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排序方式: 共有116条查询结果,搜索用时 15 毫秒
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Anubhav Jain Ivano E. Castelli Geoffroy Hautier David H. Bailey Karsten W. Jacobsen 《Journal of Materials Science》2013,48(19):6519-6534
We examine the performance of genetic algorithms (GAs) in uncovering solar water light splitters over a space of almost 19,000 perovskite materials. The entire search space was previously calculated using density functional theory to determine solutions that fulfill constraints on stability, band gap, and band edge position. Here, we test over 2500 unique GA implementations in finding these solutions to determine whether GA can avoid the need for brute force search, and thereby enable larger chemical spaces to be screened within a given computational budget. We find that the best GAs tested offer almost a 6 times efficiency gain over random search, and are comparable to the performance of a search based on informed chemical rules. In addition, the GA is almost 10 times as efficient as random search in finding half the solutions within the search space. By employing chemical rules, the performance of the GA can be further improved to approximately 12–17 better than random search. We discuss the effect of population size, selection function, crossover function, mutation rate, fitness function, and elitism on the final result, finding that selection function and elitism are especially important to GA performance. In addition, we determine that parameters that perform well in finding solar water splitters can also be applied to discovering transparent photocorrosion shields. Our results indicate that coupling GAs to high-throughput density functional calculations presents a promising method to rapidly search large chemical spaces for technological materials. 相似文献
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In the forest industry, bark is an abundant residue, predominantly converted into calorific energy. As the antioxidant potential of phenolic compounds from sugar maple (Acer saccharum Marsh.) and red maple (Acer rubrum L.) bark has previously been established, the present study focused on the hot-water extraction optimization of these barks. Several process parameters (maple species, temperature, duration, ratio bark/water, particle size) were thus studied and large disparities were found between the two species. Extraction yield, phenolic content, and antioxidant capacity of red maple extracts were several times higher than those of sugar maple extracts. Principal component analysis, applied to the selected best extraction conditions, identified 3–4 clusters depending on the maple species. These groups were sorted from the highest extraction yield and energy consumption combined with the lowest phenolic content and antioxidant capacity, to moderate extraction yield and energy consumption with the highest phenolic content and antioxidant capacity. 相似文献
5.
This paper presents a new passive technique for estimating the bottleneck bandwidth based on transferring the Gaussian kernel density estimation of the packets inter-arrival times to the frequency domain. The resulting spectrum contains information about the transmission time of the bottleneck link and can reveal information about multiple bottlenecks if they exist along the end-to-end path. The advantage of the technique is that it provides a model that can be manipulated by the digital signal processing methods and, unlike prior work in the area, it relies less on statistical methods. The proposed technique was validated using the ns2 network simulator [1] on several topologies and traffic sources. Further experiments were conducted to test the strength of the patterns between flows that share a bottleneck by applying K-means algorithm to cluster the average packet inter-arrival times of these flows. The paper also presents a set of results from real traffic experiments conducted in order to infer both the bottleneck bandwidth and the capacity of the path using a passive approach. 相似文献
6.
Alla Popova Ghita Geoffroy Marie-France Renou-Gonnord Pascal Faucon Ellis Gartner 《Journal of the American Ceramic Society》2000,83(10):2556-2560
To better understand the mechanism of interaction between hydrating silicate-based cements and polymeric dispersants of the type used as "superplasticizers" in modern construction concretes, two different types of polymeric dispersant were added (at concentrations of 1 and 10 g/L) during the synthesis of calcium silicate hydrate (C-S-H) via the "pozzolanic reaction" in dilute slurries of lime and reactive silica, at Ca/Si ratios in the range of 0.66–1.50. Although both polymers gave degrees of adsorption of >79% in all cases studied, no significant structural modifications of the resulting C-S-H products were observed via X-ray diffraction or 29 Si magic angle spinning–nuclear magnetic resonance. These results differ from recent work in which it was shown that similar types of polymer could intercalate into the interlayers of C-S-H that was made using an alternative process. It is suggested that the process by which the C-S-H is formed may have a strong influence on whether C-S-H can intercalate polymers. This observation is relevant to understanding the fate of such polymers in concrete. 相似文献
7.
