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Direct numerical simulation of hydrogen-enriched lean premixed methane-air flames
Authors:Evatt R Hawkes  Jacqueline H Chen
Affiliation:Reacting Flow Research Department, Combustion Research Facility, Sandia National Laboratories, P.O. Box 969 MS 9051, Livermore, CA 94551-0969, USA
Abstract:The effect of hydrogen blending on lean premixed methane-air flames is studied with the direct numerical simulation (DNS) approach coupled with a reduced chemical mechanism. Two flames are compared with respect to stability and pollutant formation characteristics—one a pure methane flame close to the lean limit, and one enriched with hydrogen. The stability of the flame is quantified in terms of the turbulent flame speed. A higher speed is observed for the hydrogen-enriched flame consistent with extended blow-off stability limits found in measurements. The greater flame speed is the result of a combination of higher laminar flame speed, enhanced area generation, and greater burning rate per unit area. Preferential diffusion of hydrogen coupled with shorter flame time scales accounts for the enhanced flame surface area. In particular, the enriched flame is less diffusive-thermally stable and more resistant to quenching than the pure methane flame, resulting in a greater flame area generation. The burning rate per unit area correlates strongly with curvature as a result of preferential diffusion effects focusing fuel at positive cusps. Lower CO emissions per unit fuel consumption are observed for the enriched flame, consistent with experimental data. CO production is greatest in regions which undergo significant downstream interaction. In these regions, the enriched flame exhibits faster oxidation rates as a result of higher levels of OH concentration. NO emissions are increased for the enriched flame as a result of locally higher temperature and radical concentrations found in cusp regions.
Keywords:Lean premixed combustion   Hydrogen   Methane   Direct numerical simulation
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