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排序方式: 共有405条查询结果,搜索用时 31 毫秒
1.
Taro Shimonosono Yoshihiro Hirata Mubin Changgan Syohei Kamei Rina Tokaiya Soichiro Sameshima Toshifumi Yoshidome Katsuhiko Yamaji 《Ceramics International》2018,44(8):8904-8912
This paper reports the performance of porous Gd-doped ceria (GDC) electrochemical cells with Co metal in both electrodes (cell No. 1) and with Ni metal in the cathode and Co metal in the anode (cell No. 2) for CO2 decomposition, CH4 decomposition, and the dry reforming reaction of a biogas with CO2 gas (CH4 + CO2 → 2H2 + 2CO) or with O2 gas in air (3CH4 +?1.875CO2 +?1.314O2 → 6H2 +?4.875CO +?0.7515O2). GDC cell No. 1 produced H2 gas at formation rates of 0.055 and 0.33?mL-H2/(min?m2-electrode) per 1?mL-supplied gas/(min?m2-electrode) at 600?°C and 800?°C, respectively, by the reforming of the biogas with CO2 gas. Similarly, cell No. 2 produced H2 gas at formation rates of 0.40?mL-H2/(min?m2) per 1?mL-supplied gas/(min?m2) at 800?°C from a mixture of biogas and CO2 gas. The dry reforming of a real biogas with CO2 or O2 gas at 800?°C proceeded thermodynamically over the Co or Ni metal catalyst in the cathode of the porous GDC cell. Faraday's law controlled the dry reforming rate of the biogas at 600?°C in cell No. 2. This paper also clarifies the influence of carbon deposition, which originates from CH4 pyrolysis (CH4 → C + 2H2) and disproportionation of CO gas (2CO → C + CO2), on the cell performance during dry reforming. The dry reforming of a biogas with O2 molecules from air exhibits high durability because of the oxidation of the deposited carbon by supplied air. 相似文献
2.
Animesh Chakravorty 《Israel journal of chemistry》1985,25(2):99-105
Model complexes of nickel(III) and nickel(IV) are furnished by hexadentate and tridentate oxime-imine-amine ligands derived by the condensation of biacetyl monoxime with amines. The synthesis, characterisation, structure, redox equilibria and reactivity of these complexes are critically reviewed. Correlations and generalisations pertaining to oxidation state stability, electroprotic equilibria and reaction mechanisms are examined. The possible significance of the present complexes in the context of the nickel-containing methanogenic enzymes is noted. 相似文献
3.
Lussier Isabelle; Derevensky Jeffrey L.; Gupta Rina; Bergevin Tanya; Ellenbogen Stephen 《Canadian Metallurgical Quarterly》2007,21(2):165
The study of resilient children has overturned many deficit-focused models concerning the ontogenesis of children raised in adversity. This study explored the relationship between risk and protective factors, resilience, and youth gambling behavior. More specifically, this study examined the relative contribution of various risk and protective domains in relation to problem gambling behavior and examined whether youth identified as resilient (high risk exposure- high internalized protection) were as likely as those identified as vulnerable (high risk exposure-low internalized protection) to engage in excessive gambling behavior. The sample consisted of 1,273 students ages 12 to 19. The findings demonstrated that risk and protective factors each provide a unique contribution to the prediction model of gambling problems. Resilient and vulnerable youth differed significantly in their self-reported gambling severity. As well, resilient youth were not statistically distinguishable from low-risk exposure groups in terms of their gambling severity. Findings are interpreted with respect to resilience and prevention research. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
4.
C R Chakravorty 《Bulletin of Materials Science》1994,17(6):733-745
Magnesium-lithium alloys are among the lowest density metallic materials. Addition of lithium, with a relative density of
0·53, in magnesium reduces the density of the alloy significantly. Furthermore, addition of nearly 11 wt.% lithium converts
hexagonal close packed structure of pure magnesium to a body centered cubic lattice, markedly improving formability of the
alloy. The development of these alloys, however, had been hampered due to the high reactivity of lithium and magnesium in
the molten state and also, due to poor creep resistance and instability of mechanical properties at room temperature. In an
attempt to indigenize these ultra light alloys for possible applications in Indian satellite programme, detailed research
work was initiated in DMRL. The difficulties associated with producing sound cast ingots have been overcome by controlling
melting and casting parameters of these alloys. Extensive work has been done on structure-property correlation of alloys with
varying lithium content and minor alloying additions. Based on these work, advanced magnesium-lithium alloys have been developed
with improved tensile properties, room temperature stability and creep resistance. Wrought products (plates/sheets) of magnesium-lithium
alloy have been supplied to ISAC, Bangalore and are being used in their INSAT-2 programme. This paper describes the systematic
studies carried out in the laboratory to indigenize these ultra light alloys. 相似文献
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Although the basal ganglia have been shown to be critical for the expression of emotion in prosody and facial expressions, it is unclear whether they are also critical for recognition of emotions. Selective pathology of parts of the basal ganglia is a hallmark of individuals with Parkinson's disease, and such patients have been examined in several studies of emotion. We examined 18 patients with Parkinson's disease (11 men, 7 women) and 13 age-, education-, gender ratio-, and IQ-matched normal controls on their ability to recognize emotions signaled by facial expressions. Parkinson's patients performed entirely normally on a quantitative task of recognizing emotional facial expressions. The findings do not support the notion that the sectors of basal ganglia that are dysfunctional in Parkinson's disease are essential for recognizing emotion in facial expressions. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
9.
The constitution of the Ni-Al-Ru system has been investigated in the range 0 to 50 at% Al. Isothermal sections at 1523 and 1273 K have been determined using microstructural observations, electron probe microanalysis and X-ray diffraction. The phases present were: nickel-based solid solution (); (based on Ni3Al); solid solutions based on NiAl and RuAl, respectively (designated 1 and 2), and ruthenium-based solid solution (Ru). The maximum solubility of Ru in was 5 at%. 1, and 2 show extensive range of solubilities, namely up to 20at% Ru in 1 and up to 25 to 35 at% Ni in 2. Three-phase equilibrium between , 2 and (Ru) existed at 1523 and 1273 K. Also at 1523 K, three-phase equilibria existed between , and 1 and ,1 and 2, while at 1273 K, the equilibria were between , 1,2 and , , 2 indicating the occurrence of a reaction +1, +2 at a temperature between 1523 and 1273 K. Liquidus features have been deduced from data on as-solidified structures. Lattice parameter data and hardnesses are also reported. 相似文献
10.
An investigation is reported of the 75 at% nickel section of the Ni-Cr-Al-Ru system at 1523 and 1273 K. Constitutional data obtained by electron probe microanalysis, X-ray diffraction and microscopical examination are presented as partial isothermal sections. At 1523 K, the major part of the section consists of phase, while the aluminium-rich region contains a and+ region; the extent of the solid solution of chromium and ruthenium in totals ~ 4 at%. The ruthenium-rich corner of the section shows a two-phase region consisting of + ruthenium-rich solid solution. At 1273 K the,+ and + ruthenium regions increase in extent. The/ mismatch values in the equilibrated alloys studied lie in the range ~ –0.08 to –0.39%. Constitutional features of as-cast alloys are also reported. 相似文献