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1.
The use and impacts of accelerated weathering of limestone (AWL; reaction: CO2+H2O+CaCO3→Ca2++2(HCO3−) is explored as a CO2 capture and sequestration method. It is shown that significant limestone resources are relatively close to a majority of CO2-emitting power plants along the coastal US, a favored siting location for AWL. Waste fines, representing more than 20% of current US crushed limestone production (>109 tonnes/yr), could provide an inexpensive or free source of AWL carbonate. With limestone transportation then as the dominant cost variable, CO2 mitigation costs of $3-$4/tonne appear to be possible in certain locations. Perhaps 10–20% of US point–source CO2 emissions could be mitigated in this fashion. It is experimentally shown that CO2 sequestration rates of 10−6 to 10−5 moles/sec per m2 of limestone surface area are achievable, with reaction densities on the order of 10−2 tonnes CO2 m−3day−1, highly dependent on limestone particle size, solution turbulence and flow, and CO2 concentration. Modeling shows that AWL would allow carbon storage in the ocean with significantly reduced impacts to seawater pH relative to direct CO2 disposal into the atmosphere or sea. The addition of AWL-derived alkalinity to the ocean may itself be beneficial for marine biota. 相似文献
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3.
Chang?Duk?Kang Sang?Jun?SimEmail author Young?Sang?Cho Woo?Sik?Kim 《Korean Journal of Chemical Engineering》2003,20(3):482-486
The removal of copper from wastewater by ferric/limestone coagulation followed by screen filtration was carried out at a laboratory
scale. The optimum coagulant (FeCl3) dose and working pH were 50 mg// of Fe(m) and pH 7.5, respectively, through jar tests. For the efficient removal of copper
from wastewater, we developed a novel process including the co-precipitation of copper with FeCl3, alkalization in a limestone aeration bed, and separation of precipitates in a sedimentation tank coupled with internal stainless
steel screen filter. The performance results showed that removal of copper from the solution was over 99.5%. The pH was effectively
maintained over 7.5 in limestone bed during the whole process. Ferric hydroxide/copper aggregates were removed over 99% by
stainless steel screen filter of 1,450 mesh. Periodic air backwashing alleviated fouling of the filter surface. 相似文献
4.
Rheology of cementitious paste with silica fume or limestone 总被引:1,自引:0,他引:1
The rheological behaviour of cementitious pastes where cement has increasingly been replaced by densified silica fume (SF), untreated SF or limestone has been studied. The effect of SF on the flow resistance, taken as the area under the flow curve, was found to depend on the dispersing ability of the plasticizer as illustrated by pastes with naphtalene sulphonate-formaldehyde condensate (SNF) and polyether grafted polyacrylate (PA).The gel strengths increased with increasing SF replacement of cement independently of plasticizer type. The cementitious gel strength was, however, depending on the type of SF since pastes with densified SF developed lower gel strengths than pastes with untreated SF. This phenomenon was attributed to agglomerates in the densified SF which remained unbroken by the mixing and measurement sequence.Both flow resistance and gel strength decreased with increasing limestone replacement. Thus, silica fume may have an advantage over limestone filler as stabilizing agent for self-compacting concrete preventing segregation upon standing and reduced form pressure due to a more rapid gel formation. 相似文献
5.
This work is the fourth part of an overall project the aim of which was the development of general mix design rules for concrete containing different kinds of mineral admixtures. The two first parts presented the separation and quantification, by means of an empirical model based on semi-adiabatic calorimetry measurements, of the different physical effects responsible for changes in cement hydration (short terms) when chemically inert quartz powders were used in mortars. Part three dealt with an intensive experimental program, presenting and commenting more than 2000 compressive strength measurements. This program concerned 1 day to 6 months old mortars containing up to 75% of inert and pozzolanic admixtures. All these compressive strength results are analyzed in this fourth part and the influence of three effects, namely dilution, heterogeneous nucleation and the pozzolanic effect, are discriminated and quantitatively evaluated. An efficiency concept is proposed in order to take into account the effect of mineral admixture in mortars from both the physical and chemical points of view. It uses an efficiency function ξ(p) that has notable properties: it is independent of time, independent of fineness and independent of the type of mineral admixture. 相似文献
6.
