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Vineet Kumar Md. Najib Alam Amutheesan Manikkavel Jungwook Choi Dong-Joo Lee 《乙烯基与添加剂工艺杂志》2021,27(2):254-263
New technology is constantly required for updating new generation flexible devices, such as stretchable sensors, flexible electronics, and actuators. In the present study, a stretchable strain sensor, and actuator were developed based on room-temperature-vulcanized (RTV) silicone rubber reinforced with carbon nanotubes (CNTs), nanographite (GR), and CNT-GR hybrids. A CNT-based strain sensor developed for RTV silicone rubber showed improved stiffness and brittleness. For example, at 5 phr of filler loading, the compressive and tensile modulus for the CNT-reinforced RTV silicone matrix improved by 287% and 240%, respectively. Similarly, the improvements in the compressive and tensile modulus were moderate for the CNT-GR hybrid (210% and 235%) and low for GR (135% and 125%). The improved brittleness resulted in a higher fracture strain of 170% and 155% for the CNT-GR hybrid and GR, respectively. The improved mechanical properties were tested in real-life applications of actuation. The actuation displacement at a filler loading of 2 phr increased to 1.65 mm (CNT), 1.25 mm (CNT-GR), and 0.08 mm (GR). From 2 to 8 kV, the actuation displacement increased by 825% (CNT), 830% (CNT-GR), and 32% (GR). The strain sensor showed a stretchability of >100% (CNT) and >100% (CNT-GR). In addition, the gauge factor was higher for the CNT-GR hybrid composites. The durability measurements showed that the change in resistance was negligible for up to 5000 cycles in both the CNT and CNT-GR rubber composites. A series of experiments confirmed that compared to the composite based on RTV silicone rubber and CNT, the CNT-GR hybrid showed a robust flexibility and stretchability as a piezo-resistive strain sensor and actuator. 相似文献
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