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1.
The effect of the platinum particle size was investigated for the catalytic oxidative dehydrogenation of aqueous ethanol to ethanal at a temperature of 303 K, an ethanol concentration of 260 mol m–3, a partial oxygen pressure 60 kPa, a pH of 9, and an ethanal and ethanoate concentration of 20 mol m–3. A particle size effect on the turnover frequency was observed but only for particle sizes smaller than 2 nm. Hence, the reaction shows a limited structure sensitivity. 相似文献
2.
Nickel-cobalt and nickel-iron electrodeposits were characterized as hydrogen electrodes in alkaline water electrolysis (6 mol/L KOH, 25°C). The nickel-based codeposits were fabricated with different bath compositions and at different current densities. The hydrogen evolution in water electrolysis on the nickel-based codeposits was apparently enhanced as compared with that on nickel. The improvement of the electrocatalytic behaviour of the hydrogen electrodes is attributed to their composition and an increase of their active surface, which are dependent on the electrodeposition conditions. 相似文献
3.
Requena C.G. Requena M.E.G. Rodriguez P.J.L. Marin J.F.D. 《Parallel and Distributed Systems, IEEE Transactions on》2009,20(6):802-817
Fault tolerance in the interconnection network of large clusters of PCs is an issue of growing importance, since their increasing size also increases the failure probability. The fat-tree topology is usually used in these machines since it has become very popular among high-speed interconnect manufacturers. This paper proposes a new distributed fault-tolerant routing methodology for fat trees. Unlike other previous proposals, it does not require additional network hardware, and its memory requirements, switch hardware, and routing delay scales up with the network size. Indeed, it nullifies only the strictly necessary paths, allowing adaptive routing through the healthy paths. The methodology is based on enhancing the interval routing scheme with exclusion intervals. Exclusion intervals are associated to each switch output port and represent the nodes that are unreachable from this port after a fault. We propose a methodology to identify the links where the exclusion intervals must be updated after a fault, the values to write on them, and a very efficient mechanism to distribute the required information through the network without stopping the system activity. Our methodology can tolerate a high number of network failures with a low degradation in performance. Moreover, it can achieve zero packet losing during the updating period. 相似文献
4.
L. Marin A. Karageorghis D. Lesnic B. T. Johansson 《Inverse Problems in Science & Engineering》2017,25(5):652-673
An inverse problem in static thermo-elasticity is investigated. The aim is to reconstruct the unspecified boundary data, as well as the temperature and displacement inside a body from over-specified boundary data measured on an accessible portion of its boundary. The problem is linear but ill-posed. The uniqueness of the solution is established but the continuous dependence on the input data is violated. In order to reconstruct a stable and accurate solution, the method of fundamental solutions is combined with Tikhonov regularization where the regularization parameter is selected based on the L-curve criterion. Numerical results are presented in both two and three dimensions showing the feasibility and ease of implementation of the proposed technique. 相似文献
5.
Synaptic transmission was measured at visualized terminal varicosities of the motor axon providing the sole excitatory innervation of the "opener" muscle in walking legs of crayfish (Procambarus clarkii Girard). Two questions were addressed: 1) How uniform is quantal emission at different locations along terminals innervating a single muscle fiber, and 2) can differences in quantal emission account for the different excitatory postsynaptic potential (EPSP) amplitudes generated by terminals localized in defined regions of the muscle? Extracellular "macropatch" electrodes were placed over individual varicosities, viewed after brief exposure to a fluorescent dye, and synaptic currents were recorded to determine quantal content of transmission. Along terminals supplying a single muscle fiber, nonuniform release was found: Varicosities closer to the point of origin of the terminal branch released more transmitter than those located more distally. Quantal content was higher for varicosities of the muscle's proximal region (where large EPSPs occur) than for varicosities of the central region (where small EPSPs occur). The probability of transmitter release per synapse is estimated to be greater for the proximal varicosities. At low frequencies of stimulation, quantal content per muscle fiber is two to four times larger in the proximal region. Taken in conjunction with a twofold higher mean input resistance for the proximal muscle fibers, the difference in quantal content can account for a four- to eightfold difference in EPSP amplitude. The observed mean EPSP amplitude is at least eight times larger in the proximal region. We discuss factors contributing to differences in EPSP amplitudes. 相似文献
6.
Evan J. Reed Marin Solja
i Mihai Ibanescu J. D. Joannopoulos 《Journal of Computer-Aided Materials Design》2005,12(1):1-15
We predict that reversed and anomalous non-relativistic Doppler shifts can be observed under some circumstances when light reflects from a shock wave front propagating through a photonic crystal, or material with a periodic modulation of the dielectric. This theoretical prediction is generalizable and applies to wave-like excitations in a variety of periodic media. An experimental observation of this effect has recently been made (Seddon, N. and Bearpark, T. Science, 302 (2003) 1537) and we provide a brief discussion of this experiment. 相似文献
7.
