全文获取类型
收费全文 | 3922篇 |
免费 | 507篇 |
国内免费 | 262篇 |
专业分类
电工技术 | 305篇 |
综合类 | 291篇 |
化学工业 | 1003篇 |
金属工艺 | 202篇 |
机械仪表 | 21篇 |
建筑科学 | 263篇 |
矿业工程 | 184篇 |
能源动力 | 143篇 |
轻工业 | 698篇 |
水利工程 | 665篇 |
石油天然气 | 328篇 |
武器工业 | 6篇 |
无线电 | 107篇 |
一般工业技术 | 179篇 |
冶金工业 | 210篇 |
原子能技术 | 22篇 |
自动化技术 | 64篇 |
出版年
2024年 | 16篇 |
2023年 | 88篇 |
2022年 | 151篇 |
2021年 | 158篇 |
2020年 | 146篇 |
2019年 | 127篇 |
2018年 | 113篇 |
2017年 | 148篇 |
2016年 | 146篇 |
2015年 | 166篇 |
2014年 | 232篇 |
2013年 | 253篇 |
2012年 | 315篇 |
2011年 | 287篇 |
2010年 | 176篇 |
2009年 | 220篇 |
2008年 | 166篇 |
2007年 | 245篇 |
2006年 | 226篇 |
2005年 | 212篇 |
2004年 | 175篇 |
2003年 | 169篇 |
2002年 | 134篇 |
2001年 | 119篇 |
2000年 | 102篇 |
1999年 | 68篇 |
1998年 | 59篇 |
1997年 | 43篇 |
1996年 | 44篇 |
1995年 | 31篇 |
1994年 | 21篇 |
1993年 | 15篇 |
1992年 | 14篇 |
1991年 | 12篇 |
1990年 | 18篇 |
1989年 | 12篇 |
1988年 | 5篇 |
1987年 | 11篇 |
1986年 | 9篇 |
1985年 | 12篇 |
1984年 | 12篇 |
1983年 | 6篇 |
1982年 | 5篇 |
1981年 | 1篇 |
1976年 | 1篇 |
1951年 | 2篇 |
排序方式: 共有4691条查询结果,搜索用时 15 毫秒
1.
Shingo Urata Hiroyuki Hijiya Kazuhiko Niwano Jun Matsui 《Journal of the American Ceramic Society》2022,105(6):4200-4207
To theoretically explore amorphous materials with a sufficiently low dielectric loss, which are essential for next-generation communication devices, the applicability of a nonequilibrium molecular dynamics simulation employing an external alternating electric field was examined using alkaline silicate glass models. In this method, the dielectric loss is directly evaluated as the phase shift of the dipole moment from the applied electric field. This method enabled us to evaluate the dielectric loss in a wide frequency range from 1 GHz to 10 THz. It was observed that the dielectric loss reaches its maximum at a few THz. The simulation method was found to qualitatively reproduce the effects of alkaline content and alkaline type on the dielectric loss. Furthermore, it reasonably reproduced the effect of mixed alkalines on the dielectric loss, which was observed in our experiments on sodium and/or potassium silicate glasses. Alkaline mixing was thus found to reduce the dielectric loss. 相似文献
2.
Wenshu Chen Jiajun Gu Yongping Du Fang Song Fanxing Bu Jinghan Li Yang Yuan Ruichun Luo Qinglei Liu Di Zhang 《Advanced functional materials》2020,30(25)
Large‐scale production of hydrogen from water‐alkali electrolyzers is impeded by the sluggish kinetics of hydrogen evolution reaction (HER) electrocatalysts. The hybridization of an acid‐active HER catalyst with a cocatalyst at the nanoscale helps boost HER kinetics in alkaline media. Here, it is demonstrated that 1T–MoS2 nanosheet edges (instead of basal planes) decorated by metal hydroxides form highly active / heterostructures, which significantly enhance HER performance in alkaline media. Featured with rich / sites, the fabricated 1T–MoS2 QS/Ni(OH)2 hybrid (quantum sized 1T–MoS2 sheets decorated with Ni(OH)2 via interface engineering) only requires overpotentials of 57 and 112 mV to drive HER current densities of 10 and 100 mA cm?2, respectively, and has a low Tafel slope of 30 mV dec?1 in 1 m KOH. So far, this is the best performance for MoS2‐based electrocatalysts and the 1T–MoS2 QS/Ni(OH)2 hybrid is among the best‐performing non‐Pt alkaline HER electrocatalysts known. The HER process is durable for 100 h at current densities up to 500 mA cm?2. This work not only provides an active, cost‐effective, and robust alkaline HER electrocatalyst, but also demonstrates a design strategy for preparing high‐performance catalysts based on edge‐rich 2D quantum sheets for other catalytic reactions. 相似文献
3.
