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Gradient-corrected density functional theory was used to investigate the adsorption of H2S on Pd(1 1 1) surface. Molecular adsorption was found to be stable with H2S binding preferentially at top sites. In addition, the adsorption of other S moieties (SH and S) was investigated. SH and S were found to be preferentially bind at the bridge and fcc sites, respectively. The reaction pathways and energy profiles for H2S decomposition giving rise to adsorbed S and H were determined. Both H2S(ad) → SH(ad) + H(ad) and SH(ad) → S(ad) + H(ad) reactions were found to have low barriers and high exothermicities. This reveals that the decomposition of H2S on Pd(1 1 1) surface is a facile process. 相似文献
3.
Integrated Microfluidic CustomArray Device for Bacterial Genotyping and Identification 总被引:2,自引:0,他引:2
4.
Peter K. Windsor Stephen P. Plassmeyer Dominic S. Mattock Jonathan C. Bradfield Erika Y. Choi Bill R. Miller III Byung Hee Han 《International journal of molecular sciences》2021,22(6)
Deposition of amyloid β (Aβ) fibrils in the brain is a key pathologic hallmark of Alzheimer’s disease. A class of polyphenolic biflavonoids is known to have anti-amyloidogenic effects by inhibiting aggregation of Aβ and promoting disaggregation of Aβ fibrils. In the present study, we further sought to investigate the structural basis of the Aβ disaggregating activity of biflavonoids and their interactions at the atomic level. A thioflavin T (ThT) fluorescence assay revealed that amentoflavone-type biflavonoids promote disaggregation of Aβ fibrils with varying potency due to specific structural differences. The computational analysis herein provides the first atomistic details for the mechanism of Aβ disaggregation by biflavonoids. Molecular docking analysis showed that biflavonoids preferentially bind to the aromatic-rich, partially ordered N-termini of Aβ fibril via the π–π interactions. Moreover, docking scores correlate well with the ThT EC50 values. Molecular dynamic simulations revealed that biflavonoids decrease the content of β-sheet in Aβ fibril in a structure-dependent manner. Hydrogen bond analysis further supported that the substitution of hydroxyl groups capable of hydrogen bond formation at two positions on the biflavonoid scaffold leads to significantly disaggregation of Aβ fibrils. Taken together, our data indicate that biflavonoids promote disaggregation of Aβ fibrils due to their ability to disrupt the fibril structure, suggesting biflavonoids as a lead class of compounds to develop a therapeutic agent for Alzheimer’s disease. 相似文献
5.
Dominic D. J. Chandar Jayanarayanan Sitaraman Dimitri Mavriplis 《The Journal of supercomputing》2014,67(1):47-68
The application of graphics processing units (GPU) to solve partial differential equations is gaining popularity with the advent of improved computer hardware. Various lower level interfaces exist that allow the user to access GPU specific functions. One such interface is NVIDIA’s Compute Unified Device Architecture (CUDA) library. However, porting existing codes to run on the GPU requires the user to write kernels that execute on multiple cores, in the form of Single Instruction Multiple Data (SIMD). In the present work, a higher level framework, termed CU++, has been developed that uses object oriented programming techniques available in C++ such as polymorphism, operator overloading, and template meta programming. Using this approach, CUDA kernels can be generated automatically during compile time. Briefly, CU++ allows a code developer with just C/C++ knowledge to write computer programs that will execute on the GPU without any knowledge of specific programming techniques in CUDA. This approach is tremendously beneficial for Computational Fluid Dynamics (CFD) code development because it mitigates the necessity of creating hundreds of GPU kernels for various purposes. In its current form, CU++ provides a framework for parallel array arithmetic, simplified data structures to interface with the GPU, and smart array indexing. An implementation of heterogeneous parallelism, i.e., utilizing multiple GPUs to simultaneously process a partitioned grid system with communication at the interfaces using Message Passing Interface (MPI) has been developed and tested. 相似文献
6.
Erica Glatt Dominic Pjontek Craig McKnight Jason Wiens Michael Wormsbecker Jennifer McMillan 《加拿大化工杂志》2021,99(1):209-221
FLUID COKING is a continuous process that thermally converts heavy hydrocarbons, such as oil sands bitumen, to lighter and higher‐value products by horizontal spray injection onto a fluidized bed of hot coke particles. The cyclone sections of commercial fluid coker reactors experience fouling during typical operation, which limits unit run lengths. The main objective of this work is to improve fluid coker reliability by proposing cyclone fouling mitigation strategies based on practical operation modifications. This study developed a process simulation in Aspen Plus to establish the combined impact of vapour‐liquid equilibrium, endothermic thermal cracking reactions, pressure changes, and overall fluid dynamics in the selected fluid coker control volumes. The hydrocarbon composition was defined by applying an assay characterization of distillation data for representative hydrocarbon streams. Case studies were performed to determine the sensitivity of the predicted temperatures and hydrocarbon condensate flow rates for: (a) the burner‐to‐fluid coker transfer line temperature; (b) the hot coke flow rate; (c) hot coke entrainment from the freeboard region; and (d) scouring coke flow rate in the horn chamber. The scouring coke flow rate was identified as the most promising process lever to mitigate fluid coker cyclone fouling. 相似文献
7.
