全文获取类型
收费全文 | 196篇 |
免费 | 6篇 |
国内免费 | 11篇 |
专业分类
电工技术 | 14篇 |
化学工业 | 54篇 |
金属工艺 | 7篇 |
机械仪表 | 1篇 |
建筑科学 | 9篇 |
轻工业 | 3篇 |
无线电 | 26篇 |
一般工业技术 | 42篇 |
冶金工业 | 53篇 |
原子能技术 | 3篇 |
自动化技术 | 1篇 |
出版年
2021年 | 1篇 |
2020年 | 1篇 |
2018年 | 2篇 |
2017年 | 3篇 |
2016年 | 2篇 |
2015年 | 1篇 |
2014年 | 1篇 |
2013年 | 9篇 |
2012年 | 8篇 |
2011年 | 4篇 |
2010年 | 8篇 |
2009年 | 8篇 |
2008年 | 9篇 |
2007年 | 7篇 |
2006年 | 11篇 |
2005年 | 5篇 |
2004年 | 4篇 |
2003年 | 4篇 |
2002年 | 7篇 |
2001年 | 3篇 |
2000年 | 4篇 |
1998年 | 22篇 |
1997年 | 11篇 |
1996年 | 9篇 |
1995年 | 5篇 |
1994年 | 10篇 |
1993年 | 8篇 |
1992年 | 3篇 |
1991年 | 5篇 |
1990年 | 3篇 |
1989年 | 1篇 |
1988年 | 1篇 |
1987年 | 5篇 |
1986年 | 7篇 |
1985年 | 5篇 |
1984年 | 2篇 |
1983年 | 2篇 |
1982年 | 5篇 |
1981年 | 1篇 |
1980年 | 1篇 |
1977年 | 1篇 |
1976年 | 2篇 |
1972年 | 1篇 |
1969年 | 1篇 |
排序方式: 共有213条查询结果,搜索用时 15 毫秒
1.
A new type of arc plasma reactor with 12-phase alternating current (AC) discharge for synthesis of carbon nanotubes (CNTs) is proposed. A couple of six discharge electrodes by which have mutually electrical connection between them to enlarge the high-temperature regions in the reactor are arranged to three-dimensional locations. A new method of CNTs fabrication by this reactor, which accomplishes to enlarge the suitable growth region in high purity and at high yield, was developed. 相似文献
2.
Crystallization of potassium titanate from the amorphous phase 总被引:1,自引:0,他引:1
Tadashi Endo Hiroyuki Nagayama Tsugio Sato Masahiko Shimada 《Journal of Materials Science》1988,23(2):694-698
By using amorphous potassium titanates as the starting materials, a sintered body of K2Ti4O9 or K2Ti6O13 with porous and fibrous textures was prepared. K2Ti2O5 and a new phase, K6Ti4O11 were synthesized by the thermal reaction of KNO3 with TiO2 at 1000° C for 10 to 20 h. On leaching in water to expel excess of potassium ions, both phases became amorphous. After mixing and moulding these amorphous materials in the desired proportion, a sintered body containing fibrous crystals of K2Ti4O9 was readily fabricated by heating at 1000° C for 12 h. When 5 wt % B2O3 was added to the amorphous phases, single phase K2Ti6O13, with a fibrous texture grew well on heating at 1000° C for 12 h. Addition of PVA polymer to the amorphous phases was responsible for controlling the porosity of the sintered body, e.g. about 52% theoretical density at 20 wt% PVA polymer. The optimum conditions for preparing the amorphous phases were systematically examined and the effect of the chemical reaction environments, such as different crucible materials on the calcination of KNO3 and TiO2 were also discussed. 相似文献
3.
CARBON ORDERING IN Fe-1.83C MARTENSITE Ⅰ. Crystal Structure of a Conventional Ordered Phase 总被引:1,自引:0,他引:1
采用电子衍射方法对Fe-1.83C马氏体室温时效时产生的有序相结构进行研究,确定其结构为偏离化学计量成分Fe_4C的γ′-Fe_4结构,称为γ′-Fe_xC(Ⅰ)(x=4-11)。碳原子位于单胞的1/2,1/2,1/2位置。该有序相单胞尺寸为:(a_M,c_M分别为马氏体单胞的a和c轴长度),它与母相完全共格,位向关系为(001)_Ⅰ∥(001)_M,[100]_Ⅰ∥[110]_M。根据γ′-Fe_xC(Ⅰ)晶体结构计算出的有序相衍射花样与实验得到的衍射花样全部吻合。 相似文献
4.
Tsugio Sato Kenji Dosaka Toshiaki Yoshioka Akitsugu Okuwaki Kazuo Torii Yoshiro Onodera 《Journal of the American Ceramic Society》1992,75(3):552-556
Amorphous CeO2 –ZrO2 gels were prepared by coprecipitation in ammonia solutions. The onset of crystallization of the gels, from calcining in air, was 420°C, while 200° to 250°C in the presence of water and organic solvents such as methanol and ethanol. The sintering behaviors of CeO2 –ZrO2 powders were sensitive to the crystallizing conditions, since hard agglomerates formed when the precipitated gels were crystallized by normal calcination in air, whereas soft agglomerates formed when they were crystallized in water or organic solvents. CeO2 –ZrO2 powders crystallized in methanol and water at 250°C were sintered to full theoretical density at 1150° and 1400°C, respectively, whereas that crystallized by calcination in air at 450°C was sintered to only 95.2% of theoretical density, even at 1500°C. 相似文献
5.