Bioremediation by alkaline protease (AkP) from edible mushroom Termitomyces clypeatus: optimization approach based on statistical design and characterization for diverse applications
下载免费PDF全文
![点击此处可从《Journal of chemical technology and biotechnology (Oxford, Oxfordshire : 1986)》网站下载免费的PDF全文](/ch/ext_images/free.gif)
4.
5.
6.
Robben J.; der Schueren J.Van; Verhasselt P.; Aert R.; Volckaert G. 《Protein engineering, design & selection : PEDS》1995,8(2):159-165
The deletion of nine residues from the C-terminus of the bacterialchloramphenicol acetyltransferase (CAT) results in depositionof the mutant protein in cytoplasmic inclusion bodies and lossof chloramphenicol resistance in Escherichia coli. This foldingdefect is relieved by C-terminal fusion of the polypeptide withas few as two residues. Based on these observations, efficientpositive selection for the cloning of DNA fragments has beendemonstrated. The cloning vector encodes a C-terminally truncatedCAT protein. Restriction sites in front of the stop codon allowthe insertion of target DNA, resulting in the production ofproperly folded CAT fusion proteins and regained chloramphenicolresistance. The positive selection of recombinants is accomplishedby growth of transformants on chloramphenicol-containing agarplates. The method appears particularly convenient for the cloningof DNA fragments amplified by the PCR because minimal informationto restore CAT folding can be included in the primers. The cloningof random sequences shows that the folding defect can be relievedby fusion to a wide variety of peptides, providing great flexibilityto the positive selection system. This vector may also contributeto the determination of the role of the C-terminus in CAT folding. 相似文献
7.
Angela M. Zapata-Anzola Carlos A. Rivera-Rondón Jhon Ch. Donato-Rondón 《Lakes & Reservoirs: Research and Management》2006,11(1):29-38
Guatavita Lake is a small, sheltered tropical high mountain lake located in the Colombian Andes, with a closed watershed and a maximum depth of 25 m. It is the freshwater source for human consumption in nearby small towns, as well as being a site of cultural value for the country, as it was a sacred place to indigenous peoples until about five centuries ago. As the structure and function of this aquatic ecosystem is poorly understood, this study provides initial knowledge on its phytoplankton biomass dynamics, which should be useful in designing efficient management plans with environmental baseline information for similar lakes elsewhere. Physical and chemical data, and photosynthetic pigment concentrations, were measured for the period November 1999–November 2000 at the central vertical axis of Guatavita Lake. The vertical profile of the chlorophyll‐a concentration was closely related to the dissolved inorganic nitrogen concentrations and the thermal stratification characteristics. The maximum chlorophyll‐a concentration in the metalimnion was recorded for the thermal stratification period (November 1999–June 2000). Deepening of the maximum chlorophyll‐a concentration began in February, continuing to June, when it reached its lowest value at the 15 m depth. The phytoplankton biomass values showed an increment within the entire water column at the beginning of the mixing period (July). The relation between the metalimnetic peak of chlorophyll‐a and the dissolved inorganic nitrogen concentration suggests the growth of the phytoplankton community is limited mainly by the availability of nitrogen. 相似文献
8.
