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Reduced graphene oxide–coated anode gas diffusion layer for performance enhancement of proton‐exchange membrane fuel cell
Authors:Yi‐Chen Lin  Hao‐Hsiang Chang  Du‐Cheng Tsai  Rong‐Hsin Huang  Fuh‐Sheng Shieu
Affiliation:1. Department of Materials Science and Engineering, National Chung Hsing University, Taichung, Taiwan, Republic of China;2. Innovation and Development Center of Sustainable Agriculture (IDCSA), National Chung Hsing University, Taichung, Taiwan, Republic of China;3. Fuh‐Sheng Shieu, Department of Materials Science and Engineering, National Chung Hsing University, Taichung 40227, Taiwan, Republic of China.
Abstract:In this study, we produced reduced graphene oxide (RGO) by reduction of graphene oxide (GO) in Teflon‐lined autoclave, maintained at 100°C for 12 hours, and coated on the anode gas diffusion layer (GDL) of a proton‐exchange membrane fuel cell (PEMFC) to improve the cell performance. Fourier transform infrared spectroscopy and X‐ray photoelectron spectroscopy analysis showed the presence of residual oxygen‐containing functional groups in RGO. Field‐emission scanning electron microscopy images revealed the uniform and adequate coating of the GDLs with RGO. The wettability of RGO‐coated GDL was determined by the sessile drop method and has optimum contact angle 117°. The power densities for the membrane electrode assembly (MEA) with RGO coated on the anode GDL were 30.92%, 41%, and 36.20% higher than those for the MEA without the RGO coating at anode gas humidified temperatures of 25°C, 45°C, and 65°C, respectively.
Keywords:anode gas diffusion layer  proton‐exchange membrane fuel cell  reduced graphene oxide
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