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PTFE间歇聚合反应过程变周期动态经济优化控制
引用本文:王雪松,曾祥宇,薄翠梅,汤舒淇,董超,李俊,张泉灵,金晓明,叶胜利.PTFE间歇聚合反应过程变周期动态经济优化控制[J].化工学报,1951,73(9):3973-3982.
作者姓名:王雪松  曾祥宇  薄翠梅  汤舒淇  董超  李俊  张泉灵  金晓明  叶胜利
作者单位:1.南京工业大学电气工程与控制科学学院,江苏 南京 211816;2.南京工业大学智能制造研究院,江苏 南京 211816;3.浙江大学控制科学与工程学院,浙江 杭州 310027;4.东华工程科技股份有限公司,安徽 合肥 230041
基金项目:国家重点研发计划项目(2019YFB1705800);国家自然科学基金项目(62173178)
摘    要:聚四氟乙烯(PTFE)间歇聚合生产模式可满足小批量、多用途以及高质量产品的市场需求。针对PTFE聚合过程存在强非线性和大时滞特性,提出了一种基于自由终端的动态经济优化控制方法。首先,将生产周期作为一个自由度纳入优化变量建立动态经济优化问题,采用改进控制变量参数化方法,控制输入被离散为可变长度的片状序列,便可将动态经济优化问题转换为非线性规划(NLP)问题;然后,采用基于梯度下降的内点罚函数法求解NLP问题,通过变周期预测时域的滚动优化控制方法优化控制输入和终端时间;最后将提出的变周期动态经济优化控制与传统PI控制、非线性模型预测控制进行对比测试分析,仿真结果表明本方法单位经济效益更高,生产周期更短,突显了间歇生产的灵活性。

关 键 词:聚四氟乙烯  间歇聚合反应  自由终端  经济优化控制  动态实时优化  
收稿时间:2022-03-29

Dynamic economic optimal control for PTFE batch polymerization process with free terminal
Xuesong WANG,Xiangyu ZENG,Cuimei BO,Shuqi TANG,Chao DONG,Jun LI,Quanling ZHANG,Xiaoming JIN,Shengli YE.Dynamic economic optimal control for PTFE batch polymerization process with free terminal[J].Journal of Chemical Industry and Engineering(China),1951,73(9):3973-3982.
Authors:Xuesong WANG  Xiangyu ZENG  Cuimei BO  Shuqi TANG  Chao DONG  Jun LI  Quanling ZHANG  Xiaoming JIN  Shengli YE
Affiliation:1.College of Electrical Engineering and Control Science, Nanjing Tech University, Nanjing 211816, Jiangsu, China;2.Institute of Intelligent Manufacturing, Nanjing Tech University, Nanjing 211816, Jiangsu, China;3.College of Control Science and Engineering, Zhejiang University, Hangzhou 310027, Zhejiang, China;4.East China Engineering Science and Technology Co. , Ltd. , Hefei 230041, Anhui, China
Abstract:Polytetrafluoroethylene (PTFE) batch polymerization production mode can meet the market demand of small batch, multi-purpose and high quality products. Aiming at the strong nonlinearity and large time delay in the PTFE polymerization process, a dynamic economic optimization control method based on free terminal is proposed in this paper. Firstly, the dynamic economic optimization problem is established by integrating the production cycle as a degree of freedom into the optimization variable. The control inputs are discretized into piece-wise sequences by using improved control variable parameterization method, and the dynamic economic optimization problem can be transformed into a nonlinear programming (NLP) problem. Then, the NLP problem is solved based on the penalty function method of gradient descent, and the rolling optimization control method in the free prediction time domain is used to optimize the control input and terminal time. Finally, compared with PI control and nonlinear model predictive control, the simulation results show that free terminal dynamic economic optimization control method has higher economic benefit and shorter production cycle, which highlights the flexibility of batch production.
Keywords:PTFE  batch polymerization  free terminal  economic optimization control  dynamic real-time optimization  
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