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911.
J.-H. SmåttAuthor VitaeM. LindénAuthor Vitae T. WagnerAuthor VitaeC.-D. KohlAuthor Vitae M. TiemannAuthor Vitae 《Sensors and actuators. B, Chemical》2011,155(2):483-488
We report the synthesis of mesoporous tin dioxide (SnO2) materials with well-defined particle morphology. The products consist of uniform spheres with a diameter of 5 μm. The spheres are hierarchically porous with two distinct pore modes of 5.0 nm and 52 nm, respectively. This special porosity is the result of a synthesis procedure which involves a ‘hard templating’ (nanocasting) process. The product forms an approximately homogeneous monolayer of spheres on a sensor substrate and shows promising response to methane gas with low cross-sensitivity to water. The structural properties and gas-sensing performance are compared with a mesoporous SnO2 material without defined morphology, prepared by a ‘soft templating’ procedure. 相似文献
912.
S. NazarpourAuthor Vitae C. López-GándaraAuthor VitaeC. ZamaniAuthor Vitae F.M. RamosAuthor VitaeAlbert CireraAuthor Vitae 《Sensors and actuators. B, Chemical》2011,155(2):489-499
Effect of sacrificial carbon on microstructure of protective layer and sensing properties of limiting current oxygen sensors were studied. Graphite and carbon nanofiber with different concentrations were examined as sacrificial layer. Therefore, several YSZ-based electrochemical gas sensors were fabricated with dissimilarity in the diffusivity of the layer covering their measuring electrodes.Gas sensors were tested as potentiometric and amperometric devices under O2-N2 mixtures, and synthetic gases similar to the exhaust gas mixtures from combustion engines. Sensors with low diffusivity (low concentration of sacrificial material) exhibit more abrupt and O2-sensitive potentiometric responses. Indeed, less O2-linear amperometric responses and higher response times are their characteristics. Sensors with high diffusion in their layers (high concentration of sacrificial material) show a less abrupt step-drop potentiometric response but a more linear O2 dependence for the amperometric response and, in general, lower response times.Results suggest that the configuration of the diffusive layer shall be controlled in terms of the expected performance of the sensor, as an amperometric or potentiometric device. The controlling parameters are discussed and given in this study. 相似文献
913.
Lexi Zhang Jianghong Zhao Haiqiang Lu Liming Gong Li Li Jianfeng Zheng Hui Li Zhenping ZhuAuthor vitae 《Sensors and actuators. B, Chemical》2011,160(1):364
Nanoparticle-assembled ZnO micro-octahedrons were synthesized by a facile homogeneous precipitation method. The ZnO micro-octahedrons are hexagonal wurtzite with high crystallinity. Abundant structure defects were confirmed on ZnO surface by photoluminescence. Gas sensors based on the ZnO micro-octahedrons exhibited high response, selectivity and stability to 1–1000 ppm formaldehyde at 400 °C. Especially, even 1 ppm formaldehyde could be detected with high response (S = 22.7). It is of interest to point out that formaldehyde could be easily distinguished from ethanol or acetaldehyde with a selectivity of about 3. The high formaldehyde response is mainly attributed to the synergistic effect of high contents of electron donor defects (Zni and VO) and highly active oxygen species (O2−) on the ZnO surface. 相似文献
914.
Jing Zhao Weinan Wang Yinping Liu Jinming Ma Xiaowei Li Yu Du Geyu Lu Author vitae 《Sensors and actuators. B, Chemical》2011,160(1):604
Ordered mesoporous SnO2 and mesoporous Pd/SnO2 have been successfully synthesized via nanocasting method using the hexagonal mesoporous SBA-15 as template. Two different procedures, impregnation technique and direct synthesis, were utilized for the doping of Pd in the mesoporous SnO2. The results of small angle X-ray diffraction (SAXD), nitrogen adsorption–desorption and transmission electron microscopy (TEM) demonstrate that the SnO2 and Pd/SnO2 display ordered mesoporous structures and high surface areas. Wide angle X-ray diffraction (WAXD) and X-ray photoelectron spectroscopy (XPS) reveal tetragonal structure of SnO2 and the existence of Pd element. The sensing properties of mesoporous SnO2 and mesoporous Pd/SnO2 for H2 were detected. The sensor utilizing mesoporous Pd/SnO2 via direct synthesis method exhibits excellent response and recovery behavior and much higher sensitivity to H2, compared to those using mesoporous SnO2 and mesoporous Pd/SnO2 via impregnation technique. It is believed that its high gas sensing performance is derived from the large surface area, high activity and well dispersion of Pd additive, as well as high porosity, which lead to highly effective surface interaction between the target gas molecules and the surface active sites. 相似文献
915.
A Chinese liquor classification method based on liquid evaporation with one unmodulated metal oxide gas sensor 总被引:1,自引:0,他引:1
Qiong Zhou Shunping Zhang Yuxiao Li Changsheng Xie Huayao Li Xiaohu DingAuthor vitae 《Sensors and actuators. B, Chemical》2011,160(1):483
Electronic nose has been widely used in the classification of liquid samples, such as vinegars, wines and liquors, which have complex components. The difficulty of these classifications is how to get the information of the trace components in these samples. In this paper a method for liquor recognition based on liquid evaporation was presented. This method makes use of the distinct evaporation characteristics of different components in liquor samples. And during the evaporation process, one metal oxide gas sensor was used to detect the headspace of liquor samples for classification. Due to the distinct evaporation characteristics of different components, volatile compounds in the headspace evaporating from samples would change with the testing time. Meanwhile, the gas sensor would respond to these volatile compounds. Accordingly, more information of liquor samples during evaporation may be acquired with the proposed method. To verify the performance of this method, 8 different Chinese liquors with 50% alcohol for comparison were tested under the method. The results showed that the evaporation characteristics of these liquor samples were quite distinct. The correct classification accuracy of discriminant function analysis was 100%, which indicated this method may be a simple and effective way for complex-component liquid sample analysis. 相似文献
916.
