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排序方式: 共有200条查询结果,搜索用时 78 毫秒
1.
Matteo Di Giosia Alice Soldà Markus Seeger Andrea Cantelli Fabio Arnesano Maria I. Nardella Vincenzo Mangini Francesco Valle Marco Montalti Francesco Zerbetto Stefania Rapino Matteo Calvaresi Vasilis Ntziachristos 《Advanced functional materials》2021,31(20):2101527
Fullerenes are candidates for theranostic applications because of their high photodynamic activity and intrinsic multimodal imaging contrast. However, fullerenes suffer from low solubility in aqueous media, poor biocompatibility, cell toxicity, and a tendency to aggregate. C70@lysozyme is introduced herein as a novel bioconjugate that is harmless to a cellular environment, yet is also photoactive and has excellent optical and optoacoustic contrast for tracking cellular uptake and intracellular localization. The formation, water-solubility, photoactivity, and unperturbed structure of C70@lysozyme are confirmed using UV-visible and 2D 1H, 15N NMR spectroscopy. The excellent imaging contrast of C70@lysozyme in optoacoustic and third harmonic generation microscopy is exploited to monitor its uptake in HeLa cells and lysosomal trafficking. Last, the photoactivity of C70@lysozyme and its ability to initiate cell death by means of singlet oxygen (1O2) production upon exposure to low levels of white light irradiation is demonstrated. This study introduces C70@lysozyme and other fullerene-protein conjugates as potential candidates for theranostic applications. 相似文献
2.
The TSIMMIS Approach to Mediation: Data Models and Languages 总被引:18,自引:2,他引:16
Hector Garcia-Molina Yannis Papakonstantinou Dallan Quass Anand Rajaraman Yehoshua Sagiv Jeffrey Ullman Vasilis Vassalos Jennifer Widom 《Journal of Intelligent Information Systems》1997,8(2):117-132
TSIMMIS—The Stanford-IBM Manager of Multiple InformationSources—is a system for integrating information. It offers a datamodel and a common query language that are designed to support thecombining of information from many different sources. It also offerstools for generating automatically the components that are needed tobuild systems for integrating information. In this paper we shalldiscuss the principal architectural features and their rationale. 相似文献
3.
Joan Papavasiliou George Avgouropoulos Theophilos Ioannides 《Applied catalysis. B, Environmental》2007,69(3-4):226-234
Steam reforming of methanol was carried out over a series of doped CuO–CeO2 catalysts prepared via the urea–nitrate combustion method. XRD analysis showed that at least part of the dopant cations enter the ceria lattice. The addition of various metal oxide dopants in the catalyst composition affected in a different way the catalytic performance towards H2 production. Small amounts of oxides of Sm and Zn improved the performance of CuO–CeO2, while further addition of these oxides caused a decrease in catalyst activity. XPS analysis of Zn- and Sm-doped catalysts showed that increase of dopant loading leads to surface segregation of the dopant and decrease of copper oxide dispersion. The addition of oxides of La, Zr, Mg, Gd, Y or Ca lowered or had no effect on catalytic activity, but led to less CO in the reaction products. Noble-metal modified catalysts had slightly higher activity, but the CO selectivity was also significantly higher. 相似文献
4.
Christos L. Chochos Giannis K. Govaris Fotini Kakali Joannis K. Kallitsis Vasilis G. Gregoriou 《Polymer》2005,46(13):4654-4663
New copoly(arylether)s containing substituted terphenyl, quinquephenyl, fluorene and anthracene moieties with aromatic 1,3,4-oxadiazole units were prepared and the resulting copolymers are soluble in common organic solvents. Investigation of their optical properties revealed that they emit blue and yellow light. Moreover, their photovoltaic response was studied in blends with poly(3-hexylthiophene) (P3HT) as the electron donor. Despite the low power conversion efficiencies it was shown that photo-induced electron transfer does take place and the performances are higher than a single layer P3HT device. In addition, an anthracene-fluorene-oxadiazole main chain copolymer (PAFOXD) was also examined in a single layer photovoltaic device and gave one of the highest reported open-circuit voltage (Voc) values in the literature (0.89 V). Finally, a detailed morphological study of the blends and the PAFOXD surface using the atomic force microscopy (AFM) technique, revealed the effect of solvent selection to the preparation of thin films exhibiting the desired performance characteristics. 相似文献
5.
In this paper, a two-unit multistate repairable production system is considered in which preventive maintenance (PM) is implemented in order to improve its dependability and performance. A general model is provided for the production system using a semi-Markov process, for examining system’s limiting behaviour. Apart from combining redundancy with PM, we introduce scenarios like imperfect and failed maintenance which are usually met in real life production systems. For the proposed model, we calculate the availability, the mean time to failure and the total operational cost and we formulate optimisation problems settled with respect to the system’s inspection times. The main aim of our work is to determine the optimal inspection times and consequently the optimal PM policies to be adopted in order to optimise system’s dependability and performance. 相似文献
6.
7.
AD Gouliamos DS Kontogiannis J Androulidakis AE Kalovidouris LJ Vlahos CG Papavasiliou 《Canadian Metallurgical Quarterly》1993,17(3):446-448
The MR studies of three histologically proven spinal neurilemmomas and neurofibromas were reviewed retrospectively. There were two benign neurilemmomas (schwannomas) and one neurofibroma. The common characteristic of these cases was a central low intensity focus ("dot") seen on postcontrast T1-weighted imaging. The low intensity foci corresponded histologically to a congeries of changes including edema, microcysts, foam cells, hyalinization of blood vessels, old hemorrhage, and dystrophic calcification. 相似文献
8.
9.
Christina Plati Panos Georgiou Vasilis Papavasiliou 《Structure and Infrastructure Engineering》2016,12(9):1127-1136
This article aims to investigate the feasibility of incorporating of an artificial neural network (ANN) as an innovative technique for modelling the pavement structural condition, into pavement management systems. For the development of the ANN, strain assessment criteria are set in order to characterise the structural condition of flexible asphalt pavements with regards to fatigue failure. This initial task is directly followed with the development of an ANN model for the prediction of strains primarily based on in situ field gathered data and not through the usage of synthetic databases. For this purpose, falling weight deflectometer (FWD) measurements were systematically conducted on a highway network, with ground-penetrating radar providing the required pavement thickness data. The FWD data (i.e. deflections) were back-analysed in order to assess strains that would be utilised as output data in the process of developing the ANN model. A paper exercise demonstrates how the developed ANN model combined with the suggested conceptual approach for characterising pavement structural condition with regard to strain assessment could make provisions for pavement management activities, categorising network pavement sections according to the need for maintenance or rehabilitation. Preliminary results indicate that the ANN technique could help assist policy decision makers in deriving optimum strategies for the planning of pavement infrastructure maintenance. 相似文献
10.
B. Sorkin P. Konsin S. K. Patapis I. P. Papavasiliou J. Pedarnig R. Rössler 《Journal of Low Temperature Physics》1999,117(5-6):1277-1281
In zero applied magnetic field the fluctuation conductivity is measured and analyzed for a high-quality thin film (100 nm) of Bi
2
Sr
2
CaCu
2
O
8+
grown on a MgO substrate. The two-band model formulas derived by Konsin et al. for the temperature dependence of the anisotropic three-dimensional (3D) paraconductivity in the vicinity of a superconducting phase transition are used. One of the two correlation lengths is critical and along with the other parameters of the model it determines the fluctuation conductivity (T).The global result of two-band model mimics closely d-wave-type pairing. The theory is compared with the experiment, and we obtained reasonable values and the slope of (T), the superconducting critical temperature T
c
and the coherence length (0). 相似文献