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深圳大鹏半岛沿岸海水中~(129)I的分布特征和来源
引用本文:张鸿,陈应飞,侯小琳,孙慧斌,卢勇宏,张路远.深圳大鹏半岛沿岸海水中~(129)I的分布特征和来源[J].深圳大学学报(理工版),2012,29(1):1-6.
作者姓名:张鸿  陈应飞  侯小琳  孙慧斌  卢勇宏  张路远
作者单位:1. 深圳大学物理科学与技术学院,深圳,518060
2. 西安加速器质谱中心和黄土与第四纪地质国家重点实验室,西安,710075
3. 深圳大学物理科学与技术学院,深圳518060西安,710075
4. 深圳大学化学与化工学院,深圳,518060
基金项目:国家自然科学基金资助项目
摘    要:研究核电站运行时产生并可能向周边海洋环境排放的长寿命放射性核素碘-129(129I)对生态环境的影响,应用超热中子活化分析和加速器质谱分析深圳大亚湾核电基地所处大鹏半岛沿岸海水样品中127I的质量浓度和129I的原子浓度.结果显示,核电站排水渠附近海水中129I的原子浓度(370.9×106/L),以及129I和127I原子浓度比(37.4×10-10)最大,但在5 km外的海域,即被稀释至本底量级水平,表明核电站对周边海洋环境中129I的影响甚微.该区域海水中129I仍主要来源于大气层核试验和核燃料后处理厂释放导致的全球大气放射性落尘,其目前水平对人体的辐照风险尚可忽略.

关 键 词:核安全  放射性污染监测  海洋环境  碘-129  (129I)  129I与127I原子浓度比  超热中子活化分析  加速器质谱  大亚湾核电站

The distribution and source apportionment of 129I in coastal seawater of Shenzhen Dapeng Peninsula
ZHANG Hong , CHEN Ying-fei , HOU Xiao-lin , SUN Hui-bin , LU Yong-hong , ZHANG Lu-yuan.The distribution and source apportionment of 129I in coastal seawater of Shenzhen Dapeng Peninsula[J].Journal of Shenzhen University(Science &engineering),2012,29(1):1-6.
Authors:ZHANG Hong  CHEN Ying-fei  HOU Xiao-lin  SUN Hui-bin  LU Yong-hong  ZHANG Lu-yuan
Affiliation:1)College of Physics Science and Technology,Shenzhen University,Shenzhen 518060,P.R.China 2) Xi’an AMS Center and State Key Laboratory of Loess and Quaternary Geology,Xi’an 710075,P.R.China 3) College of Chemistry and Chemical Engineering,Shenzhen University,Shenzhen 518060,P.R.China
Abstract:For exploring the radioactively ecological impact on the surrounding ocean environment caused by the long-lived radionuclide iodine-129(129I),which is generated and may be discharged into the environment during the operation process of Guangdong Daya Bay nuclear power station and Ling Ao nuclear power station,epithermal neutron activation analysis and accelerator mass spectrometry have been utilized to analyze the concentrations of 127I and 129I in the seawater samples along Dapeng Peninsula,where Daya Bay Nuclear Power base is located.The results show that the concentration of 129I(370.9×106/L) and the N(129I)/N(127I) ratio(37.4×10-10) reach maximum in the seawater near the drain of nuclear power station,whereas both of them decrease to the radiation background level in the area 5 km away,indicating that the impac of 129I from the nuclear power plant on surrounding ocean environment is little.In this sea area 129I mainly comes from the global fallout released by the atmospheric nuclear tests and nuclear fuel reprocessing plants.The radioactive risk to the human body at its current level can be ignored.
Keywords:nuclear safety  radioactive pollution monitoring  ocean environment  iodine-129(129I)  N(129I)/N(127I)  epithermal neutron activation analysis  accelerator mass spectrometer  Daya Bay nuclear power station
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