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排序方式: 共有57条查询结果,搜索用时 15 毫秒
1.
Reshef Tenne Ronit Popovitz-Biro Anton Twersky Yaron Rosenfeld Hacohen 《Israel journal of chemistry》2001,41(1):7-14
Nanoparticles of various layered compounds having a closed cage or nanotubular structure, designated also inorganic fullerene-like (IF) materials, have been reported in the past. In this work IF-CdCl2 nanoparticles were synthesized by two methods. In one technique, a high temperature evaporation and subsequent condensation of dried cadmium chloride powder was used. In the other method, electron beam irradiation of the source powder led to its recrystallization into closed nanoparticles with a nonhollow core. The two methods are shown to produce nanoparticles of different topologies. While mostly spherical nested structures are obtained from the high temperature process, polyhedra with hexagonal or elongated rectangular characters are obtained by the electron beam induced process. The analysis also shows that, while the source (dried) powder is orthorhombic cadmium chloride monohydrate, the crystallized IF cage consists of the anhydrous 3R polytype which is not stable as bulk material in ambient atmosphere. Consistent with previous observations, this study shows that the seamless structure of the IF materials can stabilize phases, which are otherwise unstable in ambient conditions. 相似文献
2.
Seung Hee Woo Lena Yadgarov Rita Rosentsveig Yuwon Park Daesun Song Reshef Tenne Sung You Hong 《Israel journal of chemistry》2015,55(5):599-603
Sodium ion batteries (SIBs) are considered as a promising alternative to threaten the reign of lithium ion batteries (LIBs) among various next-generation rechargeable energy storage systems, including magnesium ion, metal air, and metal sulfur batteries. Since both sodium and lithium are located in Group 1 of the periodic table, they share similar (electro)chemical properties with regard to ionization pattern, electronegativity, and electronic configuration; thus the vast number of compounds developed from LIBs can provide guidance to design electrode materials for SIBs. However, the larger ionic radius of the sodium cation and unique (de)sodiation processes may also lead to uncertainties in terms of thermodynamic or kinetic properties. Herein, we present the first construction of SIBs based on inorganic fullerene-like (IF) MoS2 nanoparticles. Closed-shell-type structures, represented by C60 fullerene, have largely been neglected for studies of alkali-metal hosting materials due to their inaccessibility for intercalating ions into the inner spaces. However, IF-MoS2, with faceted surfaces, can diffuse sodium ions through the defective channels, thereby allowing reversible sodium ion intercalation/deintercalation. Interestingly, Re-doped MoS2 showed good electrochemical performances with fast kinetics (ca. 74 mA h g−1 at 20 C). N-type doping caused by Re substitution of Mo in IF-MoS2 revealed enhanced electrical conductivity and an increased number of diffusion defect sites. Thus, chemical modification of fullerene-like structures through doping is proven to be a promising synthetic strategy to prepare improved electrodes. 相似文献
3.
Tenne R Rao CN 《Philosophical transactions. Series A, Mathematical, physical, and engineering sciences》2004,362(1823):2099-2125
Following the discovery of carbon fullerenes and carbon nanotubes, it was hypothesized that nanoparticles of inorganic compounds with layered (two-dimensional) structure, such as MoS(2), will not be stable against folding and form nanotubes and fullerene-like structures: IF. The synthesis of numerous other inorganic nanotubes has been reported in recent years. Various techniques for the synthesis of inorganic nanotubes, including high-temperature reactions and strategies based on 'chemie douce' (soft chemistry, i.e. low-temperature) processes, are described. First-principle, density functional theory based calculations are able to provide substantial information on the structure and properties of such nanotubes. Various properties of inorganic nanotubes, including mechanical, electronic and optical properties, are described in brief. Some potential applications of the nanotubes in tribology, protection against impact, (photo)catalysis, batteries, etc., are discussed. 相似文献
4.
A Reshef H Nissen L Triger TS Hensen O Eliav D Schurr R Safadi M Gare E Leitersdorf 《Canadian Metallurgical Quarterly》1996,98(5):581-586
Recreational SCUBA diving exposes individuals to environmental stresses not often encountered in other types of activity. These stresses include increased ambient pressure, raised partial pressure of O(2), increased resistance to movement, added weight and drag of diving equipment, cold stress, and a higher breathing resistance. One means to understand how such stresses affect a diver is to employ the stress-strain-adaptive response model. Physiologic adaptations, like an increase in VO(2) in response to cold stress, will minimize the strain placed on thermal balance. Nonphysiologic adaptive responses include those behavioral and equipment interventions that isolate the diver from a particular stress. Self-contained underwater breathing apparatus (SCUBA) isolates the diver from the inability to extract O(2) from the water; dive garments minimize the stress of cold water immersion. This review will focus on cardiorespiratory and thermal responses to SCUBA diving, using the stress-strain-adaptive response model to illustrate the interaction between diver and environment. Some responses like hyperventilation, cardiac arrhythmias, or cold injury due to vasoconstriction are not considered adaptive but are realistic possibilities in diving environments. 相似文献
5.
