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1.
Engineering new glass compositions have experienced a sturdy tendency to move forward from (educated) trial-and-error to data- and simulation-driven strategies. In this work, we developed a computer program that combines data-driven predictive models (in this case, neural networks) with a genetic algorithm to design glass compositions with desired combinations of properties. First, we induced predictive models for the glass transition temperature (Tg) using a dataset of 45,302 compositions with 39 different chemical elements, and for the refractive index (nd) using a dataset of 41,225 compositions with 38 different chemical elements. Then, we searched for relevant glass compositions using a genetic algorithm informed by a design trend of glasses having high nd (1.7 or more) and low Tg (500 °C or less). Two candidate compositions suggested by the combined algorithms were selected and produced in the laboratory. These compositions are significantly different from those in the datasets used to induce the predictive models, showing that the used method is indeed capable of exploration. Both glasses met the constraints of the work, which supports the proposed framework. Therefore, this new tool can be immediately used for accelerating the design of new glasses. These results are a stepping stone in the pathway of machine learning-guided design of novel glasses. 相似文献
2.
Laís D. Silva Fernanda C. Puosso Viviane O. Soares Oscar Peitl Filho Simone do R.F. Sabino Francisco C. Serbena Murilo C. Crovace Edgar D. Zanotto 《Ceramics International》2021,47(13):18720-18731
Bioactive glasses and glass-ceramics (GCs) effectively regenerate bone tissue, however most GCs show improved mechanical properties. In this work, we developed and tested a rarely studied bioactive glass composition (24.4K2O-26.9CaO-46.1SiO2-2.6P2O5 mol%, identified as 45S5-K) with different particle sizes and heating rates to obtain a sintered GC that combines good fracture strength, low elastic modulus, and bioactivity. We analyzed the influence of the sintering processing conditions in the elastic modulus, Vickers microhardness, density, and crystal phase formation in the GC. The best GC shows improved properties compared with its parent glass. This glass achieves a good densification degree with a two-step viscous flow sintering approach and the resulting GC shows as high bioactivity as that of the standard 45S5 Bioglass®. Furthermore, the GC elastic modulus (56 GPa) is relatively low, minimizing stress shielding. Therefore, we unveiled the glass sintering behavior with concurrent crystallization of this complex bioactive glass composition and developed a potential GC for bone regeneration. 相似文献
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J. H. Edgar C. A. Carosella C. R. Eddy Jr D. T. Smith 《Journal of Materials Science: Materials in Electronics》1996,7(4):247-253
The effects of nitrogen-beam voltage on the structure, stress, energy band gap and hardness of AIN thin films deposited on Si (111), Si (100) and sapphire (0001) by ion beam assisted deposition (IBAD) are reported. As the nitrogen-beam voltage was increased from 50 to 200 V, the stress and disorder in the AIN films increased as determined by X-ray diffraction, FTIR and Raman spectroscopy. The preferred orientation of the film's c-axis changed from completely normal to the film at 100 V, to a mixture of normal and in the plane of the film at 200 V. For AIN films deposited under the same conditions, the films were more highly oriented on sapphire (0001) than in Si (111). The hardness of the films increased from 18.2 to 23.7 GPa with the nitrogen-beam voltage, and possible reasons for this change in hardness are considered. 相似文献
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Edgar B. Gutoff 《Drying Technology》1996,14(7):1673-1693
A complete model for the drying of coated webs. as implemented in the spreadsheet DRYWEB for Lotus and for Excel, is described. The model predicts the temperatures and solvent levels throughout the length of the dryer. The initial transient as the coated web approaches the equilibrium temperature in the consiant rate period is calculated. The coating is divided into slices for a finite difference calculation of solvent diffusion to the surface, using a simple free volume model of diffusion. The semi-empirical constants needed can be found from one or two trial runs. The possible use of infra-red heating in addition to convection heating is included in both the constant and falling rates. The calculation of infra-red energy is discussed. The model assumes that the temperature is uniform from the top of the coating to the bottom of the base, and that assumption is justified. 相似文献
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Kivlighan Dennis M.; Marsh-Angelone Maureen; Angelone Edgar O. 《Canadian Metallurgical Quarterly》1994,41(1):99
Explored projection in group counseling by examining the relationship between the group members' interpersonal problems and their perception of the group leader. Before participation, 118 personal-growth group members filled out the Inventory of Interpersonal Problems by L. M. Horowitz et al (see record 1989-10599-001) and after each session they filled out the Trainer Behavior Scale (L. Bolman, 1971). A latent variable analysis revealed that during the 1st 10 group sessions, overly dominant group members perceived the group leaders as more dominant and overly cold group members perceived the group leaders as less affiliative. There was less relationship between group members' interpersonal problems and ratings for group leaders over time. Implications of these results are discussed. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
10.
Alberto A. Robles-Loaiza Edgar A. Pinos-Tamayo Bruno Mendes Ctia Teixeira Cludia Alves Paula Gomes Jos R. Almeida 《International journal of molecular sciences》2021,22(9)
Peptide-based drugs are an attractive class of therapeutic agents, recently recognized by the pharmaceutical industry. These molecules are currently being used in the development of innovative therapies for diverse health conditions, including tropical diseases such as leishmaniasis. Despite its socioeconomic influence on public health, leishmaniasis remains long-neglected and categorized as a poverty-related disease, with limited treatment options. Peptides with antileishmanial effects encountered to date are a structurally heterogeneous group, which can be found in different natural sources—amphibians, reptiles, insects, bacteria, marine organisms, mammals, plants, and others—or inspired by natural toxins or proteins. This review details the biochemical and structural characteristics of over one hundred peptides and their potential use as molecular frameworks for the design of antileishmanial drug leads. Additionally, we detail the main chemical modifications or substitutions of amino acid residues carried out in the peptide sequence, and their implications in the development of antileishmanial candidates for clinical trials. Our bibliographic research highlights that the action of leishmanicidal peptides has been evaluated mainly using in vitro assays, with a special emphasis on the promastigote stage. In light of these findings, and considering the advances in the successful application of peptides in leishmaniasis chemotherapy, possible approaches and future directions are discussed here. 相似文献