Lucas Taoro-Gonzlez Daniel Pereda Catalina Valds-Baizabal Miriam Gonzlez-Gmez Jos A. Prez Ftima Mesa-Herrera Ana Canerina-Amaro Herminia Prez-Gonzlez Covadonga Rodríguez Mario Díaz Raquel Marin 《International journal of molecular sciences》2022,23(13)
Long-chain polyunsaturated fatty acids (LCPUFA), essential molecules whose precursors must be dietary supplied, are highly represented in the brain contributing to numerous neuronal processes. Recent findings have demonstrated that LCPUFA are represented in lipid raft microstructures, where they favor molecular interactions of signaling complexes underlying neuronal functionality. During aging, the brain lipid composition changes affecting the lipid rafts’ integrity and protein signaling, which may induce memory detriment. We investigated the effect of a n-3 LCPUFA-enriched diet on the cognitive function of 6- and 15-months-old female mice. Likewise, we explored the impact of dietary n-3 LCPUFAs on hippocampal lipid rafts, and their potential correlation with aging-induced neuroinflammation. Our results demonstrate that n-3 LCPUFA supplementation improves spatial and recognition memory and restores the expression of glutamate and estrogen receptors in the hippocampal lipid rafts of aged mice to similar profiles than young ones. Additionally, the n-3 LCPUFA-enriched diet stabilized the lipid composition of the old mice’s hippocampal lipid rafts to the levels of young ones and reduced the aged-induced neuroinflammatory markers. Hence, we propose that n-3 LCPUFA supplementation leads to beneficial cognitive performance by “rejuvenating” the lipid raft microenvironment that stabilizes the integrity and interactions of memory protein players embedded in these microdomains. 相似文献
8.
Liliana Marinescu Denisa Ficai Anton Ficai Ovidiu Oprea Adrian Ionut Nicoara Bogdan Stefan Vasile Laura Boanta Alexandru Marin Ecaterina Andronescu Alina-Maria Holban 《International journal of molecular sciences》2022,23(11)
The synthesis of nanoparticles from noble metals has received high attention from researchers due to their unique properties and their wide range of applications. Silver nanoparticles (AgNPs), in particular, show a remarkable inhibitory effect against microorganisms and viruses. Various methods have been developed to obtain AgNPs, however the stability of such nanostructures over time is still challenging. Researchers attempt to obtain particular shapes and sizes in order to tailor AgNPs properties for specific areas, such as biochemistry, biology, agriculture, electronics, medicine, and industry. The aim of this study was to design AgNPs with improved antimicrobial characteristics and stability. Two different wet chemical routes were considered: synthesis being performed (i) reduction method at room temperatures and (ii) solvothermal method at high temperature. Here, we show that the antimicrobial properties of the obtained AgNPs, are influenced by their synthesis route, which impact on the size and shape of the structures. This work analyses and compares the antimicrobial properties of the obtained AgNPs, based on their structure, sizes and morphologies which are influenced, in turn, not only by the type or quantities of precursors used but also by the temperature of the reaction. Generally, AgNPs obtained by solvothermal, at raised temperature, registered better antimicrobial activity as compared to NPs obtained by reduction method at room temperature. 相似文献
9.
10.
G. Marin S. M. Wasim G. Sánchez Pérez P. Bocaranda A. E. Mora 《Journal of Electronic Materials》1998,27(12):1351-1357
A new method to grow single crystals with stoichiometry close to 1:1:2 of CuInTe2, an important member of the Cu-III-VI2 family of semiconductors is described. This consists of tellurization in the liquid phase of stoichiometric Cu and In and
later solidification under directional freezing. It is found from energy dispersive spectroscopy that the ingots obtained
with the evaporation temperature (Tt) of Te at 590 and 635°C were very close to the ideal stoichiometry 1:1:2. Samples of all ingots obtained with Tt between 530 and 690°C, as studied by x-ray and differential thermal analysis, were of single phase having chalcopyrite structure
and p-type conductivity. Optical and electrical characterization of different ingots were made. The acceptor ionization energy
EA and the density of states effective mass m
p
*
of the holes are estimated from the temperature dependence of the hole concentration p in samples of different ingots. m
p
*
= (0.78 ± 0.02) me agrees quite well with the reported value. From a combined analysis of the variation of EA with p1/3 and the knowledge of molecularity and valence stoichiometry of each sample, it is established that the shallow acceptor level
observed in different samples with EA (0) ⋍ 30 meV is due to VIn. 相似文献