1 INTRODUCTION Since Cu-ZSM-5 was reported as an effective catalyst for the selective catalytic reduction (SCR) of NO by hydrocarbons in the presence of excess oxygen, the SCR of NOx has received much attention as a kind of potential technology for cleaning NOx in various oxygen-rich exhausts of diesel engine, lean burning gasoline engine and gas engine. Although a number of catalysts have been tested, to date, it still seems to be difficult to find a catalyst that is completely suit… 相似文献
6.
A gel polymer electrolyte based on poly(acrylonitrile-co-styrene) as polymer matrix and N-methyl pyridine iodide salt as I− source was prepared. Controlling the concentration of polymer matrix of poly(acrylonitrile-co-styrene) at 17.5 wt.%, mixing the binary organic solvents mixture ethylene carbonate and propylene carbonate with 6:4 (w/w), and the concentration of N-methyl pyridine iodide and iodine with 0.5 and 0.05 M, respectively, the gel polymer electrolyte attains the maximum ionic conductivity (at 30 °C) of 4.63 mS cm−1. Based on the gel polymer electrolyte, a quasi-solid state dye-sensitized solar cell was fabricated and its overall energy conversion efficiency of light-to-electricity of 3.10% was achieved under irradiation of 100 mW cm−2. 相似文献
7.
Takeo Uchida Keita Abe Yuma Endo Shosei Ichiseki Satoru Akita Shiyun Liu Sho Aradachi Masataka Saito Akihiko Fukuchi Taiyo Kikkawa Theo Dammaretz Ibuki Kawamata Yuki Suzuki Shin‐ichiro M. Nomura Satoshi Murata 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(41)
A new kind of the Vernier mechanism that is able to control the size of linear assembly of DNA origami nanostructures is proposed. The mechanism is realized by mechanical design of DNA origami, which consists of a hollow cylinder and a rotatable shaft in it connected through the same scaffold. This nanostructure stacks with each other by the shape complementarity at its top and bottom surfaces of the cylinder, while the number of stacking is limited by twisting angle of the shaft. Experiments have shown that the size distribution of multimeric assembly of the origami depends on the twisting angle of the shaft; the average lengths of the multimer are decamer, hexamer, and tetramer for 0°, 10°, and 20° twist, respectively. In summary, it is possible to affect the number of polymerization by adjusting the precise shape and movability of a molecular structure. 相似文献
8.
Peeramed Chodkaveekityada Hajime Fukuchi 《International Journal of Satellite Communications and Networking》2017,35(4):281-293
The effects of rain attenuation on communication systems will become more pronounced in future satellite communication systems, especially with the planned use of the 21‐GHz band or higher‐frequency bands. Diversity techniques provide a solution to mitigate rain attenuation effects. This study proposes a time diversity technique, one such technique that is likely to demonstrate high effectiveness. To model the system, rainfall rate statistics are necessary, and reliability is improved as the amount of statistical data increases. This paper derives the cumulative distribution of the rainfall rate across Japan over 4 years using rain radar data from the automated meteorological data acquisition system and ground‐based rain radar network and evaluates the rainfall rate at 23 observation points across Japan. We carry out a performance evaluation for all locations within Japan to confirm the efficiency of the time diversity method. Finally, we propose prediction model of the time diversity gain for Japan and other significant parameter which is time correlation of rainfall rate that was found from the time diversity results for further investigation. Copyright © 2016 John Wiley & Sons, Ltd. 相似文献
9.
Hiroyuki Yamada Atsushi Tsurumaki‐Fukuchi Masaki Kobayashi Takuro Nagai Yoshikiyo Toyosaki Hiroshi Kumigashira Akihito Sawa 《Advanced functional materials》2015,25(18):2708-2714
Tunnel electroresistance in ferroelectric tunnel junctions (FTJs) has attracted considerable interest, because of a promising application to nonvolatile memories. Development of ferroelectric thin‐film devices requires atomic‐scale band‐structure engineering based on depolarization‐field effects at interfaces. By using FTJs consisting of ultrathin layers of the prototypical ferroelectric BaTiO3, it is demonstrated that the surface termination of the ferroelectric in contact with a simple‐metal electrode critically affects properties of electroresistance. BaTiO3 barrier‐layers with TiO2 or BaO terminations show opposing relationships between the polarization direction and the resistance state. The resistance‐switching ratio in the junctions can be remarkably enhanced up to 105% at room temperature, by artificially controlling the fraction of BaO termination. These results are explained in terms of the termination dependence of the depolarization field that is generated by a dead layer and imperfect charge screening. The findings on the mechanism of tunnel electroresistance should lead to performance improvements in the devices based on nanoscale ferroelectrics. 相似文献
10.
Makoto Hamanaka Kimie Imakawa Mizuki Yoshida Zhihuan Zhao Shu Yin Xiaoyong Wu Yunfang Huang Jihuai Wu Tsugio Sato 《Journal of Porous Materials》2016,23(5):1189-1196
The SnO2 particles with different morphologies of nanorod, nanosheet, nanoparticle and nanodot were synthesized by liquid-phase methods. In addition, Pt was loaded on each prepared SnO2 by dispersing SnO2 particles into PtCl4 2? aqueous solutions containing 0.67 vol% methanol, followed by UV light irradiation for 6 h. The products were characterized by X-ray diffraction, scanning electron microscopy, transmission electron microscopy, and Brunauer–Emmett–Teller measurement. The gas sensing properties of the synthesized SnO2 were tested by detecting the change in electric resistivity in flowing aceton and methanol gases with nitrogen base. The gas sensing properties greatly changed depending on not only the specific surface area, but also the exposed crystal plane, i.e., the SnO2 nanorods exposing (111) planes showed the excellent sensitivity and quick response ability, indicating the excellent gas sensing ability of the (111) plane. Furthermore, the Pt loading exceedingly enhanced the gas sensing properties. 相似文献