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1.
Dehydrogenation of Light Alkanes Over Rhenium Catalysts on Conventional and Mesoporous MFI Supports 总被引:1,自引:0,他引:1
Anne Krogh Rovik Anke Hagen Iver Schmidt Søren Dahl Ib Chorkendorff Claus Hviid Christensen 《Catalysis Letters》2006,109(3-4):153-156
Recently, Re/HZSM-5 (Si/Al = 15) was shown to be an efficient catalyst for ethane dehydrogenation and aromatization at 823 K
and atmospheric pressure. In this reaction, the major initial products were benzene, toluene and xylene (BTX), but increasing
amounts of ethene were produced with time on stream due to deactivation of the catalyst. We show that by use of rhenium impregnated
MFI supports with very few or no acidic sites (Si/Al > 500), highly selective ethane dehydrogenation catalysts are obtained
with ethene selectivities of 98%. By use of mesoporous MFI supports (Si/Al >500) the lifetime of the catalyst appears to be
slightly improved compared to conventional MFI crystals. The beneficial effect of a mesoporous MFI support is convincingly
demonstrated in propane dehydrogenation, where both conversion and selectivities on the mesoporous MFI (Si/Al > 500) impregnated
with Re are significantly higher than on Re supported on a comparable conventional MFI support. 相似文献
2.
Dawei Song Yanjie Shi Peng Zhang Qiang Huang Udo Kruschwitz Yuexian Hou Bo Wang 《Computational Intelligence》2015,31(4):699-720
Query language modeling based on relevance feedback has been widely applied to improve the effectiveness of information retrieval. However, intra‐query term dependencies (i.e., the dependencies between different query terms and term combinations) have not yet been sufficiently addressed in the existing approaches. This article aims to investigate this issue within a comprehensive framework, namely the Aspect Query Language Model (AM). We propose to extend the AM with a hidden Markov model (HMM) structure to incorporate the intra‐query term dependencies and learn the structure of a novel aspect HMM (AHMM) for query language modeling. In the proposed AHMM, the combinations of query terms are viewed as latent variables representing query aspects. They further form an ergodic HMM, where the dependencies between latent variables (nodes) are modeled as the transitional probabilities. The segmented chunks from the feedback documents are considered as observables of the HMM. Then the AHMM structure is optimized by the HMM, which can estimate the prior of the latent variables and the probability distribution of the observed chunks. Our extensive experiments on three large‐scale text retrieval conference (TREC) collections have shown that our method not only significantly outperforms a number of strong baselines in terms of both effectiveness and robustness but also achieves better results than the AM and another state‐of‐the‐art approach, namely the latent concept expansion model. © 2014 Wiley Periodicals, Inc. 相似文献
3.
Xiefu Jiang Qing-Long Han Shirong Liu Anke Xue 《Automatic Control, IEEE Transactions on》2008,53(4):1025-1032
This note is concerned with robust Hinfin control of linear networked control systems with time-varying network-induced delay and data packet dropout. A new Lyapunov-Krasovskii functional, which makes use of the information of both the lower and upper bounds of the time-varying network-induced delay, is proposed to drive a new delay-dependent Hinfin stabilization criterion. The criterion is formulated in the form of a non-convex matrix inequality, of which a feasible solution can be obtained by solving a minimization problem in terms of linear matrix inequalities. In order to obtain much less conservative results, a tighter bounding for some term is estimated. Moreover, no slack variable is introduced. Finally, two numerical examples are given to show the effectiveness of the proposed design method. 相似文献
4.
X-ray detectors based on straight-channel microchannel plates (MCPs) are a powerful diagnostic tool for two-dimensional, time-resolved imaging and time-resolved x-ray spectroscopy in the fields of laser-driven inertial confinement fusion and fast Z-pinch experiments. Understanding the behavior of microchannel plates as used in such detectors is critical to understanding the data obtained. The subject of this paper is a Monte Carlo computer code we have developed to simulate the electron cascade in a MCP under a static applied voltage. Also included in the simulation is elastic reflection of low-energy electrons from the channel wall, which is important at lower voltages. When model results were compared to measured MCP sensitivities, good agreement was found. Spatial resolution simulations of MCP-based detectors were also presented and found to agree with experimental measurements. 相似文献
5.
This paper investigates robust mean‐square exponential stability of a class of uncertain stochastic state‐delayed systems with Lipschitz nonlinear stochastic perturbation. Based on Lyapunov–Krasovskii functional (LKF) method and free‐weighting matrix technique, some new delay‐dependent stability conditions are established in terms of linear matrix inequalities (LMIs). In order to reduce the conservatism, (1) the delay is divided into several segments, i.e. the delay decomposition method is applied; (2) cross terms estimation is avoided; (3) some information of the cross terms relationships which has not been involved in Reference (IET Control Theory Appl. 2008; 2(11):966–973) is considered. Moreover, from the mathematical point of view, the results obtained by free‐weighting matrix technique can be equivalently re‐formulated by simpler ones without involving any additional free matrix variables. The effectiveness of the method is demonstrated by numerical examples. Copyright © 2010 John Wiley & Sons, Ltd. 相似文献
6.
Anne Köpsel Päivi Majaranta Poika Isokoski Anke Huckauf 《Behaviour & Information Technology》2016,35(12):1044-1062
Modern interaction techniques like non-intrusive gestures provide means for interacting with distant displays and smart objects without touching them. We were interested in the effects of feedback modality (auditory, haptic or visual) and its combined effect with input modality on user performance and experience in such interactions. Therefore, we conducted two exploratory experiments where numbers were entered, either by gaze or hand, using gestures composed of four stroke elements (up, down, left and right). In Experiment 1, a simple feedback was given on each stroke during the motor action of gesturing: an audible click, a haptic tap or a visual flash. In Experiment 2, a semantic feedback was given on the final gesture: the executed number was spoken, coded by haptic taps or shown as text. With simultaneous simple feedback in Experiment 1, performance with hand input was slower but more accurate than with gaze input. With semantic feedback in Experiment 2, however, hand input was only slower. Effects of feedback modality were of minor importance; nevertheless, semantic haptic feedback in Experiment 2 showed to be useless at least without extensive training. Error patterns differed between both input modes, but again not dependent on feedback modality. Taken together, the results show that in designing gestural systems, choosing a feedback modality can be given a low priority; it can be chosen according to the task, context and user preferences. 相似文献
7.
Linear programming based approximation algorithms for feedback set problems in bipartite tournaments
Anke van Zuylen 《Theoretical computer science》2011,412(23):2556-2561
We consider the feedback vertex set and feedback arc set problems on bipartite tournaments. We improve on recent results by giving a 2-approximation algorithm for the feedback vertex set problem. We show that this result is the best that we can attain when using optimal solutions to a certain linear program as a lower bound on the optimal value. For the feedback arc set problem on bipartite tournaments, we show that a recent 4-approximation algorithm proposed by Gupta (2008) [8] is incorrect. We give an alternative 4-approximation algorithm based on an algorithm for the feedback arc set on (non-bipartite) tournaments given by van Zuylen and Williamson (2009) [14]. 相似文献
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10.
Bettina?Sch?ne-SeifertEmail author Daniel?R.?Friedrich Anke?Harney Stefan?Huster Heiner?Raspe 《Ethik in der Medizin》2018,30(4):325-341