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Auguste Commeyras Hlne Collet Laurent Boiteau Jacques Taillades Odile Vandenabeele‐Trambouze Herv Cottet Jean‐Philippe Biron Raphaël Plasson Louis Mion Olivier Lagrille Herv Martin Franck Selsis Michel Dobrijevic 《Polymer International》2002,51(7):661-665
Addressing the still open question of the prebiotic origin of sequential macromolecules (peptides, nucleic acids) on the primitive Earth, we describe a molecular engine (the primary pump), which works at ambient temperature and continuously generates, elongates and complexifies sequential peptides. This new scenario is based on a cyclic reaction sequence, whose keystep is the activation of amino acids into their N‐carboxyanhydrides (NCA) through nitrosation by NOx. This process could have taken place on tidal beaches; it requires a buffered ocean, emerged land and a nitrosating atmosphere. With the help of geochemical studies and computer simulations of atmosphere photochemistry, we show that the primitive Earth during the Hadean may have satisfied all these requirements. © 2001 Society of Chemical Industry. 相似文献
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An optical nondestructive strain measurement technique was performed to analyze the mechanical deformation induced by an electrical field within the insulating materials. Poly(ethylene naphthalene 2,6‐dicarboxylate) (PEN) films were then subjected to constant electrical fields right up to their electrical breakdown. The experimental technique made it possible to follow the various stages of the mechanical behavior of PEN in real time. The final breakdown occurred in the observation zone and the related mechanical deformation was captured. A “margarita” structure was observed with a hole at the center. The experimental results indicated that the level of the induced‐mechanical deformations depended on the local environment. We defined two different zones representing the inside and the outside of the damaged area. The induced‐deformations were larger in the damaged zone. It was also observed that deformations increased when the sample had a lower degree of crystallinity. © 2008 Wiley Periodicals, Inc. J Appl Polym Sci, 2008 相似文献
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The effect of pressure on transition displacement between trickle and pulsed regimes (TPR: trickle-pulsed transition) in catalytic trickle bed reactors (CTBR) is not properly predicted by existing theoretical models and empirical correlations. Based on high pressure TPR data available to date, a modified Charpentier diagram is proposed to quantify directly the effect of pressure in non-foaming systems. 相似文献
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Mohamed S. Belhaj Andr Laurent Noë l Midoux Jean-Claude Charpentier 《Chemical Engineering Communications》1981,10(4):261-267
Solubilities and diffusivities of carbon dioxide and nitrous oxide in a mixture of toluene and isopropanol organic solution of cyclohexylamine were measured at 20°C in the range of pressures of solute from 1 to 3 bars. This was performed with an original chromatographic technique taking into account the presence of the product of the reaction. 相似文献
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A. Storck M. A. Latifi G. Barthole A. Laurent J. C. Charpentier 《Journal of Applied Electrochemistry》1986,16(6):947-963
Hydrodynamic and mass transfer parameters (pressure drop, gas and liquid hold-up, liquid-solid mass transfer coefficients) have been measured for porous electrodes with upward or downward co-current gas-liquid flow by means of several electrochemical techniques. The influence of the most important parameters (packing diameter, gas and liquid flow rates) and of the hydrodynamic flow regimes, has been studied. It is found that in the trickle flow regime the limiting current densities depend only on the liquid flow rates (with no measurable influence of the gas). In the upward flow configuration, the strong turbulence generated by the ascending gas bubbles leads to a sharp increase of current densities with the gas flow rate. A comparison between both configurations is presented. 相似文献
9.
Pons MN Potier O Pontvianne S Laurent N France X Battaglia P 《Water science and technology》2011,64(3):602-609
In order to characterize the pollution discharged into the Moselle River and some of its tributaries, spectroscopic techniques, namely UV-vis spectroscopy and synchronous fluorescence spectroscopy, have been combined. UV-visible spectra were analysed using the maximum of the second derivative at 225 nm (related to nitrates), the SUVA254 and E2/E3 indices (related to the nature of organic matter). Synchronous fluorescence spectra (delta lambda = 50 nm) presented different shapes depending upon the type of pollution. The pollution results from anthropogenic activities: untreated domestic sewage due to misconnections in a periurban river, effluent from urban WWTPS, agricultural runoff (nitrates) in several streams, discharge from a paper mill (humic-like substances due to wood processing) and from steel mills (PAHs). 相似文献
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Fothergill J.C. Montanari G.C. Stevens G.C. Laurent C. Teyssedre G. Dissado L.A. Nilsson U.H. Platbrood G. 《Dielectrics and Electrical Insulation, IEEE Transactions on》2003,10(3):514-527
The aim of the European project "ARTEMIS" is to develop a diagnostic system for assessing aging in power cable insulation. Its first task was to make a thorough characterisation of the cable insulation before aging. This is intended to provide a background against which any changes introduced by thermo-electric aging can be identified. The aging markers derived from this initial characterisation will be considered both as diagnostic indicators in their own right, and also to develop an aging model for predictive purposes, if and when possible. This stage of the ARTEMIS programme is now complete and we will present an analysis of the results, and show how they may be correlated with the concepts proposed in aging theories. 相似文献