《矿业科学技术学报(英文版)》2017,27(3):423-430
The main purpose of current study is development of an intelligent model for estimation of shear wave velocity in limestone. Shear wave velocity is one of the most important rock dynamic parameters.Because rocks have complicated structure, direct determination of this parameter takes time, spends expenditure and requires accuracy. On the other hand, there are no precise equations for indirect determination of it; most of them are empirical. By using data sets of several dams of Iran and neuro-genetic,adaptive neuro-fuzzy inference system(ANFIS), and gene expression programming(GEP) methods, models are rendered for prediction of shear wave velocity in limestone. Totally, 516 sets of data has been used for modeling. From these data sets, 413 ones have been utilized for building the intelligent model, and 103 have been used for their performance evaluation. Compressional wave velocity(V_ p), density(γ)and porosity(n), were considered as input parameters. Respectively, the amount of R for neuro-genetic and ANFIS networks was 0.959 and 0.963. In addition, by using GEP, three equations are obtained; the best of them has 0.958 R. ANFIS shows the best prediction results, whereas GEP indicates proper equations. Because these equations have accuracy, they could be used for prediction of shear wave velocity for limestone in the future. 相似文献
7.
《矿业科学技术学报(英文版)》2016,26(1):149-154
Photogrammetry, as a tool for monitoring underground mine deformation, is an alternative to traditional point measurement devices, and may be capable of accurate measurements in situations where technologies such as laser scanning are unsuited, undesired, or cost-prohibitive. An underground limestone mine in Ohio is used as a test case for monitoring of structurally unstable pillars. Seven pillars were photographed over in a 63 day period, punctuated by four visits. Using photogrammetry, point clouds of the mine geometry were obtained and triangulation surfaces were generated to determine volumes of change over time. Pillar spalling in the range of 0.29–4.03 m3 of rock on individual rib faces was detected. Isolated incidents of rock expansion prior to failure, and the isolated failure of a weak shale band were also observed. Much of the pillars remained unchanged during the monitoring period, which is indicative of proper alignment in the triangulated surfaces. The photographs of some ribs were of either too poor quality or had insufficient overlap, and were not included. However, photogrammetry was successfully applied to multiple ribs in quantifying the pillar geometry change over time. 相似文献
8.
High volume fly ash (HVFA) concrete mixtures are being considered more frequently due to their cost and sustainability advantages. While the long term performance of these HVFA concretes typically meets or exceeds that of conventional concretes, their early age performance is often characterized by excessive retardation of the hydration reactions, delayed setting times, and low strengths. Extending an HVFA mixture to a ternary blend that incorporates a fine limestone powder may provide a viable solution to these deficiencies, particularly the hydration retardation and setting issues. In this paper, a nano-limestone powder and two other limestone fillers of increasing median particle size (4.4 μm and 16.4 μm) are investigated for their propensity to accelerate early age reactions and reduce setting times in a Class C fly ash/cement blend. The fineness of the limestone has measurable effects on its efficacy in accelerating hydration and decreasing setting times. Companion specimens prepared with a fine silica powder suggest that the fine limestone may act favorably through both a physical and a chemical mechanism. Isothermal calorimetry and Vicat needle penetration measurements on pastes are accompanied by strength measurements on mortars, to verify that the limestone powder substitutions are not negatively impacting strength development. A linear relationship with a reasonable correlation is found to exist between 1 d and 7 d compressive strengths of mortars and their accompanying cumulative heat release values as determined using isothermal calorimetry. 相似文献
9.
石灰石资源的开发利用 总被引:1,自引:0,他引:1
本文比较系统地介绍了我国优势资源石灰石的性质,一般用途和矿床的工业要求,列举了主要产品17种;简述了10种(类)钙盐产品的工业生产方法,并绘出了工艺流程示意图;对当前石灰石利用前景和可能开发方向提出了参考建议,可供石灰石储量丰富地区有关企业和当地政府在规划开发资源时作参考。 相似文献
10.
The O2/CO2 coal combustion technology is an innovative combustion technology that can control CO2, SO2 and NOx emissions simultaneously. Calcination and sintering characteristics of limestone under O2/CO2 atmosphere were investigated in this paper. The pore size, the specific pore volume and the specific surface area of CaO calcined were measured by N2 adsorption method. The grain size of CaO calcined was determined by XRD analysis. The specific pore volume and the specific surface area of CaO calcined in O2/CO2 atmosphere are less than that of CaO calcined in air at the same temperature. And the pore diameter of CaO calcined in O2/CO2 atmosphere is larger than that in air. The specific pore volume and the specific surface area of CaO calcined in O2/CO2 atmosphere increase initially with temperature, and then decline as temperature exceeds 1000 °C. The peaks of the specific pore volume and the specific surface area appear at 1000 °C. The specific surface area decreases with increase in the grain size of CaO calcined. The correlations of the grain size with the specific surface area and the specific pore volume can be expressed as L = 744.67 + 464.64 lg(1 / S) and L = − 608.5 + 1342.42 lg(1 / ε), respectively. Sintering has influence on the pore structure of CaO calcined by means of influencing the grain size of CaO. 相似文献