Development and characterisation of polylactic acid–gliadin bilayer/trilayer films as carriers of thymol |
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| Authors: | Jun‐You Zhu Chuan‐He Tang Shou‐Wei Yin Xiao‐Quan Yang |
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| Affiliation: | 1. Research and Development Center of Food Proteins, Guangdong Province Key Laboratory for Green Processing of Natural Products and Product Safety, South China University of Technology, Guangzhou, China;2. State Key Laboratory of Pulp and Paper Engineering, South China University of Technology, Guangzhou, China |
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| Abstract: | Biodegradable food packaging promises a more sustainable future. Poly(lactic acid) (PLA) is a promising alternative for petroleum‐derived polymers. However, PLA films suffer from poor barrier properties compared with petroleum‐derived ones. To address this issue, we designed bilayer and sandwich‐architectured trilayer films based on PLA and gliadin. We reported firstly the direct formation of PLA–gliadin bilayer/trilayer films without surface modification on PLA film. The films were compact and uniform, and double/triple layers were combined firmly, preventing delamination. This strategy enhanced mechanical resistance, ductility and moisture barrier of gliadin films and concomitantly enhanced the oxygen barrier for PLA films. Thymol loadings endowed bilayer/trilayer films with antimicrobial activity and antioxidant activity. The antimicrobial activity of the films depended on film types, and gliadin layer presented larger inhibition zone than PLA layer, hinting that the films possessed directional releasing role. This study opens a promising route to fabricate bilayer/trilayer architecture helping to create synergism of the biopolymers. |
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| Keywords: | Antimicrobial films antioxidant films bilayer/trilayer films gliadin polylactic acid thymol |
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