Jichao ShiAuthor VitaeGujin HuAuthor Vitae Yan SunAuthor VitaeMing GengAuthor Vitae Jie WuAuthor VitaeYufeng LiuAuthor Vitae Meiying GeAuthor VitaeJunchao TaoAuthor Vitae Meng CaoAuthor VitaeNing DaiAuthor Vitae 《Sensors and actuators. B, Chemical》2011,156(2):820-824
WO3 nanocrystals have been prepared by a sol-gel route and characterized by X-ray diffractometry, scanning electron microscopy, and transmission electron microscopy. The experimental results show that WO3 nanocrystals have a high crystallographic quality and a good dispersivity. The particles’ sizes are in the range of 25-100 nm. The fabricated WO3 nanocrystal-based sensors have an excellent sensitivity and selectivity to acetone, and display a rapid response and recovery characteristics. The developed sensors exhibit a detection limit down to 0.05 ppm at 300 °C, rendering a promising application in noninvasive diagnosis of diabetes. The response mechanism of the WO3 nanocrystal sensor to low concentration of acetone has been discussed based on the depletion layer model. 相似文献
917.
K.O. RochaAuthor VitaeS.M. ZanettiAuthor Vitae 《Sensors and actuators. B, Chemical》2011,157(2):654-661
Nanocrystalline WO3/TiO2-based powders have been prepared by the high energy activation method with WO3 concentration ranging from 1 to 10 mol%. The samples were thermal treated in a microwave oven at 600 °C for 20 min and their structural and micro-structural characteristics were evaluated by X-ray diffraction, Raman spectroscopy, EXAFS measurements at the Ti K-edge, and transmission electron microscopy. Nitrogen adsorption isotherms and H2 Temperature Programmed Reduction were also carried out for physical characterization. The crystallite and particle mean sizes ranged from 30 to 40 nm and from 100 to 190 nm, respectively. Good sensor response was obtained for samples with at least 5 mol% WO3 activated for at least 80 min. Ceramics heat-treated in microwave oven for 20 min have shown similar sensor response as those prepared in conventional oven for 120 min, which is highly cost effective. These results indicate that WO3/TiO2 ceramics can be used as a humidity sensor element. 相似文献
918.
F. Aiello F.L. Bellifemine G. Fortino S. Galzarano R. Gravina 《Engineering Applications of Artificial Intelligence》2011,24(7):1147-1161
Nowadays wireless body sensor networks (WBSNs) have great potential to enable a broad variety of assisted living applications such as human biophysical/biochemical control and activity monitoring for health care, e-fitness, emergency detection, emotional recognition for social networking, security, and highly interactive games. It is therefore important to define design methodologies and programming frameworks which enable rapid prototyping of WBSN applications. Several effective application development frameworks have been already proposed for WBSNs designed for TinyOS-based sensor platforms, e.g. CodeBlue, SPINE, and Titan. In this paper we present an application of MAPS, an agent framework for wireless sensor networks based on the Java-programmable Sun SPOT sensor platform, for the development of a real-time WBSN-based system for human activity monitoring. The agent-oriented programming abstractions provided by MAPS allow effective and rapid prototyping of the sensor-side software. In particular, the architecture of the developed system is a typical star-based WBSN composed of a coordinator node and two sensor nodes located respectively on the waist and the thigh of the monitored assisted living. The coordinator relies on a JADE-based enhancement of the SPINE coordinator and allows configuring sensors, receiving their data, and recognizing pre-defined human activities. On the other hand, each sensor node runs a MAPS-based agent that performs sensing of the 3-axial accelerometer sensor, computation of significant features on the acquired data, feature aggregation and transmission to the coordinator. The experimentation phase of the prototype, which allows evaluating the obtainable monitoring performances and activity recognition accuracy, is described. Moreover, a comparison of the monitoring system based on MAPS, AFME and SPINE in terms of programming effectiveness and system performances is discussed. 相似文献
919.
针对无线传感器网络节点负载不均衡的问题,提出了一种应用相对变换的无线传感器网络分簇算法(RTCH)。在成簇阶段,节点将簇头剩余能量、簇头与节点和簇头与基站的传输能耗等参数利用该模型先进行相对变换,再计算簇头适宜度来选择加入簇头成簇,并通过簇头的反馈信息来控制簇的规模来优化网络性能。仿真实验结果表明,RTCH算法能更有效地均衡网络中的能量消耗,延长网络生命周期。 相似文献
920.
为适应无线传感器网络大数据量传输的需求,提出一种基于能量优先的拥塞缓解机制(PECR)。根据网络对整体能耗的要求,将节点剩余能量作为一项重要参考指标。节点周期性地检测缓冲区队列占用率来确定当前拥塞度,当拥塞发生时,节点依据拥塞度和剩余能量两项属性,尝试在拥塞节点周围建立临时最佳路径进行分流调节。实验结果表明,采用该机制时,在有节点冗余的网络区域内,可降低节点能耗,提高网络整体生存寿命。 相似文献