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The unique lateral confinement of a swelling polymer network leads to surface wrinkles that define a multitude of surface structures, including microlens arrays (background). The versatility of this approach, which is reported on p. 3238 by Crosby and Chan, allows for the realization of a variety of functional devices on both planar and nonplanar surfaces, such as synthetic compound lens structures (see inset). 相似文献
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D. Kisailus M. Najarian J.C. Weaver D.E. Morse 《Advanced materials (Deerfield Beach, Fla.)》2005,17(10)
A system that acts as a biomimetic of the silica‐synthesizing enzyme found in a marine sponge is reported by Morse and co‐workers on p. 1234. Gold nanoparticles (GNPs) are functionalized with the same organic moieties that are found in the enzyme's catalytic site. Interaction between the nucleophilic (OH‐terminated) and hydrogen‐bonding (imidazole‐terminated) GNPs, as shown on the cover, is required for the hydrolysis of a silicon alkoxide precursor and subsequent polycondensation to form silica at a low temperature and near‐neutral pH. Replacement of either of the required functional groups by a non‐reactive methyl group abolishes catalysis in this synthetic system, as it does in the biological enzyme. Cover art provided by Peter Allen. 相似文献
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