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排序方式: 共有4167条查询结果,搜索用时 140 毫秒
1.
《International Journal of Hydrogen Energy》2022,47(79):33765-33780
This work investigates selective Ni locations over Ni/CeZrOx–Al2O3 catalysts at different Ni loading contents and their influences on reaction pathways in ethanol steam reforming (ESR). Depending on the Ni loading contents, the added Ni selectively interacts with CeZrOx–Al2O3, resulting in the stepwise locations of Ni over CeZrOx–Al2O3. This behavior induces a remarkable difference in hydrogen production and coke formation in ESR. The selective interaction between Ni and CeZrOx for 10-wt.% Ni generates more oxygen vacancies in the CeZrOx lattice. The Ni sites near the oxygen vacancies enhance reforming via steam activation, resulting in the highest hydrogen production rate of 1863.0 μmol/gcat·min. In contrast, for 15 and 20-wt.% Ni, excessive Ni is additionally deposited on Al2O3 after the saturation of Ni–CeZrOx interactions. These Ni sites on Al2O3 accelerate coking from the ethylene produced on the acidic sites, resulting in a high coke amount of 19.1 mgc/gcat·h (20Ni/CZ-Al). 相似文献
2.
《International Journal of Hydrogen Energy》2022,47(2):1306-1318
The effective and efficient utilization of low-calorific value (LCV) gases has gained increasing attention in scientific research and industrial fields. In this study, the combustion characteristics of three LCV gases in practical devices are analyzed by using a nonadiabatic perfectly stirred reactor model. The complete steady-state solution in the temperature-residence time parameter space is obtained with arc-length continuation. The stable operation region is quantified by the eigenvalue analysis. The transition of solution curves is quantified with heat loss coefficient. Five key system parameters are systematically investigated on their effects on stability limits. With the combustion performance being quantified by a combustion state index, a combustion state regulation method is proposed to find the optimal regulation path of system parameters. Active subspace method is further applied to shorten the regulation step by identifying the active direction. The proposed method and findings are useful for optimal regulation of burning LCV gases in industrial burners. 相似文献
3.
《International Journal of Hydrogen Energy》2022,47(48):20999-21012
Micro-combustor is a portable power device that can provide energy efficiently, heat recirculating is considered to be an important factor affecting the combustion process. For enhancing the heat recirculating and improving the combustion stability, we proposed a heat-recirculating micro-combustor embedded with porous media, and the numerical simulation was carried out by CFD software. In this paper, the effect of porous media materials, thickness and inlet conditions (equivalence ratio, inlet velocity) on the temperature distribution and exhaust species in the micro combustor are investigated. The results showed that compared with the micro combustor without embedded porous media (MCNPM), micro-combustor embedded with porous media (MCEPM) can improve the temperature uniformity distribution in the radial direction and strengthen the preheating capacity. However, it is found that the embedding thickness of porous media should be reasonably arranged. Setting the thickness of porous media to 15 mm, the combustor can obtain excellent comprehensive capacity of steady combustion and heat recirculating. Compared the thermal performance of Al2O3, SiC, and ZrO2 porous media materials, indicating that SiC due to its strong thermal conductivity, its combustion stabilization and heat recirculating capacity are obviously better than that of Al2O3 and ZrO2. With the porous media embedded in the micro combustor, the combustion has a tempering limit of more than 10 m/s, and the flame is blown out of the porous media area over 100 m/s. The reasonable equivalence ratio of CH4/air combustion should be controlled within the range of 0.1–0.5, and “super-enthalpy combustion” can be realized. 相似文献
4.
根据延迟焦化装置露天栈桥的工程设计实践,围绕一炉两塔(一个加热炉两个焦炭塔)的焦化装置,分析了露天栈桥设计中的要点及难点,对其在平面布置、基础安排和吊车梁选型等设计方面做一些介绍和论述。 相似文献
5.
对菱镁矿在固体燃料燃烧过程中的固硫特性进行了理论研究,所得结论对进一步将菱镁矿作为固体燃料燃烧过程中的固硫剂具有非常重要的意义。 相似文献
6.
杨承志 《自动化与仪器仪表》1994,(4):38-41
本文论述了对小型工业炉窑燃烧过程进行智能控制的一种设计思想。该控制器用智能PID调节器控制炉温作为主控回路,用自寻最优控制空燃比作为副控回路。是一种既满足燃烧过程多目标要求,又造价低廉的智能控制器。 相似文献
7.
Seong-Ku Kim Joon Kyu Lee Yong-Mo Kim Jae-Hyun Ahn 《Journal of Mechanical Science and Technology》2002,16(7):1009-1018
The Representative Interactive Flamelet (RIF) concept has been applied to numerically simulate the combustion processes and
pollutant formation in the direct injection diesel engine. Due to the ability for interactively describing the transient behaviors
of local flame structures with CFD solver, the RIF concept has the capabilities to predict the auto-ignition and subsequent
flame propagation in the diesel engine combustion chamber as well as to effectively account for the detailed mechanisms of
soot formation, NOX formation including thermal NO path, prompt and nitrous NOX formation, and reburning process. Special emphasis is given to the turbulent combustion model which properly accounts for
vaporization effects on the mixture fraction fluctuations and the pdf model. The results of numerical modeling using the RIF
concept are compared with experimental data and with numerical results of the commonly applied procedure which the low-temperature
and high-temperature oxidation processes are represented by the Shell ignition model and the eddy dissipation model, respectively.
Numerical results indicate that the RIF approach including the vaporization effect on turbulent spray combustion process successfully
predicts the ignition delay time and location as well as the pollutant formation. 相似文献
8.
S. ReppA. Sadiki C. SchneiderA. Hinz T. LandenfeldJ. Janicka 《International Journal of Heat and Mass Transfer》2002,45(6):1271-1285
This work aims to compare numerical results obtained by using the Monte Carlo composition-PDF method and a presumed-β-PDF in order to reveal their effects on the prediction of flow and scalar fields in swirling confined methane diffusion flame. Using the intrinsic low dimensional manifolds method for modelling the chemistry and a second moment closure for the turbulence, it is shown that both PDF-methods provide a similar accuracy level of the prediction of mean quantities. While the presumed-β-PDF performs using reasonable computational efforts, the Monte Carlo-PDF allows to capture well the turbulence-chemistry interaction and strong finite-chemistry effects such as local extinction. 相似文献
9.
10.
针对梅山自产焦炭,利用梅山焦炭反应性试验设备,通过改变焦炭块数、CO2流量和温度等控制参数,讨论了这些参数对焦炭反应性和反应后强度检测值的影响,以及保证测定可靠性应采取的控制措施。 相似文献