Kinema is a fermented soya bean food of Nepal and the hilly regions of North-eastern States of India. Generally, the fermentation is dominated by Bacillus spp. that often cause alkalinity and desirable stickiness in the product. The present study was undertaken in a limited number of commercial (market) kinema samples to test for the presence of foodborne pathogens and their properties. Bacillus cereus was present in numbers exceeding 104 cfu/g product in five of the tested 15 market samples. Enterobacteriaceae and coliform bacteria exceeded 105 cfu/g in 10 of the 15 samples. Escherichia coli exceeding 105 cfu/g was found in two samples. Staphylococcus aureus was not detected in any of the tested samples. Of 31 isolated typical and atypical strains of B. cereus, 18 representative strains were tested qualitatively for the ability to produce diarrhoeal type enterotoxin (BCET) using an Oxoid BCET-RPLA test kit. Overall, BCET was formed by 12 strains in BHIG (brain heart infusion broth +1% glucose), by seven strains on sterilized cooked rice, and by five strains on sterilized cooked soya beans. Semi-quantitative tests on BCET revealed that levels exceeding 256 ng/g soya beans, produced by single pure culture inoculation with the isolated B. cereus strains, were reduced to ≤ 8 ng/g by frying kinema in oil, a common procedure when making kinema curry. It was also shown in a mixed pure culture experiment that a kinema strain B. Subtilis DK-W1, is able to suppress growth and BCET formation by a selected toxin producing strain (BC7-5) of B. cereus. It is concluded that the traditional way of making kinema and its culinary use in curries is safe. However, for novel applications of kinema, safety precautions are advisable. 相似文献
9.
Lake-Level Change and Water Balance Analysis at Lake Qinghai,West China during Recent Decades 总被引:7,自引:0,他引:7
Xiao-Yan Li He-Ye Xu Yong-Liang Sun Deng-Shan Zhang Zhi-Peng Yang 《Water Resources Management》2007,21(9):1505-1516
Lake Qinghai, the largest saline lake with an area of 4,260 km2 (2000) and average depth of 21 m (1985) in West China, has experienced severe decline in water level in recent decades. This
study aimed to investigate water balance of the lake and identify the causes for the decline in lake level. There was a 3.35-m
decline in water level with an average decreasing rate of 8.0 cm year−1 between 1959 and 2000. The lake water balance showed that mean annual precipitation between 1959 and 2000 over the lake was
357 ± 10 mm, evaporation was 924 ± 10 mm, surface runoff water inflow was 348 ± 21 mm, groundwater inflow was 138 mm ± 9 and
the change in lake level was −80 ± 31 mm. The variation of lake level was highly positively correlated to surface runoff and
precipitation and negatively to evaporation, the correlation coefficients were 0.89, 0.81 and −0.66, respectively. Water consumption
by human activities accounts for 1% of the evaporation loss of the lake, implying that water consumption by human activities
has little effect on lake level decline. Most dramatic decline in lake level occurred in the warm and dry years, and moderate
decline in the cold and dry years, and relatively slight decline in the warm and wet years, therefore, the trend of cold/warm
and dry climate in recent decades may be the main reasons for the decline in lake level. 相似文献
10.
RM Martín‐Aranda E Ortega‐Cantero ML Rojas‐Cervantes MA Vicente‐Rodríguez MA Baares‐Muoz 《Journal of chemical technology and biotechnology (Oxford, Oxfordshire : 1986)》2005,80(2):234-238
α,β‐Unsaturated nitriles have been synthesized by Knoevenagel condensation of a carbonylic compound with malononitrile, assisted by sonochemical irradiation. Two alkaline‐promoted clays (Li+‐ and Cs+‐exchanged saponites) have been employed as catalysts. The influence of the carbonylic compound (benzaldehyde or cyclohexanone) and the use of a solvent on the catalytic activity have been studied. Remarkable increase in the conversion values has been found when the reaction is activated by ultrasound, as compared with the thermal activation. In this green, solvent‐free procedure, α,β‐unsaturated nitriles have been produced in very high yields (97%) when the Cs+‐saponite is used as catalyst. Copyright © 2004 Society of Chemical Industry 相似文献