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Green Synthesis of Hierarchically Porous Carbon Nanotubes as Advanced Materials for High‐Efficient Energy Storage
Authors:Jian‐Gan Wang  Hongzhen Liu  Xingyuan Zhang  Xu Li  Xingrui Liu  Feiyu Kang
Affiliation:1. State Key Laboratory of Solidification Processing, Center for Nano Energy Materials, School of Materials Science and Engineering, Northwestern Polytechnical University and Shaanxi Joint Lab of Graphene (NPU), Xi'an, China;2. Engineering Laboratory for Functionalized Carbon Materials and Shenzhen Key Laboratory for Graphene‐based Materials, Graduate School at Shenzhen, Tsinghua University, Shenzhen, China
Abstract:Hierarchically porous carbon nanomaterials with well‐defined architecture can afford a promising platform for effectively addressing energy and environmental concerns. Herein, a totally green and straightforward synthesis strategy for the fabrication of hierarchically porous carbon nanotubes (HPCNTs) by a simple carbonization treatment without any assistance of soft/hard templates and activation procedures is demonstrated. A high specific surface area of 1419 m2 g?1 and hierarchical micro‐/meso‐/macroporosity can be achieved for the HPCNTs. The unique porous architecture enables the HPCNTs serving as excellent electrode/host materials for high‐performance supercapacitors and Li–sulfur batteries. The design strategy may pave a new avenue for the rational synthesis of hierarchically porous carbon nanostructures for high‐efficient energy storage applications.
Keywords:green synthesis  high performance  Li–  S batteries  porous carbon nanotubes  supercapacitors
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