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旋转填料床中硝酸吸收NO_x的实验研究(英文)
引用本文:李裕,刘有智,张路遥,苏强,金国良.旋转填料床中硝酸吸收NO_x的实验研究(英文)[J].中国化学工程学报,2010,18(2):244-248.
作者姓名:李裕  刘有智  张路遥  苏强  金国良
作者单位:1. Research Center of Shanxi Province for High Gravity Engineering and Technology, Institute of Chemical Engineering and Environment, North University of China, Taiyuan 030051, China;2. Gansu Yinguang Chemical Group Co., Ltd., Baiyin 730900, China
基金项目:Supported by the Fund of Science and Technology of Shanxi for Young Scholars(2007021012);Research Project of Shanxi Provincial Science and Technology Department(20090321113)
摘    要:Absorption of NOx into nitric acid solutions was studied in the presence of ozone by using a rotating packed bed (RPB) contactor. The influences of operating parameters, such as high gravity number, amount of ozone, gas velocity, liquid spray density and inlet concentration of NOx, on the removal efficiency of NOx were investigated, among which the high gravity number and ozone amount are more important. Ozone was introduced to oxidize HNO2 to HNO3 to prevent the decomposition of HNO2 in the liquid phase. The high gravity number presents the effective external force for enhancing the mass transfer of ozone from gas phase to liquid phase. Under the experimental condition, the removal efficiency of NOx is higher than 90% and the concentration of nitric acid product exceeds 45%.

关 键 词:nitrogen  oxides  rotating  packed  bed  ozone  oxidation  absorption  
收稿时间:2009-6-19
修稿时间:2009-6-19  

Absorption of NOx into nitric acid solution in rotating packed bed
LI Yu,LIU Youzhi,ZHANG Luyao,SU Qiang,JIN Guoliang.Absorption of NOx into nitric acid solution in rotating packed bed[J].Chinese Journal of Chemical Engineering,2010,18(2):244-248.
Authors:LI Yu  LIU Youzhi  ZHANG Luyao  SU Qiang  JIN Guoliang
Affiliation:1. Research Center of Shanxi Province for High Gravity Engineering and Technology, Institute of Chemical Engineering and Environment, North University of China, Taiyuan 030051, China;2. Gansu Yinguang Chemical Group Co., Ltd., Baiyin 730900, China
Abstract:Absorption of NOx into nitric acid solutions was studied in the presence of ozone by using a rotating packed bed(RPB)contactor.The influences of operating parameters,such as high gravity number,amount of ozone,gas velocity,liquid spray density and inlet concentration of NOx,on the removal efficiency of NOx were investi gated,among which the high gravity number and ozone amount are more important.Ozone was introduced to oxidize HNO2 to HNO3 to prevent the decomposition of HNO2 in the liquid phasc.The high gravity number presents the effective external force for enhancing the mass transfer of ozone from gas phase to liquid phase.Under the ex perimental condition,the removal efficiency of NOx is higher than 90% and the concentration of nitric acid product exceeds 45%.
Keywords:nitrogen oxides  rotating packed bed  ozone oxidation  absorption
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