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排序方式: 共有480条查询结果,搜索用时 15 毫秒
1.
Keita Ikeue Shingo Ando Tomohiro Mitsuyama Yusuke Ohta Keishi Arayama Akiko Tsutsumi Masato Machida 《Topics in Catalysis》2008,47(3-4):175-180
Lanthanide-based oxysulfides and sulfide, LnTaO3.5S0.5, Ln10OS14 (Ln = La, Pr, Nd, Sm) and La4In5S13, were successively synthesized by sulfurization in a flowing H2S. The sulfurization decreased the band-gap energies from >4 eV to <3eV, because of the formation of occupied S3p orbitals
on the top of valence band. In accordance with the small band gap, the H2 evolution from a 0.01 M Na2S and 0.01 M Na2SO3 solution system was observed under irradiation of light up to >500 nm. The rate of H2 evolution under light irradiation of >500 nm increased in the order of Ni/LaTaO3.5S0.5 < Ru/La10OS14 < Pt/La4In5S13. 相似文献
2.
Keiji Itabashi Takuji Ikeda Akihiko Matsumoto Kunikazu Kamioka Masanao Kato Kazuo Tsutsumi 《Microporous and mesoporous materials》2008,114(1-3):495-506
Four types of Rb-aluminosilicate zeolites were hydrothermally synthesized in pure phase for the first time from Rb-aluminosilicate gels without using any organic structure-directing agent (SDA) under stirring conditions. The crystal structure of each zeolite was refined by Rietveld analysis of the X-ray diffraction (XRD) data. These crystal structures were confirmed to be Rb-mordenite, Rb-merlinoite, a new aluminosilicate zeolite with an ATT framework topology, and Rb-offretite denoted by RMA-1, RMA-2, RMA-3, and RMA-4, respectively. The Si/Al ratio of RMA-1 with an MOR topology varied from 5.3 to 8.0; however, the variation of the Si/Al ratios of the other zeolites was rather small. The crystal system of RMA-2 was tetragonal with space group I4/mmm, where two Rb sites were distributed at the center of an 8-membered ring (MR). On the other hand, two Rb sites in RMA-3 were located at the center of the 8-MR in small two cages. The structure of RMA-4 was identified as the OFF type with a local disorder or defect, which included a small amount of an intergrown ERI phase. 相似文献
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5.
Toshihide Suzuki Teruo Miyazawa Kenshiro Fujimoto Miki Otsuka Masako Tsutsumi 《Lipids》1993,28(8):775-778
The levels of phosphatidylcholine hydroperoxide in serially cultured human fetal diploid fibroblasts at various population
doubling levels were determined by high-performance liquid chromatography combined with chemiluminescence detections. This
methodology utilizes a mixture of cytochromec and luminol as post-column hydroperoxide group specific luminescent reagents. The cellular hydroperoxide content increased
with age from 0.34 to 27.72 pmol/106 cells. At the end of the cells'in vitro lifespan (51st population doubling level), the hydroperoxide content per 106 cells reached about 80 times the level found in cells of the 20th population doubling level. Supplementation of exogenous
α-tocopherol to the culture medium prevented hydroperoxide accumulation, but did not extent the lifespanin vitro. The results indicate that substantial intracellular phospholipid hydroperoxide accumulation occurred in the course of aging
of human fetal liploid fibroblasts. 相似文献
6.
Atsuhiko Yamanaka Tooru Kitagawa Masayuki Tsutsumi Toshihiro Kashima Hiroyuki Fujishiro Kimiko Ema Yoshinobu Izumi Shigehiro Nishijima 《应用聚合物科学杂志》2004,93(6):2918-2925
High strength polyethylene fiber (Toyobo, Dyneema® fiber: hereinafter abbreviated to DF) has a negative thermal expansion coefficient. Relation between fiber structure and thermal strain of DF used as reinforcement of DF reinforced plastic (DFRP) for cryogenic use was investigated. The crystallinities and orientation angles of several kinds of polyethylene fibers having different modulus from 15 to 134Gpa (herein after abbreviated to DFs) were measured by NMR and X‐ray. We obtained the parameters of the mechanical series‐parallel model composed of crystal and amorphous by crystallinity and modulus. Thermal expansion coefficients of DFs were estimated by mechanical series‐parallel model. All DFs having different modulus showed negative thermal expansion coefficients in the temperature range from 180 to 300K, and absolute values of those markedly increased by increasing tensile modulus of DF. The estimated thermal expansion coefficients showed negative values, and thermal strains showed a similar curve to observed ones mostly. Average thermal expansion coefficients in the temperature range from 180 to 300K estimated by mechanical model agreed with the observed ones. © 2004 Wiley Periodicals, Inc. J Appl Polym Sci 93: 2918–2925, 2004 相似文献
7.
