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The Hammett equation correlates the effects of Y on many different chemical properties of YC(6)H(4)ZX families of compounds. One of the most surprising is that the Z-X bond dissociation enthalpy (BDE), a homolytic property, can be correlated for some 4-YC(6)H(4)ZX families with electrophilic substituent constants, sigma(p)(+)(Y), which were largely derived from the rates of the heterolytic S(N)1 solvolyses of para-substituted cumyl chlorides. Although there is no Hammett correlation of the C-X BDEs in 4-YC(6)H(4)CH(2)X (X = H, halide, OPh) families, there are good correlations of N-X BDEs with sigma(p)(+)(Y) in 4-YC(6)H(4)NHX (X = H, CH(3), OH, F) and excellent correlations of O-X BDEs with sigma(p)(+)(Y) in 4-YC(6)H(4)OX (X = H, CH(3), CH(2)Ph) families. The reasons for this varied behavior are discussed. 相似文献
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Andre Suslik Spritzer Jeremy Boy Pierre Dragicevic Jean‐Daniel Fekete Carla Maria Dal Sasso Freitas 《Computer Graphics Forum》2015,34(3):461-470
Node‐link infographics are visually very rich and can communicate messages effectively, but can be very difficult to create, often involving a painstaking and artisanal process. In this paper we present an investigation of node‐link visualizations for communication and how to better support their creation. We begin by breaking down these images into their basic elements and analyzing how they are created. We then present a set of techniques aimed at improving the creation workflow by bringing more flexibility and power to users, letting them manipulate all aspects of a node‐link diagram (layout, visual attributes, etc.) while taking into account the context in which it will appear. These techniques were implemented in a proof‐of‐concept prototype called GraphCoiffure, which was designed as an intermediary step between graph drawing/editing software and image authoring applications. We describe how GraphCoiffure improves the workflow and illustrate its benefits through practical examples. 相似文献
5.
Gino Canella 《Digital Creativity》2017,28(1):24-37
ABSTRACTScholars and activists have studied social movement media for its potential to challenge dominant narratives, build community relationships and create social change. This paper presents a case study of two short-form documentary projects with Black Lives Matter 5280 and the Service Employees International Union, Local 105 in Denver, Colorado to explore how collaborative media-making projects assist in building local grassroots campaigns of racial and economic justice. The communication strategies as well as the distribution efforts via online social networks and community screenings are discussed in order to analyse how documentaries rely upon personal narratives to animate members and allies’ feelings and then connect them with traditional forms of organizing like community meetings and public demonstrations. The participatory aspects of filmmaking are viewed through democratic theory, which emphasizes the social relations of citizenship and shared communal values over material and cultural resources, rather than visual aesthetics or technical processes. 相似文献
6.
Non-photorealistic (illustrative) rendering augments typical rendering models to selectively emphasize or de-emphasize specific
structures of rendered objects. Illustrative techniques may affect not only the rendering style of specific portions of an
object but also their visibility, ensuring that less important regions do not occlude more important ones. Cutaway views completely
remove occluding, unimportant structures—possibly also removing valuable context information—while existing solutions for
smooth reduction of occlusion based on importance lack precise visibility control, simplicity and generality. We introduce
a new front-to-back fragment composition equation that directly takes into account a measure of sample importance and allows smooth and precise
importance-based visibility control. We demonstrate the generality of our composition equation with several illustrative effects,
which were obtained by using a set of importance measures calculated on the fly or defined by the user. The presented composition
method is suitable for direct volume rendering as well as rendering of layered 3D models. We discuss both cases and show examples,
though focusing mainly on illustration of volumetric data. 相似文献
7.
E. Mancini F. Campana M. Sasso G. Newaz 《The International Journal of Advanced Manufacturing Technology》2012,61(1-4):63-72
In cold rolling some surface defects, known as pits, are due to lubricant that, entrapped in the deep valleys of the surface roughness, is nearly incompressible and acts like an inclusion avoiding microcavity elimination. During the rolling process, when specific favorable conditions can be set up, the lubricant may be expelled by the microplasto-hydrodynamic lubrication (MPHL) mechanism and pits may be recovered. In this paper the Λm parameter, index of the MPHL, is investigated together with the neutral point position to better understand the practical process recommendations for surface defect recovery. By means of finite element analysis of a Sendzimir’cold rolling process, the sensitivity of these objective functions are studied by means of a design of experiment analysis changing the major process variables like back tension, friction coefficient, reduction parameter, initial thickness, and roll diameter. 相似文献
8.
La Russa Mauro F. Ruffolo Silvestro A. de Buergo Mónica Álvarez Ricca Michela Belfiore Cristina M. Pezzino Antonino Crisci Gino M. 《Bulletin of Engineering Geology and the Environment》2017,76(1):115-124
Bulletin of Engineering Geology and the Environment - Salt crystallization is a strong weathering agent in porous building materials. The crystallization pressure exerted by salt crystals, growing... 相似文献
9.
数字单边带下变频器是软件无线电中不可缺少的组成部分,也是射电观测中,数据采集设备的重要组成部分,由于该模块紧接高速A/D采样器之后,所以对其运算处理能力有很高的要求.本文提出了实现宽带数字单边带下变频器的一种可行方案——并行处理,可以从根本上解决数字信号处理的瓶颈效应. 相似文献
10.
Beatrice Piola Maurizio Sabbatini Sarah Gino Marco Invernizzi Filippo Ren 《International journal of molecular sciences》2022,23(1)
In recent years, bioprinting has attracted much attention as a potential tool for generating complex 3D biological constructs capable of mimicking the native tissue microenvironment and promoting physiologically relevant cell–cell and cell–matrix interactions. The aim of the present study was to develop a crosslinked 3D printable hydrogel based on biocompatible natural polymers, gelatin and xanthan gum at different percentages to be used both as a scaffold for cell growth and as a wound dressing. The CellInk Inkredible 3D printer was used for the 3D printing of hydrogels, and a glutaraldehyde solution was tested for the crosslinking process. We were able to obtain two kinds of printable hydrogels with different porosity, swelling and degradation time. Subsequently, the printed hydrogels were characterized from the point of view of biocompatibility. Our results showed that gelatin/xanthan-gum bioprinted hydrogels were biocompatible materials, as they allowed both human keratinocyte and fibroblast in vitro growth for 14 days. These two bioprintable hydrogels could be also used as a helpful dressing material. 相似文献