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CONTROL OF MOLECULAR WEIGHT IN A BATCH POLYMERIZATION REACTOR USING LONG-RANGE PREDICTIVE CONTROL METHODS
Authors:C. Kiparissides   E. Sidiropoulou  S. Voutetakis  C. Frousakis
Affiliation: a Department of Chemical Engineering, Chemical Process Engineering Research Institute Aristotle University of Thessaloniki, Thessaloniki, Greece
Abstract:Recently two powerful control algorithms, namely, dynamic matrix control (DMC) and extended self-tuning regulator (ESTR), have been advocated for the design of robust industrial controllers. The present paper demonstrates the application of DMC and ESTR algorithms to a bulk methyl methacrylate batch polymerization reactor operating under strong diffusional limitations of termination and propagation reactions. A realistic mathematical model is employed to simulate the strong nonlinear, time-varying dynamics of the polymerization process. The general control objective is to maintain the monomer conversion and number-average molecular weight along some desired state trajectories despite the presence of process disturbances in the total initiator concentration. It is shown that both controllers can satisfactorily control the monomer conversion and number-average molecular weight by manipulating the polymerization temperature. The similarities and the main operating features of the two controllers are examined and their closed-loop performance is directly compared to the performance of a conventional linear quadratic controller (LQC). Finally the effects of DMC and ESTR tuning parameters on the calculated control action are investigated.
Keywords:Control  Predictive  Batch reactor  Polymerization
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