Y. Tsutsumi 《Powder Technology》1973,7(3):181-188
The volume of the unit cell of a powder bed in a general case is calculated, and an equation is proposed for calculating the porosity of the bed consisting of uniformly sized ellipsoidal particles in contact and regularly arranged. In the case of uniformly sized spherical particles in contact, the equation can be simplified.Three dimensions and face angles of the unit cell are given for each regular arrangement both in cases of ellipsoidal and spherical particles. The values of the porosity are calculated by using the author's equation: the results for both ellipsoids and spheres are equal when tire particle arrangements are the same.The face angles of the unit cells proposed by Graton and Fraser are modified in two cases by the author's method of calculation and a system omitted from their classification is described. Other equations for calculation of the porosity are discussed. 相似文献
8.
Toshihiro Nagao Yuji Shimada Yoshie Yamauchi-Sato Takaya Yamamoto Masaaki Kasai Kentaro Tsutsumi Akio Sugihara Yoshio Tominaga 《Journal of the American Oil Chemists' Society》2002,79(3):303-308
A commercial product of CLA contains almost equal amounts of cis-9,trans-11 (c9,t11)-CLA and trans-10,cis-12 (t10,c12)-CLA. We attempted to enrich the two isomers by a two-step selective esterification using Candida rugosa lipase that acted on c9,t11-CLA more strongly than on t10,c12-CLA. An FFA mixture containing CLA isomers was esterified with an equimolar amount of lauryl alcohol in a mixture of 20%
water and the lipase. When the esterification of total FA reached 50%, two isomers were fractionated in a good yield: t10,c12-CLA was enriched in FFA, and c9,t11-CLA was recovered in lauryl esters. The FFA were esterified again to enrich t10,c12-CLA. At 27.3% esterification of total FA, the t10,c12-CLA content in FFA increased to 64.8 wt% with 89.3% recovery: The ratio of the content of t10,c12-CLA to that of two isomers was 95.9%. Lauryl esters obtained by the single esterification were employed for enrichment
of c9,t11-CLA. After the esters were hydrolyzed, the resulting FFA were esterified again with lauryl alcohol. At 62.0% esterification
of total FA, the c9,t11-CLA content in lauryl esters increased to 73.3 wt% with 79.4% recovery: The ratio of the content of c9,t11-CLA to that of two isomers was 95.6%. In a 600-g-scale purification, molecular distillation was effective in separating
the reaction mixture into lauryl alcohol, FFA, and lauryl ester fractions. 相似文献
9.
Amari S 《Neural computation》2007,19(10):2780-2796
When there are a number of stochastic models in the form of probability distributions, one needs to integrate them. Mixtures of distributions are frequently used, but exponential mixtures also provide a good means of integration. This letter proposes a one-parameter family of integration, called alpha-integration, which includes all of these well-known integrations. These are generalizations of various averages of numbers such as arithmetic, geometric, and harmonic averages. There are psychophysical experiments that suggest that alpha-integrations are used in the brain. The alpha-divergence between two distributions is defined, which is a natural generalization of Kullback-Leibler divergence and Hellinger distance, and it is proved that alpha-integration is optimal in the sense of minimizing alpha-divergence. The theory is applied to generalize the mixture of experts and the product of experts to the alpha-mixture of experts. The alpha-predictive distribution is also stated in the Bayesian framework. 相似文献
10.
Jun Xin Jianjun Li Anthony Vetro Shun-ichi Sekiguchi 《Multimedia Tools and Applications》2007,35(2):203-223
This paper describes novel transcoding techniques aimed for low-complexity MPEG-2 to H.264/AVC transcoding. An important application
for this type of conversion is efficient storage of broadcast video in consumer devices. The architecture for such a system
is presented, which includes novel motion mapping and mode decision algorithms. For the motion mapping, two algorithms are
presented. Both efficiently map incoming MPEG-2 motion vectors to outgoing H.264/AVC motion vectors regardless of the block
sizes that the motion vectors correspond to. In addition, the algorithm maps motion vectors to different reference pictures,
which is useful for picture type conversion and prediction from multiple reference pictures. We also propose an efficient
rate-distortion optimised macroblock coding mode decision algorithm, which first evaluates candidate modes based on a simple
cost function so that a reduced set of candidate modes is formed, then based on this reduced set, we evaluate the more complex
Lagrangian cost calculation to determine the coding mode. Extensive simulation results show that our proposed transcoder incorporating
the proposed algorithms achieves very good rate-distortion performance with low complexity. Compared with the cascaded decoder-encoder
solution, the coding efficiency is maintained while the complexity is significantly reduced.
相似文献
Shun-ichi SekiguchiEmail: |