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1.
2.
Effect of Particle Size on Monometallic and Bimetallic (Au,Pd)/C
on the Liquid Phase Oxidation of Glycerol 总被引:2,自引:0,他引:2
Nikolaos Dimitratos Jose Antonio Lopez-Sanchez David Lennon Francesca Porta Laura Prati Alberto Villa 《Catalysis Letters》2006,108(3-4):147-153
The influence of metal particle size of monometallic and bimetallic supported catalysts (Au, Pd, Au–Pd)/C was studied using
as a model reaction the liquid phase oxidation of glycerol. By tuning the metal particle size from 2 to 16 nm a progressive
decrease of activity and simultaneously an increase in the selectivity to sodium glycerate was observed. Moreover, the influence
of the temperature was studied and it was found that by increasing the temperature, only with a large particle size the formed
glycerate was retained and not over-oxidized to tartronate. 相似文献
3.
Prati C. Rocca F. Kost Y. Damonti E. 《Geoscience and Remote Sensing, IEEE Transactions on》1991,29(6):934-941
For high-quality SAR (synthetic aperture radar) processing, the Doppler centroid frequency is needed. However, SAR data are sampled along the azimuth direction at the pulse repetition frequency (PRF); the estimation of the Doppler centroid frequency by means of spectral analysis techniques may produce ambiguous results due to aliases. The mathematical expression of the residual error that occurs when SAR data are focused with an incorrect alias of the PRF is thus derived. Then, a blind deconvolution technique is used to estimate the actual PRF replica from the focused image. Squinted X -band data, corresponding to those that will be generated by the SIR-C mission, have been generated from the JPL-AirSAR L - and C -band data by means of an inversion of the focusing process. Even if the real data may show differences with respect to the simulated data, the blind deconvolution method appears to be more precise and robust than the other conventional techniques tested 相似文献
4.
Laura Prati Alberto Villa Francesca Porta Di Wang Dangsheng Su 《Catalysis Today》2007,122(3-4):386-390
The liquid phase oxidation of glycerol with oxygen has been studied using mono and bimetallic catalysts based on Au and Pd metals supported on activated carbon, in order to study the effect of the metal on the distribution of the products and on activity of catalysts. It was found that by using bimetallic catalysts (Au–Pd) a strong synergistic effect was shown. By using a preformed nucleating centre we were able to obtain a single alloyed phase, which allowed us to address the synergistic effect to the presence of alloyed Au/Pd. The advantage of using this latter catalyst lies not only in the high activity but also in a prolonged catalyst life. Although a partial leaching of palladium and assembling of the particles have been revealed by ICP and HRTEM respectively, activity after 10 re-cycles decreased less than expected (about 10%). 相似文献
5.
E. Ferraro M. De Michielis G. Mazzeo M. Fanciulli E. Prati 《Quantum Information Processing》2014,13(5):1155-1173
Quantum dot hybrid qubits formed from three electrons in double quantum dots represent a promising compromise between high speed and simple fabrication for solid state implementations of single-qubit and two-qubits quantum logic ports. We derive the Schrieffer–Wolff effective Hamiltonian that describes in a simple and intuitive way the qubit by combining a Hubbard-like model with a projector operator method. As a result, the Hubbard-like Hamiltonian is transformed in an equivalent expression in terms of the exchange coupling interactions between pairs of electrons. The effective Hamiltonian is exploited to derive the dynamical behavior of the system and its eigenstates on the Bloch sphere to generate qubits operation for quantum logic ports. A realistic implementation in silicon and the coupling of the qubit with a detector are discussed. 相似文献
6.
Nikolaos Dimitratos Jose Antonio Lopez-Sanchez David Morgan Albert Carley Laura Prati Graham J. Hutchings 《Catalysis Today》2007,122(3-4):317-324
Solvent free oxidation of benzyl alcohol was investigated in the absence of a base using Au catalysts prepared by sol immobilization on titania and carbon supports. Comparison between the Au supported catalysts revealed that activity and distribution of products was dependent on the nature of support and heat treatment. Specifically, heat pre-treatment of the Au catalysts has a beneficial effect in terms of activity, but is detrimental in terms of selectivity to the benzaldehyde. We conclude that sol immobilization is a suitable technique for preparing gold catalysts with small particle size and narrow particle size distributions and very high activity and selectivity for benzyl alcohol oxidation. 相似文献
7.
