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Pierre Santucci Christina Dedaki Alexandros Athanasoulis Laura Gallorini Anaïs Munoz Dr. Stéphane Canaan Dr. Jean-François Cavalier Dr. Victoria Magrioti 《ChemMedChem》2019,14(3):349-358
In the quest for new antibacterial agents, a series of novel long- and medium-chain mono- and disubstituted β-lactones was developed. Their activity against three pathogenic mycobacteria—M. abscessus, M. marinum, and M. tuberculosis—was assessed by the resazurin microtiter assay (REMA). Among the 16 β-lactones synthesized, only 3-hexadecyloxetan-2-one (VM005) exhibited promising activity against M. abscessus, whereas most of the β-lactones showed interesting activities against M. marinum, similar to that of the classical antibiotic, isoniazid. Regarding M. tuberculosis, six compounds were found to be active against this mycobacterium, with β-lactone VM008 [trans-(Z)-3-(hexadec-7-en-1-yl)-4-propyloxetan-2-one] being the best growth inhibitor. The promising antibacterial activities of the best compounds in this series suggest that these molecules may serve as leads for the development of much more efficient antimycobacterial agents. 相似文献
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Thomas S. Lowry John C. Bright Murray E. Close Christina A. Robb Paul A. White Stewart G. Cameron 《国际水资源开发杂志》2003,19(4):579-592
The primary objective of this project is to identify gaps, whether real or perceived, that hinder effective groundwater management in New Zealand. These gaps show as gaps in information, gaps in implementation, gaps in technological and management tools, and gaps in understanding of fundamental processes. The secondary objective is to propose a management strategy to close the identified gaps. Several methods are used to meet these objectives: surveys distributed to selected staff in each regional council; the review of various written reports; the analysis of land-use databases; and private consultation within each regional council. Results show that groundwater management in New Zealand is generally reactionary with the main gaps being in strategic planning and national guidelines. Most gaps appear to be predominantly information and implementation issues. In some cases there are gaps in the understanding of fundamental processes within an aquifer system, including the long-term effects of land-use on groundwater quality. An adaptive management approach is suggested as a means of closing these gaps. 相似文献
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The Kerendan carbonate platform (Oligocene Berai Limestone) covers a subsurface area measuring approximately 11 by 16 km in the westernmost Kutei Basin, Central Kalimantan. Aggradation of the Kerendan platform occurred during a major Oligocene transgression, and is contemporaneous with aggradation and backstepping of the Barito shelf margin which was located approximately 30 km to the south. The Kerendan platform is approximately 1,000 m thick, and comprises three aggrading seismic sequences identified by the downlap of basinal strata at the platform margin and downlap of transgressive strata within the platform. Carbonate deposition started in the Late Eocene, and ended when the upper limestone sequence drowned and was covered with shale in the Late Oligocene (approximately 28.6 Ma). Three depositional areas can be distinguished in seismic sections: (1) a platform interior (lagoon); (2) a slightly raised platform rim (1–2 km wide); and (3) a basinward‐dipping platform margin and slope. The margin of the platform is identified by inflections on the seismic profiles where the relatively flat platform top begins to slope basinward. Depositional models from outcrops combined with core from three Kerendan wells were used to extrapolate depositional facies onto the seismically‐defined platform. Platform‐interior (lagoon) facies consist largely of fossiliferous wackestones and packstones, and porosities are generally lower than 5%. The platform rim is characterized by interbedded bioclastic wackestones, packstones, grainstones and boundstones, with grainstones increasing toward the platform margin. Porosity preferentially occurs in packstones, grainstones and boundstones. The platform‐rim deposits have greater porosity (5–13%) than the platform interior because the platform run is more grainstone‐rich, and because acidic waters compacting out of basinal shales concentrated dissolution near the platform margin. Pore types include vuggy porosity, microporosity within grains, and intercrystalline porosity in dolomite in the upper part of the platform rim. Different pore types have resulted in variable but locally very high permeabilities (greater than 100 mD). Permeabilities decrease with depth as vuggy pores decrease, and microporosity becomes dominant. 相似文献
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SIMULATION STUDIES OF THE REMOVAL OF WATER FROM ETHANOL BY A CATALYTIC DISTILLATION PROCESS 总被引:1,自引:0,他引:1
Christina B. Dirk-Faitakis Karl T. Chuang 《Chemical Engineering Communications》2005,192(11):1541-1557
A new approach based on catalytic distillation (CD) technology was proposed to remove water from ethanol. Isobutylene was introduced to react with water in the CD column. The commercial software simulation tool Aspen Plus was used to investigate the effects of key design factors such as operating pressure and temperature, reactant ratios, reflux and distillate to feed ratios, number of separation and reaction stages, and feed and reaction zone location. It was found that the CD technology offers potential advantages of reduced energy consumption and reduced capital cost over traditional approaches for the removal of water from ethanol. 相似文献
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Christina Dirk‐Faitakis D Grant Allen 《Journal of chemical technology and biotechnology (Oxford, Oxfordshire : 1986)》2005,80(7):737-745
This paper describes the development and simulation of an unsteady state biofilter model used to predict dynamic behaviour of cyclically‐operated biofilters and compares it with experimental results obtained from three, parallel, bench‐scale biofilters treating both periodically fluctuating concentrations and constant concentrations of an α‐pinene‐laden gas stream. The dynamic model, using kinetic parameters estimated from the constant concentration biofilter, was able to predict the performance of cyclic biofilters operating at short cycle periods (ie, in the order of minutes and hours). Steady state kinetic data from a constant concentration biofilter can be used to predict unsteady state biofilter operation. At a 24 h cycle period, the dynamic model compared well with experimental results. For long cycle periods (ie, hours and days), removal efficiency decreased after periods of non‐loading: the longer the period of non‐loading, the poorer the biofilter's performance at the re‐commencement of pollutant loading. At longer time scales the model did not effectively predict transient behaviour, as adsorption and changes in kinetic parameters were not accounted for. Modelling results showed that similar biofiltration performance for the cyclic and constant concentration biofiltration of α‐pinene is expected for biofilters operating solely in the first order kinetics regime. Poorer performance for cyclic biofilters following Monod kinetics spanning the entire kinetics range is expected as the cycle amplitude increases. The most important parameters affecting the performance of a cyclically‐operated biofilter with short cycle periods are: amplitude of cyclic fluctuations, Cg, max/Cg, relative value of the half‐saturation constant in the Monod expression, Ks, and effective diffusivity of α‐pinene in the biofilm, De. Copyright © 2005 Society of Chemical Industry 相似文献
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Izard Carroll E.; Fantauzzo Christina A.; Castle Janine M.; Haynes O. Maurice; Rayias Maria F.; Putnam Priscilla H. 《Canadian Metallurgical Quarterly》1995,31(6):997
Four studies examined aspects of the differential emotions theory (DET) hypothesis of expressive behavior development. In Study 1, facial-expressive movements of 108 2.5–9-mo-old infants were video recorded in positive and negative mother–infant interactions (conditions). As expected, Max-specified full-face and partial expressions of interest, joy, sadness, and anger were morphologically stable between the 2 ages. Studies 1 and 2 confirmed predicted differential responding to mother sadness and anger expressions and to composite positive and negative conditions. Discrete negative expressions exceeded negative blends, and the amount of both expression types remained stable across ages. Studies 3 and 4 provided varying degrees of support for the social validity of Max-specified infant negative affect expressions. Conclusions include revisions and clarifications of DET. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献