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1.
Wenjia Jing Baoqiang Hou Jinxiao Wang Qiang Zhi Jianfeng Yang Bo Wang 《Journal of the American Ceramic Society》2022,105(5):3141-3146
Photocatalysts often show excellent performances on the basis of their surface state of exposed faces with high reactivity, but unfortunately surfaces of this type are usually concealed into the interior of crystals for their high surface energy. We report here a possibility that for fluorine-terminated surfaces of monoclinic ZrO2, these higher-energy surfaces could be retained and exposed. Urchin-like ZrO2 hollow microspheres (UZHS) composed of nanoribbons with exposed (010) facets are obtained through a fluoride mediately solvothermal method. We prove the stabilization effect of fluorine adsorption on (010) facets by density functional theory calculations. More interestingly, UZHS exhibit tunable photocatalytic selectivity in dye degradation. The fluorinated UZHS exhibit good performances both on decomposing Congo red (CR) and methylene blue, while the surface-modified UZHS by calcination only favor decomposition of CR. 相似文献
2.
《Food Control》2015
This study aims to assess the degree of HACCP implementation in small business butcher shops and understand which factors most influence butchers' intention to fully implement it, through the application of the Theory of Planned Behaviour. One hundred and one butchers managing or owning small butcher's responded to the interview regarding their Attitudes, Subjective Norm, Perceived Behavioural Control, Personal Norm, and Knowledge with regard to their Intention to fully implement a HACCP system in their shops. Before the interviews, a certified veterinarian visited all the shops. Visits included an inspection of the establishments using the Official Portuguese Control Plan checklist for meat retailers. Conformance level measured past performance regarding food safety practices. Based on past performance, butchers were divided into “high performers” and “low performers”. “High performers” yielded high values of Attitude and Intention towards the Behaviour. For these, Attitude and Personal Norm emerge as predictors of the Intention to fully implement a HACCP system. For “low performers”, Personal Norm was the strongest predictor of Intention, with results pointing to the need for an intervention from the authorities to promote increased conformance to food safety practices. For both groups, neither Social Norm nor Perceived Behavioural Control acted as significant predictors of Intention. 相似文献
3.
论文在对现有一类典型图像混沌加密算法的分析基础上,提出了一种改进的图像混沌加密算法。该算法引入小波变换,可以有效地克服一些混沌加密算法不能抵御已知/选择明文攻击的缺陷。 相似文献
4.
论文将Fermat素性检验的思想运用于不可约多项式的判断,给出了一个对于不可约判断问题的Monte Carlo 算法,分析了该算法的计算复杂度问题,并且给出了次数在200以内的检验结果。 相似文献
5.
Recently, in our laboratory a closed form expression for the correlation function of the hard-sphere dimer fluid obtained
from Wertheims multidensity Ornstein-Zernike integral equation theory with Percus-Yevick approximation was presented by Kim
et al. [2001]. However, it is difficult to apply its expression to perturbation theory and vapor-liquid equilibria calculations,
since it is of very complex form. In this work, we present a simplified expression for the first shell of the radial distribution
function (RDF) of the hard-sphere dimer fluid using a series expansion of the analytical expression. The expansion is carried
out in terms of both the packing fraction and the radial distance. Expressions are also obtained for the coordination number
and its first and second derivatives as functions of radial distance and packing fraction. These expressions, which are useful
in perturbation theory, are simpler to use than those obtained from the starting equation, while giving good agreement with
the original expression results. Then we present an simplified equation of state for the square-well dimer fluid of variable
well width (λ) based on Barker-Henderson perturbation theory using its expression for the radial distribution function of
the hard-sphere dimer fluid, and test its expression with NVT and Gibbs ensemble Monte Carlo simulation data [Kim et al.,
2001]. 相似文献
6.
A revision algorithm is a learning algorithm that identifies the target concept, starting from an initial concept. Such an algorithm is considered efficient if its complexity (in terms of the resource one is interested in) is polynomial in the syntactic distance between the initial and the target concept, but only polylogarithmic in the number of variables in the universe. We give an efficient revision algorithm in the model of learning with equivalence and membership queries for threshold functions, and some negative results showing, for instance, that threshold functions cannot be revised efficiently from either type of query alone. The algorithms work in a general revision model where both deletion and addition type revision operators are allowed. 相似文献
7.
This paper presents a mechanism which infers a user's plans from his/her utterances by directing the inference process towards the more likely interpretations of a speaker's statements among many possible interpretations. Our mechanism uses Bayesian theory of probability to assess the likelihood of an interpretation, and it complements this assessment by taking into consideration two aspects of an interpretation: its coherence and its information content. The coherence of an interpretation is determined by the relationships between the different statements in the discourse. The information content of an interpretation is a measure of how well defined the interpretation is in terms of the actions to be performed on the basis of this interpretation. This measure is used to guide the inference process towards interpretations with higher information content. The information content of an interpretation depends on the specificity and the certainty of the inferences in it, where the certainty of an inference depends on the knowledge on which the inference is based. Our mechanism has been developed for use in task-oriented consultation systems. The particular domain that we have chosen for exploration is that of travel booking. 相似文献
8.
批评是理论与实践的重要中介。建筑批评变革的普遍要求反映了人们对批评现状的不满和对批评中理论建设的呼声。批评的理论化和理论的批评化是探索这种理论建设的一条重要途径,它为我们重建思想的能力提供了可能性。 相似文献
9.
Consistent calculation of fugacities of fluid mixtures remains as one of the most important subjects in contemporary molecular
thermodynamics. In practice, equations of state (EOSs) and gE-models have been used. However, most EOSs are erroneous for condensed phases at high densities and gE-models are inapplicable for pressuresensitive systems. Recently to remedy the shortcomings in both approaches, there has
been a surge of new gE-EOS mixing rules. By equating any set of EOS and gE-models, the limitations in both approaches could be resolved significantly. However, the self-consistency in the underlying
concept of those mixing rules remains controversial. During the last several years, the present authors proposed a new lattice-fluid
EOS and its simplification relevant to phase equilibrium calculations. Without employing any gE-EOS mixing rule and with only two parameters for a pure component and one adjustable interaction energy parameter for a binary
mixture, results obtained to date demonstrated that the EOSs are quantitatively applicable to a great variety of phase equilibrium
properties of mixtures, especially, for complex and/or macromolecular systems. In the present article we summarize the EOSs
and extended the applications to liquid-liquid Equilibria. In part I, we discussed briefly the molecular thermodynamic aspects
of general derivation of the EOS and a brief discussion of applying the EOSs to pure fluids while the illustrative application
to various real mixture systems is discussed in part II. 相似文献
10.
相似理论在真空灭弧室研究和设计中的应用 总被引:1,自引:1,他引:0
本文应用相似理论得出,真空灭弧室中电弧运动速度与电流强度成线性关系的相似准则,和极限开断电流与触头直径、开距间的经验公式。认为用小电流模型来研究大电流真空灭弧室是可行的。 相似文献