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1.
Vladimir Rozenshtein Alexander Berg Haim Levanon Uwe Krueger Dietmar Stehlik Yuri Kandrashkin Art Van Der Est 《Israel journal of chemistry》2003,43(3-4):373-381
Light-induced spin-polarized transient EPR spectra are reported for several water-soluble copper porphyrins. The spectra are assigned to the doublet ground state, with emissive spin polarization resulting from photoexcitation and subsequent electronic relaxation. In contrast to other systems for which polarization of a doublet ground state has been observed, the exchange interactions in the copper porphyrins are strong and the geometry is fixed. It is proposed that intersystem crossing from the photoexcited trip-doublet to the trip-quartet state can lead to net polarization of the spin system and that this polarization is maintained during electronic decay, possibly via charge-transfer and exciplex states. The intensity of the observed spin polarization is essentially independent of the molecular orientation in the external field, but is strongly dependent on the nature of the charged peripheral groups. Possible reasons for this behavior are discussed. 相似文献
2.
Dietmar Schulze 《化学,工程师,技术》1995,67(1):60-68
Flowability of Bulk Solids – Definition and Measuring Principles . The flowability of bulk solids has to be known for many practical applications. The present paper describes how the flowability is defined and on which physical properties it depends. Experimental determination of the flowability using a shear test is demonstrated. Conditions influencing measuremed results are described. Finally an overview of various methods used for characterization of the flowability of bulk solids is given. 相似文献
3.
Cell suspensions of Escherichia coli as a model for bacterial populations in wastewaters were treated with ozone as a disinfectant in a continuously operated pilot plant with a plug flow reactor. Suspensions with an initial number of CFU (colony forming units) of 108 mL?1 were ozonized with ozone concentrations up to 12 mg/L. Metabolic activities and membrane functions break down with increasing ozone concentrations. The fluorochromization using 3′,6′-diacetylfluorescein (FDA) proved to be a suitable method for the detection of an alteration in permeability of the cell membranes and an inactivation of metabolic activity. By fluorescence microscopic and photometric investigations it could be clearly demonstrated that, in the case of disinfection with ozone, inactivation of the cells includes first of all a damage of the cell membranes. In contrast to the determination of the number of CFU, fluorochromization allows the detection of alteration in metabolic activities. 相似文献
4.
A technique is described to image two phases (alumina and spinel) within a metal-matrix composite which takes advantage of charging effects that occur during examination in an SEM. Microscope and specimen parameters which affect the amount of contrast generated via charging are discussed, and imaging strategies are introduced to optimize the effect. “Model” metal-matrix composite specimens were developed to verify the degree of charging in each phase. 相似文献
5.
6.
Optical DPSK at 565 Mb/s is performed by direct modulation of a narrow-linewidth 1.5-μm SL-QW-DFB (strain layer-quantum well-distributed feedback) transmitter laser. The bipolar RZ drive signal has no DC component which allows penalty-free transmission of 2 23-1 bit patterns. The heterodyne receiver contains an endless polarization controller with <6.3 or >12 rad/s tracking speed, depending on the tolerable intensity loss. A loss span of 62.3 dB is achieved,without degradation due to stimulated Brillouin scattering 相似文献
7.
8.
Georg Birkenheuer Andr�� Brinkmann Mikael H?gqvist Alexander Papaspyrou Bernhard Schott Dietmar Sommerfeld Wolfgang Ziegler 《Journal of Grid Computing》2011,9(3):355-377
Infrastructure federation is becoming an increasingly important issue for modern Distributed Computing Infrastructures (DCIs):
Dynamic elasticity of quasi-static Grid environments, incorporation of special-purpose resources into commoditized Cloud infrastructures,
cross-community collaboration for increasingly diverging areas of modern e-Science, and Cloud Bursting pose major challenges
on the technical level for many resource and middleware providers. Especially with respect to increasing costs of operating
data centers, the intelligent yet automated and secure sharing of resources is a key factor for success. With the D-Grid Scheduler
Interoperability (DGSI) project within the German D-Grid Initiative, we provide a strategic technology for the automatically
negotiated, SLA-secured, dynamically provisioned federation of resources and services for Grid-and Cloud-type infrastructures.
This goal is achieved by complementing current DCI schedulers with the ability to federate infrastructure for the temporary
leasing of resources and rechanneling of workloads. In this work, we describe the overall architecture and SLA-secured negotiation
protocols within DGSI and depict an advanced mechanism for resource delegation through means of dynamically provisioned, virtualized
middleware. Through this methodology, we provide the technological foundation for intelligent capacity planning and workload
management in a cross-infrastructure fashion. 相似文献
9.
For the development of practical semantic applications, ontologies are commonly used with rule extensions. Prominent examples of semantic applications not only are Semantic Wikis, Semantic Desktops, but also advanced Web Services and agents. The application of rules increases the expressiveness of the underlying knowledge in many ways. Likewise, the integration not only creates new challenges for the design process of such ontologies, but also existing evaluation methods have to cope with the extension of ontologies by rules.Since the verification of Owl ontologies with rule extensions is not tractable in general, we propose to verify ontologies at the symbolic level by using a declarative approach: With the new language Datalog?, known anomalies can be easily specified and tested in a compact manner. We introduce supplements to existing verification techniques to support the design of ontologies with rule enhancements, and we focus on the detection of anomalies that especially occur due to the combined use of rules and ontological definitions. 相似文献
10.
This paper proposes a clustering asset allocation scheme which provides better risk-adjusted portfolio performance than those obtained from traditional asset allocation approaches such as the equal weight strategy and the Markowitz minimum variance allocation. The clustering criterion used, which involves maximization of the in-sample Sharpe ratio (SR), is different from traditional clustering criteria reported in the literature. Two evolutionary methods, namely Differential Evolution and Genetic Algorithm, are employed to search for such an optimal clustering structure given a cluster number. To explore the clustering impact on the SR, the in-sample and the out-of-sample SR distributions of the portfolios are studied using bootstrapped data as well as simulated paths from the single index market model. It was found that the SR distributions of the portfolios under the clustering asset allocation structure have higher mean values and skewness but approximately the same standard deviation and kurtosis than those in the non-clustered case. Genetic Algorithm is suggested as a more efficient approach than Differential Evolution for the purpose of solving the clustering problem. 相似文献