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High‐Performance Integrated Perovskite and Organic Solar Cells with Enhanced Fill Factors and Near‐Infrared Harvesting 下载免费PDF全文
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Zhi Jiang Kenjiro Fukuda Wenchao Huang Sungjun Park Roda Nur Md. Osman Goni Nayeem Kilho Yu Daishi Inoue Masahiko Saito Hiroki Kimura Tomoyuki Yokota Shinjiro Umezu Daisuke Hashizume Itaru Osaka Kazuo Takimiya Takao Someya 《Advanced functional materials》2019,29(6)
Flexible and stretchable organic photovoltaics (OPVs) are promising as a power source for wearable devices with multifunctions ranging from sensing to locomotion. Achieving mechanical robustness and high power conversion efficiency for ultraflexible OPVs is essential for their successful application. However, it is challenging to simultaneously achieve these features by the difficulty to maintain stable performance under a microscale bending radius. Ultraflexible OPVs are proposed by employing a novel metal‐oxide‐free cathode that consists of a printed ultrathin metallic transparent electrode and an organic electron transport layer to achieve high electron‐collecting capabilities and mechanical robustness. In fact, the proposed ultraflexible OPV achieves a power conversion efficiency of 9.7% and durability with 74% efficiency retention after 500 cycles of deformation at 37% compression through buckling. The proposed approach can be applied to active layers with different morphologies, thus suggesting its universality and potential for high‐performance ultraflexible OPV devices. 相似文献
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Gyudo Lee Hyungbeen Lee Kihwan Nam Jae-Hee Han Jaemoon Yang Sang Woo Lee Dae Sung Yoon Kilho Eom Taeyun Kwon 《Nanoscale research letters》2012,7(1):1-11
Core/shell nanostructured carbon materials with carbon nanofiber (CNF) as the core and a nitrogen (N)-doped graphitic layer as the shell were synthesized by pyrolysis of CNF/polyaniline (CNF/PANI) composites prepared by in situ polymerization of aniline on CNFs. High-resolution transmission electron microscopy (TEM), X-ray diffraction (XRD), Fourier transform infrared and Raman analyses indicated that the PANI shell was carbonized at 900°C. Platinum (Pt) nanoparticles were reduced by formic acid with catalyst supports. Compared to the untreated CNF/PANI composites, the carbonized composites were proven to be better supporting materials for the Pt nanocatalysts and showed superior performance as catalyst supports for methanol electrochemical oxidation. The current density of methanol oxidation on the catalyst with the core/shell nanostructured carbon materials is approximately seven times of that on the catalyst with CNF/PANI support. TEM tomography revealed that some Pt nanoparticles were embedded in the PANI shells of the CNF/PANI composites, which might decrease the electrocatalyst activity. TEM-energy dispersive spectroscopy mapping confirmed that the Pt nanoparticles in the inner tube of N-doped hollow CNFs could be accessed by the Nafion ionomer electrolyte, contributing to the catalytic oxidation of methanol. 相似文献
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This paper concerns the application of component mode synthesis for biomolecule modeling to understand protein dynamics. As for protein dynamics, eigenvalue problem should be formulated to obtain eigenvalue, eigenvector and thermal fluctuation. To describe the thermal fluctuation of protein, normal mode analysis is introduced and normal modes identify the dynamic behavior of protein very well. Component mode synthesis considers the given complex structure as an assembly of smaller components. The selection of a component may be arbitrary. When the component mode synthesis is applied to formulate the eigenvalue problem of protein structure, we selected a protein which may be composed of two and/or four domains. The domain of protein can be considered as a component. In this sense the number of component is increased as necessary, and the size of each component is decreased for fast calculation. The component mode synthesis widely used in engineering was well applied to understand protein dynamics in present study. 相似文献
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Young-Soo Sohn Jinsung Park Gwonchan Yoon Jiseok Song Sang-Won Jee Jung-Ho Lee Sungsoo Na Taeyun Kwon Kilho Eom 《Nanoscale research letters》2010,5(1):211-216
Nanowires have been taken much attention as a nanoscale building block, which can perform the excellent mechanical function as an electromechanical device. Here, we have performed atomic force microscope (AFM)-based nanoindentation experiments of silicon nanowires in order to investigate the mechanical properties of silicon nanowires. It is shown that stiffness of nanowires is well described by Hertz theory and that elastic modulus of silicon nanowires with various diameters from ~100 to ~600 nm is close to that of bulk silicon. This implies that the elastic modulus of silicon nanowires is independent of their diameters if the diameter is larger than 100 nm. This supports that finite size effect (due to surface effect) does not play a role on elastic behavior of silicon nanowires with diameter of >100 nm. 相似文献
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Kilho Eom Jeong-Hee Ahn Jae-In Kim Gwon-Chan Yoon Sungsoo Na 《Journal of Mechanical Science and Technology》2008,22(3):506-513
A dynamic model applicable to biomolecular structures for understanding the dynamics and the vibrational behaviors of protein
is considered. A mechanical mass-spring model represented by point masses and harmonic springs is presented. The biomolecular
structure may be envisioned by a mass and spring system with multi-degrees-of-freedom because dominant atoms in protein may
be considered to be point masses, and bonding and non-bonding interactions between atoms of interest and surrounding atoms
within some critical distances are implemented by a spring. Furthermore, a model condensation scheme is to be introduced because
most proteins have large degree of freedom requiring large computation time and memory, which results in reducing computational
cost and maintaining the accurate predictions. From solving the corresponding eigenvalue problem constructed from a multi-degree-of-freedom
system, our results show the modified mechanical spring-mass model of a biostructure through a condensation scheme is very
successful in predicting the dynamics of molecular structures in terms of thermal fluctuations and eigenmode, etc. 相似文献