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1.
NO2 fission is regarded to be the most important initial decomposition process of 2,4,6,8,10,12-hexanitro-2,4,6,8,10,12-hexaazaisowurtzitane (CL-20). In this study, four CL-20 conformers based on the ε-CL-20 were obtained after the optimization at m062x/cc-pvtz level, and the bond length, bond order and bond dissociation energy of the N-N bonds were examined to investigate the stability of these bonds. In addition, the rate constants and activation energy of the NO2 fission were evaluated using the microcanonical variational transition state theory (μVT). The calculation results have shown that N-N bonds in the case of pseudo-equatorial and axial of nitro groups are the most stable and the least stable, respectively, by evaluating the bond length, bond order and minimum energy path (MEP). The NO2 fission rate constants are affected by not only the stability of N-N bonds but also the repulsion forces from the other nitro groups, and the fission process for pseudo-equatorial positioning of nitro groups is easier to be accelerated due to the increase of the repulsion forces. The decomposition of CL-20 conformer may mainly originate from the fission of the pseudo-equatorial positioning of nitro groups, especially for CL-20 III conformer because of the significant low activation energy. 相似文献
2.
C Brito L Niklitschek L H Molina I Molina 《International Journal of Dairy Technology》2002,55(1):32-39
This study was performed to obtain an adequate tool for predicting the yield of Chilean Gouda cheese. The theoretical yields were calculated by applying equations derived from technical references to industrial cheese production and were compared with their own actual yields, thus selecting those equations showing the best correlation with the actual yield.
The manufacturing and ripening of the cheese were controlled through the chemical composition of milk, whey and cheese, and the weight of the product before and after ripening was recorded.
The actual and theoretical yield values derived from each formula were compared using the mean yield graphs. Furthermore, the global concordance coefficient ( W ) of Kendall and Smith was also applied, showing the lack of significant discrepancy between actual and theoretical yield values [ P > 0.01 ( W = 27; W ≥ 18.48)] for either 3- or 30-day cheeses. Out of the 11 formulae used to measure the yield of cheese, six showing a good correlation between the yields were selected through the comparison of error sums and Pearson correlation analysis. However, two formulae showed the best yield results for practical use. 相似文献
The manufacturing and ripening of the cheese were controlled through the chemical composition of milk, whey and cheese, and the weight of the product before and after ripening was recorded.
The actual and theoretical yield values derived from each formula were compared using the mean yield graphs. Furthermore, the global concordance coefficient ( W ) of Kendall and Smith was also applied, showing the lack of significant discrepancy between actual and theoretical yield values [ P > 0.01 ( W = 27; W ≥ 18.48)] for either 3- or 30-day cheeses. Out of the 11 formulae used to measure the yield of cheese, six showing a good correlation between the yields were selected through the comparison of error sums and Pearson correlation analysis. However, two formulae showed the best yield results for practical use. 相似文献
3.
Wallace Manheiemr 《Journal of Fusion Energy》2006,25(3-4):121-139
As apparent from the title, this author feels that civilization faces a real threat, one which will become obvious and serious within the lifetimes of many readers of this article. This threat is not global warming, but lack of affordable energy. We take for granted turning on a light, or adjusting our thermostats in winter or summer, or filling our cars gas tank; and lose sight of the fact that there are huge and complicated industrial systems which make this possible. But as we run out of petroleum and natural gas, and worry about the environmental and climatic effects of burning coal on the required scale, how can this continue? This paper makes the case that breeding nuclear fuel, by both fusion and fission, is the only way our civilization as we know it, can continue beyond the next half century or so. 相似文献
4.
Results from long-term field experiments in south-western Australia are presented in the form of relationships between yield, expressed as a percentage of the maximum yield, and soil test for phosphorus (P) values. Maximum yields were not always indicated by well defined yield plateaux. Different methods have been used to estimate the maximum yield value which is used to calculate yield as a percentage of the maximum yield so as to remove interseasonal variation. For all of these methods and for the same site, the same P fertilizer (superphosphate), and the same plant species, the relationship between yield and soil test P differed for different years. Consequently fertilizer recommendations based on the assumption that this relationship is constant are likely to be incorrect. We therefore question the validity of the common practice in soil testing programmes of using percentage yield values to remove interseasonal variation. 相似文献
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6.
应用磷灰石裂变径迹研究大民屯凹陷的古地温 总被引:4,自引:0,他引:4
为深刻认识辽河盆地古地温特征,利用裂变径迹分析方法,对大民屯凹陷钻井岩心中19块磷灰石样品的裂变径迹年龄和长度做了测试。结果表明,随井深增加,径迹年龄和平均径迹长度有减少、变短的显著趋势,ES3^4地层磷灰石裂变径迹表观年龄比地层年龄年轻得多,说明沉积后曾长时间处于退火带中,退火带古地温为74~130℃,有效加热时间为4l~45Ma,2300~4000m深度地层处于退火过渡带。将径迹长度分布特征与地史、热史模拟结果相结合,认为该区在ES4段末经历一次短时间迅速增温后,ES3^1亚段存在一个区域抬升降温的热事件过程,其后地层稳定下降,沉降幅度小、沉积物较薄,温度增加缓慢,古地温梯度高于今地温梯度,对生、排烃较为有利。 相似文献
7.
本文着重于辐射作用于物质最初生成的产物,包括激发态的离子与分子,能量超过热能的次级电子等的反应以及电荷和激发能的转移,并试图论述它们的最新发展。 相似文献
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9.
Benjamin F. Myers 《Journal of the American Ceramic Society》1992,75(3):686-693
The hydrolysis of uranium oxycarbide (UCO) was studied by injecting water vapor into a fuel element containing a known number of high-temperature, gas-cooled reactor (HTGR) coated particles with exposed fuel kernels. The experiments were conducted in the High Flux Isotope Reactor (HFIR) at temperatures between 700° and 1000°C, a system pressure of 200 kPa, and partial pressures of water vapor between 21 and 199 Pa. The general sequential response of the exposed fuel kernels to water vapor addition consisted of (1) a rapid release of stored fission gas with a concomitant increase in the steady-state release and (2) a period of constant steady-state release. Upon cessation of the addition of water vapor, a decline in the release to prehydrolysis values generally occurred. The release of stored fission gas was dependent on the square of the partial pressure of water vapor. The ratio of the constant steady-state release to the prehydrolysis value was independent of the partial pressure of water vapor. The time constant for the decline in the release was the same in all of the hydrolysis tests. 相似文献
10.
研究了热中子反应堆屏蔽准确性优化设计问题.由于传统的反应堆屏蔽计算并未考虑引发裂变的中子对裂变能谱的影响,使得燃耗加深时仿真计算结果与实际情况差别较大.针对上述问题,提出从与入射中子能量相关的Maxwell谱出发,对入射中子的能量进行分群,构造出矩阵谱,然后确定了仿真计算中对裂变中子能量的抽样步骤,并在中子输运计算软件MCNP程序上进行了仿真计算.结果表明,根据矩阵谱计算得到的结果能够反映出燃耗变化对屏蔽计算的影响,能够为反应堆屏蔽设计提供更为准确的依据. 相似文献