Further insights into thermoelectric properties of nonstoichiometric titanium oxide fabricated by high pressure and high temperature |
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Authors: | Haiqiang Liu Hongan Ma Fei Wang Binwu Liu Baomin Liu Jiaxiang Chen Xiaopeng Jia |
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Affiliation: | State Key Laboratory of Superhard Materials, College of Physics, Jilin University, Changchun 130012, China |
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Abstract: | The present work explores the feasibility of advancing the thermoelectric properties of nonstoichiometric TiO2?x through introducing more and more oxygen deficiencies. Compared with previous work, it is found that this compositional manipulation induces phase transition; in addition, the scattering mechanisms of both carrier and phonon have changed, resulting in the temperature-independent electrical resistivity, inferior electrical performance and an unexpected high thermal conductivity. As a consequence, a moderate zT value of 0.13 is obtained in TiO1.72 at 600?℃. Through this work, we understand deeply about thermoelectric properties of nonstoichiometric titanium oxide by high pressure and high temperature, and further investigations about this system have been directed. |
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Keywords: | Titanium oxide Thermoelectric properties High pressure High temperature |
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