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An in situ fully light‐driven switching of superhydrophobic adhesion is demonstrated based on simply spin‐coating a hydrophobic azo‐polymer on an optimized micro‐nanopost arrayed silicon substrate. Furthermore, the detailed designing principles are discussed, which might shed light on efficient exploitation of superhydrophobic liquid/solid interfaces for smart microfluidic control.  相似文献   
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One of the most fascinating properties of materials in nature is the superhydrophobic and self‐cleaning capabilities of different plant surfaces. This is usually achieved by the hydrophobic cuticles that are made of cutin and contain wax crystals both within them and on their surfaces. Here, bioinspired n‐hexatriacontane wax films are deposited via thermal evaporation and it is shown that the surface evolves in time via self‐assembly. This leads to a dramatic change in the wetting properties with a transition from hydrophobic to superhydrophobic characteristics, which takes place within several days at room temperature. This phenomenon is investigated and strain‐induced recrystallization is proposed to be the mechanism for it. This work could become the basis for the inspiration and production of tuned, time‐dependant, temperature‐sensitive, variable‐wettability surfaces.  相似文献   
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Liquid marble (LM) is a droplet that is wrapped by hydrophobic solid particles, which behave as a non-wetting soft solid. Based on these properties, LM can be applied in fluidics and soft device applications. A wide variety of functional particles have been synthesized to form functional LMs. However, the formation of multifunctional LMs by integrating several types of functional particles is challenging. Here, a general strategy for the flexible patterning of functional particles on droplet surfaces in a patchwork-like design is reported. It is shown that LMs can switch their macroscopic behavior between a stable and active state on super-repellent surfaces in situ by jamming/unjamming the surface particles. Active LMs hydrostatically coalesce to form a self-sorted particle pattern on the droplet surface. With the support of LM handling robotics, on-demand cyclic activation–manipulation–coalescence–stabilization protocols by LMs with different sizes and particle types result in the reliable design of multi-faced LMs. Based on this concept, a single bi-functional LM is designed from two mono-functional LMs as an advanced droplet carrier.  相似文献   
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A novel fabrication method is developed for the preparation of superhydrophobic surfaces. The procedure uses focal conic structures of semi‐fluorinated smectic liquid crystals (LCs) whose periodic toric focal conic domains (TFCDs) are prepared on a surface modified substrate. Reactive ion etching (RIE) on the periodic TFCD surface leads to a superhydrophobic surface with a water contact angle of ~160° and a sliding angle of ~2° for a 10 µL water droplet. The results show that this phenomenon is due to the development of a dual‐scale surface roughness arising from the nanoscale protuberance caused by applying the RIE process to the top of the microscale TFCD arrays. The unique surface behavior is further verified by demonstrating that RIE on a flat lamellar liquid crystal film, in which the director is aligned parallel with surface, results in a relatively low hydrophobicity as compared to when periodic TFCDs are subjected to REI. The observations made in this publication suggest that a new approach exists for selecting potential candidates of superhydrophic surface formation based on spontaneous self‐assembly in smectic liquid‐crystalline materials.  相似文献   
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Antigravity transportation of water, which is often observed in nature, is becoming a vital demand for advanced devices and new technology. Many studies have been devoted to the motion of a single droplet on a horizontal or inclined substrate under specific assistance. However, the self‐propelled water motion, especially continuous antigravity water delivery, still remains a considerable challenge. Here, a novel self‐ascending phenomenon driven only by the surface energy release of water droplets is found, and a superhydrophobic mesh to pump water up to a height of centimeter scale is designed. An integrated antigravity transportation system is also demonstrated to continuously and spontaneously pump water droplets without additional driving forces. The present novel finding and integrated devices should serve as a source of inspiration for the design of advanced materials and for the development of new technology with exciting applications in microfluidics, microdetectors, and intelligent systems.  相似文献   
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Fog formation decreases light transmission of optically clear materials. A promising approach to address this problem is to control the wetting properties of the material at extremes states, which requires imparting micro and nano morphology features on the surface. However, such features may affect the optical properties of the surface. In this work, superhydrophobic and superhydrophilic surfaces, with different morphology characteristics ranging from nanoscale to hierarchical micro-nanoscale are fabricated and evaluated in order to investigate which wetting extreme and surface morphology is more suitable to preserve the light-transmitting properties and exhibit antifogging functionalities. The performance of the aforementioned surfaces is compared for the first time in two different testing modes: under intense fog flow and no surface cooling, and under no-flow and surface cooling, which enhances dew condensation on the surfaces. It is demonstrated that superhydrophilic surfaces with nanoscale morphology maintain their optical transmittance under fog flow for more than 20 min. This duration is one of the longest reported in the literature revealing the long-term antifogging functionality of the proposed surfaces. Finally, by tailoring the morphology and the surface wetting properties, an optically switching surface (initially “milky” which becomes “clear”) when exposed to humidity is demonstrated.  相似文献   
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A superelastic aerogel with fast shape recovery performance from large compressive strain is highly desired for numerous applications such as thermal insulation in clothing, high-sensitive sensors, and oil contaminant removal. Fabrication of superelastic cellulose nanofibrils (CNF) aerogels is challenging as the CNF can assemble into non-elastic sheet-like cell walls. Here, a dual ice-templating assembly (DITA) strategy is proposed that can control the assembly of CNF into sub-micrometer fibers by extremely low temperature freezing (–196 °C), which can further assemble into an elastic aerogel with interconnected sub-micron fibers by freezer freezing (−20 °C) and freeze drying. The CNF aerogel from the DITA process demonstrates isotropic superelastic behavior that can recover from over 80% compressive strain along both longitudinal and cross-sectional directions, even in an extremely cold liquid nitrogen environment. The elastic CNF aerogel can be easily modified by chemical vapor deposition of organosilane, demonstrating superhydrophobicity (164° water contact angle), high liquid absorption (489 g g−1 of chloroform absorption capacity), self-cleaning, thermal insulating (0.023 W (mK)−1), and infrared shielding properties. This new DITA strategy provides a facile design of superelastic aerogels from bio-based nanomaterials, and the derived high performance multifunctional elastic aerogel is expected to be useful for a wide-range of applications.  相似文献   
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