Davide Rotta Marco De Michielis Elena Ferraro Marco Fanciulli Enrico Prati 《Quantum Information Processing》2016,15(6):2253-2274
Scalability from single-qubit operations to multi-qubit circuits for quantum information processing requires architecture-specific implementations. Semiconductor hybrid qubit architecture is a suitable candidate to realize large-scale quantum information processing, as it combines a universal set of logic gates with fast and all-electrical manipulation of qubits. We propose an implementation of hybrid qubits, based on Si metal-oxide-semiconductor (MOS) quantum dots, compatible with the CMOS industrial technological standards. We discuss the realization of multi-qubit circuits capable of fault-tolerant computation and quantum error correction, by evaluating the time and space resources needed for their implementation. As a result, the maximum density of quantum information is extracted from a circuit including eight logical qubits encoded by the [[7, 1, 3]] Steane code. The corresponding surface density of logical qubits is 2.6 Mqubit/cm\(^2\). 相似文献
8.
Gualdi G Prati A Cucchiara R 《IEEE transactions on pattern analysis and machine intelligence》2012,34(8):1589-1604
The common paradigm employed for object detection is the sliding window (SW) search. This approach generates grid-distributed patches, at all possible positions and sizes, which are evaluated by a binary classifier: The tradeoff between computational burden and detection accuracy is the real critical point of sliding windows; several methods have been proposed to speed up the search such as adding complementary features. We propose a paradigm that differs from any previous approach since it casts object detection into a statistical-based search using a Monte Carlo sampling for estimating the likelihood density function with Gaussian kernels. The estimation relies on a multistage strategy where the proposal distribution is progressively refined by taking into account the feedback of the classifiers. The method can be easily plugged into a Bayesian-recursive framework to exploit the temporal coherency of the target objects in videos. Several tests on pedestrian and face detection, both on images and videos, with different types of classifiers (cascade of boosted classifiers, soft cascades, and SVM) and features (covariance matrices, Haar-like features, integral channel features, and histogram of oriented gradients) demonstrate that the proposed method provides higher detection rates and accuracy as well as a lower computational burden w.r.t. sliding window detection. 相似文献
9.
Cache performance is strongly influenced by the type of locality embodied in programs. In particular, multimedia programs handling images and videos are characterized by a bidimensional spatial locality, which is not adequately exploited by standard caches. In this paper we propose novel cache prefetching techniques for image data, called neighbor prefetching, able to improve exploitation of bidimensional spatial locality. A performance comparison is provided against other assessed prefetching techniques on a multimedia workload (with MPEG-2 and MPEG-4 decoding, image processing, and visual object segmentation), including a detailed evaluation of both the miss rate and the memory access time. Results prove that neighbor prefetching achieves a significant reduction in the time due to delayed memory cycles (more than 97% on MPEG-4 with respect to 75% of the second performing technique). This reduction leads to a substantial speedup on the overall memory access time (up to 140% for MPEG-4). Performance has been measured with the PRIMA trace-driven simulator, specifically devised to support cache prefetching. 相似文献
10.
Maria Luisa Introvigne Magdalena A. Taracila Prof. Fabio Prati Prof. Emilia Caselli Prof. Robert A. Bonomo 《ChemMedChem》2020,15(14):1283-1288
Boronic acids are known reversible covalent inhibitors of serine β-lactamases. The selectivity and high potency of specific boronates bearing an amide side chain that mimics the β-lactam's amide side chain have been advanced in several studies. Herein, we describe a new class of boronic acids in which the amide group is replaced by a bioisostere triazole. The boronic acids were obtained in a two-step synthesis that relies on the solid and versatile copper-catalyzed azide–alkyne cycloaddition (CuAAC) followed by boronate deprotection. All of the compounds show very good inhibition of the Klebsiella pneumoniae carbapenemase KPC-2, with Ki values ranging from 1 nM to 1 μM, and most of them are able to restore cefepime activity against K. pneumoniae harboring blaKPC-2. In particular, compound 1 e , bearing a sulfonamide substituted by a thiophene ring, proved to be an excellent KPC-2 inhibitor (Ki=30 nM); it restored cefepime susceptibility in KPC-Kpn cells (MIC=0.5 μg/mL) with values similar to that of vaborbactam (Ki=20 nM, MIC in KPC-Kpn 0.5 μg/mL). Our findings suggest that α-triazolylboronates might represent an effective scaffold for the treatment of KPC-mediated infections. 相似文献