Seena K. Thomas P. M. Sabura Begum C. D. Midhun Dominic Nisa V. Salim Nishar Hameed Sanjay Mavinkere Rangappa Suchart Siengchin Jyotishkumar Parameswaranpillai 《应用聚合物科学杂志》2021,138(15):50213
Acacia caesia (L.) Willd (soap bark) fiber is an abundant natural resource, that is rich in cellulose. The study reports the effective utilization of underutilized Acacia caesia fiber for the isolation of nanocellulose whiskers. The nanocellulose whiskers were isolated successfully from Acacia caesia fibers by following alkali, bleaching, and sulfuric acid treatment. The obtained nanocellulose whiskers were carefully investigated for its chemical composition, structure, morphology, crystallinity, and thermal stability. The chemical composition and Fourier transform infrared spectra of nanocellulose whiskers showed the elimination of the non-cellulosic parts present in the raw Acacia caesia fibers. The X-ray diffraction analysis showed an upsurge in the crystallinity of the cellulose fibers after the chemical treatments. The isolation of nanocellulose whiskers from Acacia caesia raw fiber was confirmed by electron microscopy analysis. The thermogravimetric analysis showed remarkably high char residue for the nanocellulose whiskers compared to raw fibers. Based on the properties of nanocellulose whiskers, it can be concluded that the nanocellulose whiskers produced from Acacia caesia raw fibers are potential reinforcing material for developing high-performance green composites. 相似文献
8.
Abstract This article reports findings of a study of how leaders of virtual information systems development teams improve team trust and cooperation by managing adaptation of information and communications tools. Results indicate how Theory X (command and control) and Theory Y (facilitate and support) styles of leadership enable and hinder effective outcomes. 相似文献
9.
Mayuresh Patole Santanu Bandyopadhyay Dominic C. Y. Foo Raymond R. Tan 《Clean Technologies and Environmental Policy》2017,19(7):1967-1975
Pinch analysis was initially developed as a methodology for optimizing energy efficiency in process plants. Applications of pinch analysis applications are based on common principles of using stream quantity and quality to determine optimal system targets. This initial targeting step identifies the pinch point, which then allows complex problems to be decomposed for the subsequent design of an optimal network using insights drawn from the targeting stage. One important class of pinch analysis problems is energy planning with footprint constraints, which began with the development of carbon emissions pinch analysis; in such problems, energy sources and demands are characterized by carbon footprint as the quality index. This methodology has been extended by using alternative quality indexes that measure different sustainability dimensions, such as water footprint, land footprint, emergy transformity, inoperability risk, energy return on investment and human fatalities. Pinch analysis variants still have the limitation of being able to use one quality index at a time, while previous attempts to develop pinch analysis methods using multiple indices have only been partially successful for special cases. In this work, a multiple-index pinch analysis method is developed by using an aggregate quality index, based on a weighted linear function of different quality indexes normally used in energy planning. The weights used to compute the aggregate index are determined via the analytic hierarchy process. A case study for Indian power sector is solved to illustrate how this approach allows multiple sustainability dimensions to be accounted for in energy planning. 相似文献
10.
Gregory K Miller David A Petti Dominic J Varacalle Jr. John T Maki 《Journal of Nuclear Materials》2003,317(1):69-82
The fundamental design for a gas-cooled reactor relies on the behavior of the coated particle fuel. The coating layers, termed the TRISO coating, act as a mini-pressure vessel that retains fission products. Results of US irradiation experiments show that many more fuel particles have failed than can be attributed to one-dimensional pressure vessel failures alone. Post-irradiation examinations indicate that multi-dimensional effects, such as the presence of irradiation-induced shrinkage cracks in the inner pyrolytic carbon layer, contribute to these failures. To address these effects, the methods of prior one-dimensional models are expanded to capture the stress intensification associated with multi-dimensional behavior. An approximation of the stress levels enables the treatment of statistical variations in numerous design parameters and Monte Carlo sampling over a large number of particles. The approach is shown to make reasonable predictions when used to calculate failure probabilities for irradiation experiments of the New Production - Modular High Temperature Gas Cooled Reactor Program. 相似文献