A multilink system consists of several full-duplex parallel links that carry data between two nodes. The authors construct a protocol-the multilink protocol (MLP)-that simulates a single full-duplex link system. They show that the multilink protocol proposed by the existing standard is not reliable, and they define a new multilink protocol that is proved to be reliable 相似文献
6.
7.
YA Mekori D Baram A Goldberg R Hershkoviz T Reshef D Sredni 《Canadian Metallurgical Quarterly》1993,91(3):817-824
Nedocromil sodium, a topical antiinflammatory agent recommended as a prophylactic regimen for asthma, is known to inhibit both allergic and nonallergic inflammatory processes in which an essential role for T cells has been implicated. Therefore the direct effects of this drug on several aspects of T-cell activity were analyzed in the present study. By using murine lymphocytes we found that NS at concentrations of 10(-8) to 10(-6) mol/L inhibited the mitogen- or antigen-induced proliferative responses of these cells. It is interesting to note that higher concentrations were ineffective. Preincubation of immune lymph node cells from contact sensitized mice with the drug abrogated their ability to transfer contact sensitivity to naive recipients, an effect that was found to be specific for the treated cells. Nedocromil sodium also interfered with the mitogen-induced interleukin-2 and tumor necrosis factor production by T cells and with their ability to adhere to the bound protein components of the extracellular matrix laminin and fibronectin. All these effects may be attributed to the inhibition of the increase of cytosolic calcium, which accompanies the early phase of T-cell activation and which is an essential step in inducing the aforementioned phenomena. 相似文献
8.
Privatisation has been part of Israeli housing policy since the first public housing units were built in 1949. It has involved the sale of publicly‐owned dwellings to sitting tenants, but also the shift to residents of responsibilities usually associated with ownership, such as maintenance and tax liabilities. The evolution of this policy is examined by considering the social, economic and political factors which have shaped the development of Israeli public housing policy from its beginning. 相似文献
9.
Mark Shneider Hanna Dodiuk Reshef Tenne Shmuel Kenig 《Polymer Engineering and Science》2013,53(12):2624-2632
Closed‐cage (fullerene‐like) nanoparticles (NPs) of WS2 are currently produced in large amounts and were investigated as additives to thermoplastics and thermosetting polymers. The nanoinduced morphology and the resulting enhanced fracture toughness of epoxy/WS2 nanocomposites were studied. The morphology of the epoxy nanocomposites was induced by controlled WS2 surface chemistry. The WS2 NPs used were either untreated or chemically treated with acryloxy, which is compatible, and alkyl silane, which is incompatible, respectively, with the epoxy matrix. In the case where the acryloxy silane was used to treat the WS2 particles, good dispersion and compatibility were obtained in the epoxy resin. Moreover, a distinct nodular morphology was induced on fracture as a result of nucleation by the compatible NPs. In the case where the alkyl silane treatment was used cavitation morphology was induced, following mechanical loading, which is the result of incompatibility with the epoxy resin. The fracture toughness results showed an increase of 70% for nanocomposites contains alkyl‐treated WS2 compared with the neat epoxy. Modeling of the nodular morphology enabled the determination of optimal concentration of the WS2 in epoxy (0.3% by weight). Two main fracture mechanisms were observed, crack bowing around the nodular boundaries in the case of compatibility between the nanoparticle and the epoxy and particle‐induced cavitation in the case of incompatibility, respectively. These results are of significant importance both for epoxy‐based adhesives and fiber composites. POLYM. ENG. SCI., 53:2624–2632, 2013. © 2013 Society of Plastics Engineers 相似文献
10.
Inna Wiesel Hamutal Arbel Ana Albu-Yaron Ronit Popovitz-Biro Jeffrey M. Gordon Daniel Feuermann Reshef Tenne 《Nano Research》2009,2(5):416-424
Inorganic fullerene-like WS2 and MoS2 nanoparticles have been synthesized using exclusively solid precursors, by reaction of the corresponding metal oxide nanopowder,
sulfur and a hydrogen-releasing agent (NaBH4 or LiAlH4), achieved either by conventional furnace heating up to ∼900 °C or by photothermal ablation at far higher temperatures driven
by highly concentrated white light. In contrast to the established syntheses that require toxic and hazardous gases, working
solely with solid precursors permits relatively safer reactor conditions conducive to industrial scale-up.
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