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排序方式: 共有151条查询结果,搜索用时 31 毫秒
1.
Pierre Santucci Christina Dedaki Alexandros Athanasoulis Laura Gallorini Anaïs Munoz Dr. Stéphane Canaan Dr. Jean-François Cavalier Dr. Victoria Magrioti 《ChemMedChem》2019,14(3):349-358
In the quest for new antibacterial agents, a series of novel long- and medium-chain mono- and disubstituted β-lactones was developed. Their activity against three pathogenic mycobacteria—M. abscessus, M. marinum, and M. tuberculosis—was assessed by the resazurin microtiter assay (REMA). Among the 16 β-lactones synthesized, only 3-hexadecyloxetan-2-one (VM005) exhibited promising activity against M. abscessus, whereas most of the β-lactones showed interesting activities against M. marinum, similar to that of the classical antibiotic, isoniazid. Regarding M. tuberculosis, six compounds were found to be active against this mycobacterium, with β-lactone VM008 [trans-(Z)-3-(hexadec-7-en-1-yl)-4-propyloxetan-2-one] being the best growth inhibitor. The promising antibacterial activities of the best compounds in this series suggest that these molecules may serve as leads for the development of much more efficient antimycobacterial agents. 相似文献
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Graziosi Fabio Ruggieri Marina Santucci Fortunato 《Wireless Personal Communications》2002,21(2):141-162
In this paper the performance of a packet mobile radio network is studied inthe presence of shadow fading outage intervals.Under quite general assumptions for the medium access protocol,the probability mass function of the sequence of packets that may be lostdue to an outage interval is derived. It is seen that long sequences of lostpackets are likely to occur for typical values of the mobile speed andshadowing correlation parameters.For delay constrained sources, e.g., voice, the analysis is mainly focused atderiving the probability function of the sequence of dropped packetsand the probability of dropping. For data sources, the delay statistic isalso derived. In the latter case, the effect of finite buffer length isaddressed. Simulation is used to verify the accuracy of approximations introduced in the analysis. 相似文献
5.
G Perini MF Saettone M Carafa E Santucci F Alhaique 《Canadian Metallurgical Quarterly》1996,135(2):145-146
This report provides X-ray diffraction and Raman spectral evidence that, when 2,6-dichlorobenzonitrile is present in the culture medium, Acetobacter xylinum, which is a model system for investigation of the biosynthesis of native cellulose, produces cellulose II, as well as cellulose I. The significance of the observations with respect to the mechanism of biosynthesis of cellulose is discussed briefly. 相似文献
6.
Catarci T. Shi-Kuo Chang Costabile M.F. Levialdi S. Santucci G. 《Knowledge and Data Engineering, IEEE Transactions on》1996,8(3):455-475
Describes an approach for multiparadigmatic visual access integration of different interaction paradigms. The user is provided with an adaptive interface augmented by a user model, supporting different visual representations of both data and queries. The visual representations are characterized on the basis of the chosen visual formalisms, namely forms, diagrams and icons. To access different databases, a unified data model called the “graph model” is used as a common underlying formalism to which databases, expressed in the most popular data models, can be mapped. Graph model databases are queried through the adaptive interface. The semantics of the query operations is formally defined in terms of graphical primitives. Such a formal approach permits us to define the concept of an “atomic query”, which is the minimal portion of a query that can be transferred from one interaction paradigm to another and processed by the system. Since certain interaction modalities and visual representations are more suitable for certain user classes, the system can suggest to the user the most appropriate interaction modality as well as the visual representation, according to the user model. Some results on user model construction are presented 相似文献
7.
