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1.
The tetrametallic ruthenium-oxo-hydroxo-hydride complex {[(PCy(3))(CO)RuH](4)(mu(4)-O)(mu(3)-OH)(mu(2)-OH)} (1) was synthesized in two steps from the monomeric complex (PCy(3))(CO)RuHCl (2). The tetrameric complex 1 was found to be a highly effective catalyst for the transfer dehydrogenation of alcohols. Complex 1 showed a different catalytic activity pattern towards primary and secondary benzyl alcohols, as indicated by the Hammett correlation for the oxidation reaction of p-X-C(6)H(4)CH(2)OH (rho = -0.45) and p-X-C(6)H(4)CH(OH)CH(3) (rho = +0.22) (X = OMe, CH(3), H, Cl, CF(3)). Both a sigmoidal curve from the plot of initial rate vs [PhCH(OH)CH(3)] (K(0.5) = 0.34 M; Hill coefficient, n = 4.2+/-0.1) and the phosphine inhibition kinetics revealed the highly cooperative nature of the complex for the oxidation of secondary alcohols. 相似文献
2.
Indicating that CBMC does not satisfy the monotonic property in terms of the number of interactions, Xu and Zhou proposed an augmented definition of CBMC by adopting cut set instead of glue methods. The augmented CBMC clearly satisfies the monotonic property. However, CBMC is designed to overcome the problem with respect to the number of interactions and, therefore, focuses on the interaction pattern, especially, member connectivity. Consequently, it does not make sense to mention the monotonic property of CBMC with respect to interaction number. Moreover, the notion of glue methods allows several interpretations on the design quality of a class. However, that meaningful interpretation is not possible for the augmented definition due to the removal of the notion of glue methods. Copyright © 2001 John Wiley & Sons, Ltd. 相似文献
3.
Considering the robustness, stability and reduced volume of data, researchers have focused on using edge information in various
video processing applications including moving object detection, tracking and target recognition. Though the edge information
is more robust compared to intensity, it also exhibits variations in different frames due to illumination change and noise.
In addition to this, the amount of variation varies from edge to edge. Thus, without making use of this variability information,
it is difficult to obtain an optimal performance during edge matching. However, traditional edge pixel-based methods do not
keep structural information of edges and thus they are not suitable to extract and hold this variability information. To achieve
this, we represent edges as segments that make use of the structural and relational information of edges to allow extraction
of this variability information. During edge matching, existing algorithms do not handle the size, positional and rotational
variations to deal with edges of arbitrary shapes. In this paper, we propose a knowledge-based flexible edge matching algorithm
where knowledge is obtained from the statistics on the environmental dynamics, and flexibility is to deal with the arbitrary
shape and the geometric variations of edges by making use of this knowledge. In this paper, we detailed the effectiveness
of the proposed matching algorithm in moving object detection and also indicated its suitability in other applications like
target detection and tracking. 相似文献
4.
Young-Hyun Baek Jin-Ho Lee Sang-Jin Chang Yuri Chae Myung-Hun Lee Sun-Hong Kim Kwon-Il Han Tack-Joong Kim 《International journal of molecular sciences》2022,23(10)
Minoxidil is the most widely used treatment for hair growth, but has been associated with several side effects. In this study, we investigated the effects of heat-killed Enterococcus faecalis EF-2001 on hair loss prevention and regrowth using human dermal papilla cells and male C57BL/6 mice. To examine the effects of EF-2001, we used minoxidil as the positive control. In the in vitro experiments, EF-2001 treatment (75–500 μg/mL) led to the proliferation of human dermal papilla cells in a concentration-dependent manner. In the in vivo experiment, the topical application of 200 µL EF-2001 on the dorsal surface of C57BL/6 male mice led to hair growth. Changes in hair regrowth were examined by visual comparison and hematoxylin and eosin staining of skin sections. We also determined the expression levels of marker genes (Wnt) and growth factors (fibroblast growth factor, insulin growth factor 1, and vascular endothelial growth factor) in the skin tissues of the back of each mouse using a quantitative polymerase chain reaction. EF-2001 accelerated the progression of hair regrowth in mice and promoted hair-follicle conversion from telogen to anagen, likely by increasing the expression levels of growth factors and marker genes. 相似文献
5.
