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1.
《International Journal of Hydrogen Energy》2022,47(12):7836-7845
Catalyst samples for CH4 decomposition were prepared from red mud (RM) by an acid-leaching neutralization precipitation approach. Water-washing the resultant precipitates multiple times, followed by drying at 105 °C and calcination at 500 °C, resulted in a threshold of residual Na2O, equivalent to 96% Na2O removal. Drying the precipitate at a higher temperature of 200 °C, followed by repeated water washing, provided a deeper Na2O removal of 99% and made the resultant samples more active for the targeted reaction. Subsequently, four catalyst samples with a simulated red mud composition and NaOH contents from 0 to 0.3 wt% were prepared and the catalytic test results revealed that the Na2O remaining in the RM-derived catalysts did not only inhibit their activation in CH4 but also lower their maximal activities for CH4 decomposition. Finally, two catalysts with the same simulated red mud composition and their Na impregnated respectively on Fe2O3 and a mixture support of Al2O3-SiO2-TiO2 were prepared and tested to explore the effect of Na distribution on the activation behavior of RM-derived catalysts for CH4 decomposition. The activity testing results showed that it was the Na residual dispersed on iron oxides in the RM-derived samples to significantly inhibit the activation of CH4 decomposition. 相似文献
2.
Qian Wu Xiangmei Liu Bo Li Lei Tan Yong Han Zhaoyang Li Yanqin Liang Zhenduo Cui Shengli Zhu Shuilin Wu Yufeng Zheng 《材料科学技术学报》2021,67(8):70-79
Pathogens pose a serious challenge to environmental sanitation and a threat to public health.The frequent use of chemicals for sterilization in recent years has not only caused secondary damage to the environment but also increased pathogen resistance to drugs,which further threatens public health.To address this issue,the use of non-chemical antibacterial means has become a new trend for environmental disinfection.In this study,we developed red phosphorus nanoparticles(RPNPs),a safe and degradable photosensitive material with good photocatalytic and photothermal properties.The red phosphorus nanoparticles were prepared using a template method and ultrasonication.Under the irradiation of simulated sunlight for 20 min,the RPNPs exhibited an efficiency of 99.98%in killing Staphylococcus aureus due to their excellent photocatalytic and photothermal abilities.Transmission electron microscopy and ultraviolet–visible spectroscopy revealed that the RPNPs exhibited degradability within eight weeks.Both the RPNPs and their degradation products were nontoxic to fibroblast cells.Therefore,such RPNPs are expected to be used as a new type of low-cost,efficient,degradable,biocompatible,and eco-friendly photosensitive material for environmental disinfection. 相似文献
3.
《Ceramics International》2022,48(13):18793-18802
The luminescence center energy transfer, crystal field strength, and covalency are limited by the crystal structure of the host and subsequently affect the luminescence efficiency, color, and intensity. Here, we report an excellent red phosphor BaLaLiWO6:0.40Eu3+ and the dependence between symmetry and luminous performance. A model for changing symmetry is drawn by analyzing the Coulomb potential and structure for the application of a double-perovskite phosphor BLLWO: Dy3+, Eu3+ in white light LEDs. The addition of Dy3+/Eu3+ makes the W-O bond formed by the B-site and oxygen ion longer and the Li-O bond shorter, and the difference between the eight octahedral around the A-site is reduced, increasing the symmetry of the A-site. Local symmetry was successfully modulated by changing the Eu3+ concentration to control the Y/B ratio of Dy3+ and the R/O ratio of Eu3+ and smoothly achieved (0.382, 0.373) warm white light color coordinate. The phosphor has excellent thermal stability and still has 92.3% intensity at 475 K. The above results show that the wavelength composition of the luminescence is tunable by changing the symmetry of the environment in which the doped ions are located. It applies to single hosts for the regulation of white light emission. 相似文献
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实验室质量体系的建立与运行 总被引:2,自引:0,他引:2
详细论述了质量和质量体系的基本概念、建立质量体系的必要性、质量体系的构成和建立过程、质量体系文件的编制、质量体系的运行和持续改进以及中国实验室国家认可委员会的有关政策。 相似文献
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交互控制是计算机程序的重要功能 ,也是实现人—机对话的基本途径。VisualBasic编程语言以其易学习掌握、开发灵活的特点而成为目前流行的程序开发工具 ,本文以VisualBasic语言为例介绍了交互控制程序编程方法 ,并对具体的每一种方法编写了相应的示例。 相似文献
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数据采集与监控软件Genie 总被引:2,自引:0,他引:2
Genie是具有国际先进水平的数据采集与监控软件,它提供了一个面向对象的图形化用户界面,因此简化了数据采集过程、控制应用程序开发和操作员界面。本文介绍了Genie的特点、功能、基本用途以及VISUALBA-SIC在设计这类监控软件中的作用。 相似文献
10.
分析了大亚湾核电站18个月换料对流体系统可能产生的影响,根据改进后的燃料管理策略以及相关参数变化,遵照系统设计准则的要求。对14个流体系统的容量和能力进行了计算和论证。论证结果表明,大亚湾核电站现有系统基本满足18个月换料的需求 相似文献