Large‐scale production of hydrogen from water‐alkali electrolyzers is impeded by the sluggish kinetics of hydrogen evolution reaction (HER) electrocatalysts. The hybridization of an acid‐active HER catalyst with a cocatalyst at the nanoscale helps boost HER kinetics in alkaline media. Here, it is demonstrated that 1T–MoS2 nanosheet edges (instead of basal planes) decorated by metal hydroxides form highly active / heterostructures, which significantly enhance HER performance in alkaline media. Featured with rich / sites, the fabricated 1T–MoS2 QS/Ni(OH)2 hybrid (quantum sized 1T–MoS2 sheets decorated with Ni(OH)2 via interface engineering) only requires overpotentials of 57 and 112 mV to drive HER current densities of 10 and 100 mA cm?2, respectively, and has a low Tafel slope of 30 mV dec?1 in 1 m KOH. So far, this is the best performance for MoS2‐based electrocatalysts and the 1T–MoS2 QS/Ni(OH)2 hybrid is among the best‐performing non‐Pt alkaline HER electrocatalysts known. The HER process is durable for 100 h at current densities up to 500 mA cm?2. This work not only provides an active, cost‐effective, and robust alkaline HER electrocatalyst, but also demonstrates a design strategy for preparing high‐performance catalysts based on edge‐rich 2D quantum sheets for other catalytic reactions. 相似文献
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