Syadaruddin Syachrani Hyung Seok Jeong Vajra Rai Myung Jin Chae Tom Iseley 《Tunnelling and Underground Space Technology incorporating Trenchless Technology Research》2010,25(6):681-688
Proper functioning of culverts is not only critical to protecting the transportation system from flooding but also critical to maintaining the expected service life of the overall transportation system. During the service life of culverts, they deteriorate due to many reasons such as corrosion caused by road salt, blockage by debris and sediment, poor construction techniques, etc. Trenchless technologies have been used by several State Departments of Transportation (DOTs) to rehabilitate deteriorated drainage structures without disrupting the traffic and within a relatively short span of time. These technologies provide many benefits in terms of cost, time, quality, and expected service life. However, the safety aspects of these techniques have not been discussed and documented in detail probably due to the complexity and the lack of safety standards and specifications directly associated with the techniques. This paper discusses the application of a risk assessment framework to assess potential safety issues of currently available trenchless technologies for culvert rehabilitation. The findings of the study will provide additional information to improve the decision making process in selecting and planning culvert rehabilitation projects. 相似文献
6.
In this letter, we propose a novel design scheme for an optimal non‐uniform planar array geometry in view of maximum side‐lobe reduction. This is implemented by a thinned array using a genetic algorithm. We show that the proposed method can maintain a low side‐lobe level without pattern distortion during beam steering. 相似文献
7.
8.
Hong Chae Woo 《Electronics letters》1998,34(13):1300-1301
The performance of a stochastic gradient adaptive filter can be significantly improved by introducing a forgetting factor. The complexity of the original algorithm can also be reduced by using only the signs of error signals and input signals in the gradient adaptive step size computation 相似文献
9.
Joonho Lim Kipaek Kwon Soo-Ik Chae 《Electronics letters》1998,34(4):344-346
The authors propose a reversible energy recovery logic (RERL) circuit for ultra-low-energy consumption, which consumes only adiabatic energy loss and leakage current loss by completely eliminating non-adiabatic energy loss. It is a dual-rail adiabatic circuit using the concept of reversible logic with a new eight-phase clocking scheme. Simulation results show that at low-speed operation, the RERL consumes much less energy than the complementary static CMOS circuit and other adiabatic logic circuits 相似文献
10.
Effect of surface modification of anode with surfactant on the performance of microbial fuel cell 下载免费PDF全文
Young‐Chae Song Dae‐Sup Kim Jung‐Hui Woo Bakthavachallam Subha Seong‐Ho Jang Subpiramaniyam Sivakumar 《国际能源研究杂志》2015,39(6):860-868
Surface modification of anode using surfactant has great influence on the electrical performance of a microbial fuel cell (MFC). In this study, the effect of surface‐modified exfoliated graphite used for anode fabrication on a cube‐type MFC batch reactor was examined. The surface exfoliated graphite was modified with 5‐mM anionic surfactant, sodium dodecyl sulfate. Anaerobic sludge used as inoculum containing 70% (v/v) of artificial wastewater and 30% (v/v) of seed sludge in an anode chamber and air cathode was used in cathode side. Anode modification was explored as an approach to enhance the start‐up and improve the performance of the reactor. Scanning electron microscopy was used to evaluate the morphology and activity of electrochemically active bacteria. In the study, the start‐up time of MFC required to approach stable voltage was substantially reduced, and the maximum stable voltage was higher than the control. In addition, the activation resistance of the MFC was considerably reduced, and the maximum power density (1640 mW/m2) was 20% higher than control. However, when the surface of exfoliated graphite was modified with over 10‐mM anionic surfactant, some negative effects on start‐up time, activation resistance and maximum power density were observed. This modification also enhanced the bacterial attachment and biofilm formation on the modified anode surface. The result suggested that surface modification anode with surfactant is effective for electrical responses achieved in the MFC. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献