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1.
David J. Lawrence Brianna L. Smith Cameron D. Collard Keyton A. Elliott Kyle L. Fakhoury Jeffery D. Mangold Anna N. Soyka 《International Journal of Hydrogen Energy》2021,46(2):1642-1655
Monolithically-integrated tandem photoanodes were fabricated on substrates consisting of epitaxial n-GaAs1-xPx (x ? 0.32) grown on n+-GaAs wafers. A p+-n junction photovoltaic (PV) cell was first formed by zinc diffusion into the n-GaAs0.68P0.32 from a deposited ZnO coating. After diffusion the ZnO serves as a transparent electrical contact to the resulting p+-GaAs0.68P0.32 surface layer. Transparent, conducting SnO2:F provides chemical and mechanical protection for the ZnO and the underlying PV cell, and it electrically connects this cell to a top BiVO4 photocatalyst layer. In some photoanodes, a WO3 thin film was interposed between the SnO2:F and BiVO4. All oxide coatings were produced by ultrasonic spray pyrolysis except WO3, which was spin coated. Unassisted (unbiased) solar water splitting was achieved, with a solar-to-hydrogen efficiency approaching 2%, without addition of any co-catalyst to the BiVO4 surface. This work can provide insights to other researchers regarding scalable, low cost approaches for the planar monolithic integration of oxide photoanode materials with PV cells to create new tandem devices. 相似文献
2.
Topic models are a useful and ubiquitous tool for understanding large corpora. However, topic models are not perfect, and for many users in computational social science, digital humanities, and information studies—who are not machine learning experts—existing models and frameworks are often a “take it or leave it” proposition. This paper presents a mechanism for giving users a voice by encoding users’ feedback to topic models as correlations between words into a topic model. This framework, interactive topic modeling (itm), allows untrained users to encode their feedback easily and iteratively into the topic models. Because latency in interactive systems is crucial, we develop more efficient inference algorithms for tree-based topic models. We validate the framework both with simulated and real users. 相似文献
3.
Brianna L. Musicó Quinton Wright Cordell Delzer T. Zac Ward Claudia J. Rawn David G. Mandrus Veerle Keppens 《Journal of the American Ceramic Society》2021,104(7):3750-3759
The multicomponent approach has been successfully expanded to the Ruddlesden–Popper structure with the synthesis of two different high-entropy cuprate compositions: (La0.2Nd0.2Gd0.2Tb0.2Dy0.2)2CuO4 and (La0.2Pr0.2Nd0.2Sm0.2Eu0.2)2CuO4. The effect of synthesis method is explored using both solid-state reaction and polymeric steric entrapment (PSE) methods. It is found that PSE leads to more randomly distributed cation species, providing an advantageous method of synthesis for the growing field of high entropy oxides. In situ high-temperature x-ray diffraction tracks the amorphous to crystalline phase transformation in (La0.2Nd0.2Gd0.2Tb0.2Dy0.2)2CuO4 powder, synthesized using the PSE method. Using the High-Temperature XRD data, a method for gaining information on the kinetic behavior is also applied. Magnetometry of both compositions indicates ferrimagnetic behavior at low temperatures. 相似文献
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Naglieri Jack A.; De Lauder Brianna Y.; Goldstein Sam; Schwebech Adam 《Canadian Metallurgical Quarterly》2006,21(1):62
The relationships between Wechsler Intelligence Scale for Children-Third Edition (WISC-III) and the Cognitive Assessment System (CAS) with the Woodcock-Johnson Tests of Achievement (WJ-III) were examined for a sample of 119 children (87 males and 32 females) ages 6 to 16. The sample was comprised of children who were referred to a specialty clinic for evaluation. Participants were administered the WISC-III, the CAS, and the WJ-III, in that order. Results indicated that CAS/WJ-III correlations were consistently significantly higher than those found for the WISC-III/WJ-III. The four separate CAS scales added more variance above and beyond the four separate WISC-III scales than the WISC-III added above and beyond the CAS. In addition, the CAS Full Scale accounted for more unique variance and was a stronger predictor of WJ-III Academic Skills Cluster than the WISC-III Full Scale IQ. These results support the validity of the Planning, Attention, Simultaneous, and Successive theory as measured by the CAS in relation to the general intelligence model measured using the WISC-III for explaining variance in achievement for this clinical sample. (PsycINFO Database Record (c) 2011 APA, all rights reserved) 相似文献
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Brianna E. George Monica H. Dawes Emily G. Peck Sara R. Jones 《International journal of molecular sciences》2022,23(15)
Administration of heroin results in the engagement of multiple brain regions and the rewarding and addictive effects are mediated, at least partially, through activation of the mesolimbic dopamine system. However, less is known about dopamine system function following chronic exposure to heroin. Withdrawal from chronic heroin exposure is likely to drive a state of low dopamine in the nucleus accumbens (NAc), as previously observed during withdrawal from other drug classes. Thus, we aimed to investigate alterations in NAc dopamine terminal function following chronic heroin self-administration to identify a mechanism for dopaminergic adaptations. Adult male Long Evans rats were trained to self-administer heroin (0.05 mg/kg/inf, IV) and then placed on a long access (FR1, 6-h, unlimited inf, 0.05 mg/kg/inf) protocol to induce escalation of intake. Following heroin self-administration, rats had decreased basal extracellular levels of dopamine and blunted dopamine response following a heroin challenge (0.1 mg/kg/inf, IV) in the NAc compared to saline controls. FSCV revealed that heroin-exposed rats exhibited reduced stimulated dopamine release during tonic-like, single-pulse stimulations, but increased phasic-like dopamine release during multi-pulse stimulation trains (5 pulses, 5–100 Hz) in addition to an altered dynamic range of release stimulation intensities when compared to controls. Further, we found that presynaptic D3 autoreceptor and kappa-opioid receptor agonist responsivity were increased following heroin self-administration. These results reveal a marked low dopamine state following heroin exposure and suggest the combination of altered dopamine release dynamics may contribute to increased heroin seeking. 相似文献
8.