O. R. Ghita M. A. Beard J. McCabe R. Bottom J. Richmond K. E. Evans 《Journal of Materials Science》2008,43(14):4988-4995
Thermal and spectral analysis is conducted routinely to characterise a large range of materials and compounds. However, tests
are often conducted independently on separate samples where comparison between essentially the same material can provide conflicting
results. Simultaneous thermal and spectral measurements have the advantage of being able to directly compare results using
the same sample. A novel design of a simultaneous thermal and spectral technique is described along with application examples
that highlight the benefits of this technique. The thermal analysis was conducted using Differential Scanning Calorimetry
(DSC) and the in situ spectral analysis was conducted using a Fourier Transform Near Infrared (FT-NIR) spectrometer. Two examples
are used to illustrate the versatility and potential advantages of the combined thermal and spectral method. Analysis of the
first and second order transitions of polyethylene terephthalate (PET) is presented along with the pharmaceutical polymorphic
conversion of carbamazepine from Form III to Form I through an isothermal hold at 160 °C. 相似文献
8.
Alla Popova Ghita Geoffroy Ellis M. Gartner A. Lapp 《Journal of the American Ceramic Society》2002,85(5):1303-1305
Small-angle neutron scattering (SANS) was used to study calcium silicate hydrate (C-S-H) formed via pozzolanic reaction between calcium oxide and ultrafine silica in water or polymer solutions at a temperature of 20°C. The SANS profile of this product was consistent with a structure that consisted of platelets with maximum diameters of ∼20 nm (± 5 nm) in the x – y plane, which was similar to a structure that had been deduced in previous work via X-ray diffractometry. The presence of two different types of superplasticizer in solution (at a concentration of 10 g/L) had no significant effect on its formation kinetics or its SANS profile. 相似文献
9.
Cellular response to radiation damage is made by a complex network of pathways and feedback loops whose spatiotemporal organisation is still unclear despite its decisive role in determining the fate of the damaged cell. Revealing the dynamic sequence of the repair proteins is therefore critical in understanding how the DNA repair mechanisms work. There are also still open questions regarding the possible movement of damaged chromatin domains and its role as trigger for lesion recognition and signalling in the DNA repair context. The single-cell approach and the high spatial resolution offered by microbeams provide the perfect tool to study and quantify the dynamic processes associated with the induction and repair of DNA damage. We have followed the development of radiation-induced foci for three DNA damage markers (i.e. γ-H2AX, 53BP1 and hSSB1) using normal fibroblasts (AG01522), human breast adenocarcinoma cells (MCF7) and human fibrosarcoma cells (HT1080) stably transfected with yellow fluorescent protein fusion proteins following irradiation with the QUB X-ray microbeam (carbon X-rays <2 μm spot). The size and intensity of the foci has been analysed as a function of dose and time post-irradiation to investigate the dynamics of the above-mentioned DNA repair processes and monitor the remodelling of chromatin structure that the cell undergoes to deal with DNA damage. 相似文献
10.
JM Tronchet L Brenas F Barbalat-Rey M Zsély M Geoffroy 《Canadian Metallurgical Quarterly》1998,17(6):1019-1031
Bicyclonucleosides bearing a 5-deoxy-5-N-hydroxyamino-3,N5-(1,1-ethano)-beta-D-furanosyl sugar moiety (15-18) have been prepared by glycosidation of the corresponding bicyclosugars obtained via an intramolecular reverse Cope elimination. The configuration of the asymmetric carbon of the 1,1-ethano bridge is the most important factor directing the conformation of the N-hydroxypyrrolidine ring and its invertomers ratio as shown by variable temperature H NMR experiments. 相似文献