In this paper we present the results of XPS study of the surface chemistry of L-CVD SnO2 thin films onto Si(100) before and after subsequent additional oxidation. Moreover, the ageing effect was also studied in order to check the influence of ambient oxidation. As-deposited L-CVD SnO2 thin films exhibit evident nonstoichiometry with the relative concentration [O]/[Sn] equal to 1.29 ± 0.1. After in situ oxidation at high temperature (800 K) the relative concentration [O]/[Sn] increases to 1.95 ± 0.05 which corresponds to the almost stoichiometric SnO2. Almost the same relative concentration [O]/[Sn] of L-CVD SnO2 thin films has been obtained after long term exposure to air. The oxidation states of L-CVD SnO2 thin films in both cases were confirmed by the shape analysis of corresponding XPS O1s and Sn3d5/2 peaks using the decomposition procedure. For the as-deposited L-CVD SnO2 thin films a mixture of SnO and SnO2 was observed, while for the oxidized L-CVD SnO2 thin films the domination of SnO2 was determined. 相似文献
8.
Intrinsic Fluorescence of the Active and the Inactive Functional Forms of Human Thymidylate Synthase
Dr. Simone Vitiello Dr. Monica Caselli Dr. Giorgia Pavesi Dr. Matteo Santucci Dr. Stefania Ferrari Prof. Maria Paola Costi Prof. Glauco Ponterini 《Chembiochem : a European journal of chemical biology》2021,22(10):1800-1810
The observables associated with protein intrinsic fluorescence – spectra, time decays, anisotropies – offer opportunities to monitor in real time and non-invasively a protein‘s functional form and its interchange with other forms with different functions. We employed these observables to sketch the fluorometric profiles of two functional forms of human thymidylate synthase (hTS), a homodimeric enzyme crucial for cell proliferation and thus targeted by anticancer drugs. The protein takes an active and an inactive form. Stabilization of the latter by peptides that, unlike classical hTS inhibitors, bind it at the monomer/monomer interface offers an alternative inhibition mechanism that promises to avoid the onset of drug resistance in anticancer therapy. The fluorescence features depicted herein can be used as tools to identify and quantify each of the two protein forms in solution, thus making it possible to investigate the kinetic and thermodynamic aspects of the active/inactive conformational interchange. Two examples of fluorometrically monitored interconversion kinetics are provided. 相似文献
9.
S. Tosti A. Santucci A. Pietropaolo S. Brutti O. Palumbo F. Trequattrini A. Paolone 《International Journal of Hydrogen Energy》2018,43(5):2817-2822
An alloy with nominal composition V85Ni15 was prepared in a vacuum induction melting apparatus. The chemical analysis of the sample showed a V (Ni) content of 82.63 (15.68) at% and small contaminations by carbon and aluminum. XRD measurements confirmed that the bcc Ni-V solid solution phase is the main constituent of the sample. However, a minor impurity (approximately 6.5 wt%) due to the precipitation of the sigma NiV3-x phase is present in the sample.Hydrogen sorption measurements extending from 150 °C up to 400 °C in a wide pressure range (up to 90 bar) were performed. Upon hydrogenation below 250 °C, one observes the subsequent presence of an α phase and of two hydride phases with different values of dehydrogenation enthalpy: ΔHdehydr = 21 ± 1 kJ/mol for 0.15 ≤ H/M ≤ 0.30 and ΔHdehydr = 26 ± 2 kJ/mol for 0.53 ≤ H/M ≤ 0.59. Above 300 °C, there is no evidence of the formation of hydrides and only an α phase is present up to the maximum measured composition, with a hydrogenation enthalpy ΔHhydr = 10.0 ± 0.5 kJ/mol. 相似文献
10.
In this letter, we propose an exact analytical framework for analyzing the performance of impulse radio (IR) ultra wide band (UWB) receiver architectures. In particular, the framework can handle i. various multipath fading distributions, ii. correlated fading, iii. channel sparseness, iv. time overlap among multipath components (MPCs), i.e., intra-pulse interference and v. both all-rake and transmitted-reference (TR) receiver architectures. The proposed methodology is based on estimating the characteristic function (CF) of the signal-to- noise ratio at the receiver, which can be reduced to a quadratic form of a random vector. 相似文献