Jason Cory Brunson Steve Fassino Antonio McInnes Monisha Narayan Brianna Richardson Christopher Franck Patrick Ion Reinhard Laubenbacher 《Scientometrics》2014,99(3):973-998
This study examines long-term trends and shifting behavior in the collaboration network of mathematics literature, using a subset of data from Mathematical Reviews spanning 1985–2009. Rather than modeling the network cumulatively, this study traces the evolution of the “here and now” using fixed-duration sliding windows. The analysis uses a suite of common network diagnostics, including the distributions of degrees, distances, and clustering, to track network structure. Several random models that call these diagnostics as parameters help tease them apart as factors from the values of others. Some behaviors are consistent over the entire interval, but most diagnostics indicate that the network’s structural evolution is dominated by occasional dramatic shifts in otherwise steady trends. These behaviors are not distributed evenly across the network; stark differences in evolution can be observed between two major subnetworks, loosely thought of as “pure” and “applied”, which approximately partition the aggregate. The paper characterizes two major events along the mathematics network trajectory and discusses possible explanatory factors. 相似文献
9.
The effectiveness of ozone and acidulant treatments in extending the refrigerated shelf life of fresh-cut potatoes 总被引:1,自引:0,他引:1
Calder BL Skonberg DI Davis-Dentici K Hughes BH Bolton JC 《Journal of food science》2011,76(8):S492-S498
Abstract: The objective of the study was to determine the effectiveness of acidulant dip treatments (with or without aqueous ozone) to reduce enzymatic browning and to extend the shelf life of fresh‐cut potato slices during refrigerated storage (4 °C) for 28 d. Potato slices subjected to aqueous ozone (2 ppm) had significantly (P≤ 0.05) higher L‐values and lower a‐values, but ozone did not appear to have any effect on aerobic plate counts (APCs) or polyphenol oxidase (PPO) activity. NatureSeal (NS) and sodium acid sulfate (SAS) were the most effective acidulant treatments in reducing browning (significantly [P≤ 0.05] higher L‐values, lower a‐values, and browning index values) regardless of ozone treatment. NS and SAS also had lower PPO activity compared to other treatments on days 0 and 28, and significantly (P≤ 0.05) lower APCs (≤2.00 log CFU/g) over refrigerated storage. Therefore, the SAS treatment was comparable to NS, a commercially available product, and showed promise as an effective antibrowning dip to reduce browning and spoilage in fresh‐cut potato products. Practical Application: A 1% SAS dip treatment which included 1% citric and 1% ascorbic acid was found to be an effective antibrowning dip for fresh‐cut potatoes along with NatureSeal®'s PS‐10, compared to other treatments. They were both effective in maintaining low microbial counts over refrigerated storage. Additionally, aqueous ozone washes (2 ppm) showed significant benefits to reduce browning; however, ozone did not affect microbial counts or PPO enzyme activity. Therefore, the SAS treatment could have potential use in the fruit and vegetable industry to reduce browning and spoilage in fresh‐cut potato products. 相似文献
10.
A. Pollatsek, E. D. Reichle, and K. Rayner (see record 2006-22004-014) argue that the critical findings in A. W. Inhoff, B. M. Eiter, and R. Radach (see record 2005-13471-012) are in general agreement with core assumptions of sequential attention shift models if additional assumptions and facts are considered. The current authors critically discuss the hypothesized time line of processing and indicate that the success of Pollatsek et al.'s simulation is predicated on a gross underestimation of the pretarget word's viewing duration in Inhoff et al. and that the actual data are difficult to reconcile with the strictly serial attention shift assumption. The authors also discuss attention shifting and saccade programming assumptions in the E-Z Reader model and conclude that these are not in harmony with research in related domains of study. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献